
1.Department of Physics of Complex Systems, Weizmann Institute of Science, Rehovot 76100, Israel
2.Institut für Physik, Carl von Ossietzky Universität Oldenburg, Oldenburg 26129, Germany
3.Department of Electrical Engineering, Technion 32000, Haifa, Israel
Y Silberberg, Email: hadas.frostig@weizmann.ac.il
Published:2017-12,
Published Online:07 August 2017,
Received:13 November 2016,
Revised:28 July 2017,
Accepted:04 August 2017
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Frostig, H. et al. Revealing true coupling strengths in two-dimensional spectroscopy with sparsity-based signal recovery. Light: Science & Applications, 6, e17115 (2017).
Frostig, H. et al. Revealing true coupling strengths in two-dimensional spectroscopy with sparsity-based signal recovery. Light: Science & Applications, 6, e17115 (2017). DOI: 10.1038/lsa.2017.115.
Two-dimensional (2D) spectroscopy is used to study the interactions between energy levels in both the field of optics and nuclear magnetic resonance (NMR). Conventionally
the strength of interaction between two levels is inferred from the value of their common off-diagonal peak in the 2D spectrum
which is termed the cross peak. However
stronger diagonal peaks often have long tails that extend into the locations of the cross peaks and alter their values. Here
we introduce a method for retrieving the true interaction strengths by using sparse signal recovery techniques and apply our method in 2D Raman spectroscopy experiments.
multidimensional spectroscopynonlinear opticssparsity-based algorithms
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