
1.The Organic Photonics and Electronics Group, UmeåUniversity, Umeå, Sweden
2.LunaLEC AB, Umeå, Sweden
3.Future Industries Institute, University of South Australia, Mawson Lakes, SA 5095, Australia
L Edman, Email: ludvig.edman@umu.se
Published:2016-06,
Published Online:25 November 2015,
Received:21 August 2015,
Revised:21 November 2015,
Accepted:22 November 2015
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Lindh, E. M. et al. Luminescent line art by direct-write patterning. Light: Science & Applications, 5, e16050 (2016).
Lindh, E. M. et al. Luminescent line art by direct-write patterning. Light: Science & Applications, 5, e16050 (2016). DOI: 10.1038/lsa.2016.50.
We present a direct-write patterning method for the realization of electroluminescent (EL) line art using a surface-emissive light-emitting electrochemical cell with its electrolyte and EL material separated into a bilayer structure. The line-art emission is achieved through subtractive patterning of the electrolyte layer with a stylus
and the single-step patterning can be either manual for personalization and uniqueness or automated for high throughput and repeatability. We demonstrate that the light emission is effectuated by cation-assisted electron injection in the patterned regions and that the resulting emissive lines can be as narrow as a few micrometers. The versatility of the method is demonstrated through the attainment of a wide range of light-emission patterns and colors using a variety of different materials. We propose that this low-voltage-driven and easy-to-modify luminescent line-art technology could be of interest for emerging applications
such as active packaging and personalized gadgets.
direct-write patterninglight-emitting electrochemical cellluminescent line artorganic electronics
Sandström A, Edman L. Towards high-throughput coating and printing of light-emitting electrochemical cells: a review and cost analysis of current and future methods.Energy Technol2015;3: 329–339..
Arias AC, MacKenzie JD, McCulloch I, Rivnay J, Salleo A. Materials and applications for large area electronics: solution-based approaches.Chem Rev2010;110: 3–24..
Carmon A, Vronsky E. Method and system for patterning an organic light emittingdiode display by printing. Patent US20070069634 A1; 2007.
OLED-info. Upgraded image lighting technology from ITRI. Updated 12 May 2015.http://www.oled-info.com/itri-upgrades-their-image-lighting-technologyhttp://www.oled-info.com/itri-upgrades-their-image-lighting-technology(accessed24 June 2015).
Matsuzawa T, Aoki Y, Takeuchi N, Murayama Y. A new long phosphorescent phosphor with high brightness, SrAl2O4: Eu2+, Dy3+.J Electrochem Soc1996;143: 2670–2673..
Bessière A, Jacquart S, Priolkar K, Lecointre A, Viana Bet al. ZnGa2O4: Cr3+: a new red long-lasting phosphor with high brightness.Opt Express2011;19: 10131–10137..
Hölsä J, Jungner H, Lastusaari M, Niittykoski J. Persistent luminescence of Eu2+doped alkaline earth aluminates, MAl2O4: Eu2+.J Alloy Compd2001;323–324: 326–330..
Bube RH. Luminescence and trapping in zinc sulfide phosphors with and without copper activator.Phys Rev1950;80: 655–666..
Tada K, Onoda M. Patterned emission from polymeric light-emitting device realized by photo-irradiation in air.Thin Solid Films2000;363: 195–197..
Konica-Minolta. Flexible OLED lighting. Updated 2015.http://www.konicaminolta.com/oled/products/index.htmlhttp://www.konicaminolta.com/oled/products/index.html(accessed 24 June 2015).
OLED-info. Custom designed structured artwork OLED panels from Philips. Updated 14July 2013.http://www.oled-info.com/philips-now-offer-your-own-design-structuredartwork-oled-panels-%E2%82%AC120http://www.oled-info.com/philips-now-offer-your-own-design-structuredartwork-oled-panels-%E2%82%AC120(accessed 24 June 2015).
Mauthner G, Landfester K, Köck A, Brückl H, Kast Met al. Inkjet printed surface cell light-emitting devices from a water-based polymer dispersion.Org Electron2008;9: 164–170..
Zheng H, Zheng YN, Liu NL, Ai N, Wang Qet al. All-solution processed polymer light-emitting diode displays.Nat Commun2013;4: 1971..
Shimoda T, Morii K, Seki S, Kiguchi H. Inkjet printing of light-emitting polymer displays.MRS Bull2003;28: 821–827..
Hernandez-Sosa G, Tekoglu S, Stolz S, Eckstein R, Teusch Cet al. The compromises of printing organic electronics: a case study of gravure-printed light-emitting electrochemical cells.Adv Mat2014;26: 3235–3240..
Sandström A, Dam HF, Krebs FC, Edman L. Ambient fabrication of flexible and large-area organic light-emitting devices using slot-die coating.Nat Commun2012;3: 1002..
Asadpoordarvish A, Sandström A, Larsen C, Bollström R, Toivakka Met al. Light-emitting paper.Adv Funct Mat2015;25: 3238–3245..
Asadpoordarvish A, Sandström A, Tang S, Granström J, Edman L. Encapsulating light-emitting electrochemical cells for improved performance.Appl Phys Lett2012;100: 193508..
Matyba P, Andersson MR, Edman L. On the desired properties of a conjugated polymer-electrolyte blend in a light-emitting electrochemical cell.Org Electron2008;9: 699–710..
Shoji TD, Zhu ZH, Leger JM. Characterizing ion profiles in dynamic junction light-emitting electrochemical cells.ACS Appl Mater Interfaces2013;5: 11509–11514..
Pei QB, Yu G, Zhang C, Yang Y, Heeger AJ. Polymer light-emitting electrochemical-cells.Science1995;269: 1086–1088..
van Reenen S, Matyba P, Dzwilewski A, Janssen RAJ, Edman Let al. A unifying model for the operation of light-emitting electrochemical cells.J Am Chem Soc2010;132: 13776–13781..
Lenes M, Garcia-Belmonte G, Tordera D, Pertegás A, Bisquert Jet al. Operating modes of sandwiched light-emitting electrochemical cells.Adv Funct Mat2011;21: 1581–1586..
Lindh EM, Sandström A, Edman L. Inkjet printed bilayer light-emitting electrochemical cells for display and lighting applications.Small2014;10: 4148–4153..
Sandström A, Matyba P, Inganäs O, Edman L. Separating ion and electron transport: the bilayer light-emitting electrochemical cell.J Am Chem Soc2010;132: 6646–6647..
Liu J, Engquist I, Berggren M. Double-gate light-emitting electrochemical transistor: confining the organic p-n junction.J Am Chem Soc2013;135: 12224–12227..
Liu J, Engquist I, Crispin X, Berggren M. Spatial control of p-n junction in an organic light-emitting electrochemical transistor.J Am Chem Soc2012;134: 901–904..
Hu YF, Gao J. Direct imaging and probing of the p-n junction in a planar polymer light-emitting electrochemical cell.J Am Chem Soc2011;133: 2227–2231..
Fang JF, Matyba P, Robinson ND, Edman L. Identifying and alleviating electrochemical side-reactions in light-emitting electrochemical cells.J Am Chem Soc2008;130: 4562–4568..
Saxena K, Jain VK, Mehta DS. A review on the light extraction techniques in organic electroluminescent devices.Opt Mater2009;32: 221–233..
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