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1.State Key Laboratory of Precision Measurement Technology and Instruments, Department of Precision Instrument, Tsinghua University, Beijing 100084, China
2.State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, 2699 Qianjin Street, Changchun 130012, China
Hong-Hua Fang (hfang@mail.tsinghua.edu.cn)
Hong-Bo Sun (hbsun@tsinghua.edu.cn)
Received:02 August 2023,
Revised:07 December 2023,
Accepted:2023-12-08,
Published Online:02 January 2024,
Published:31 March 2024
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Wang, X. J. et al. Laser manufacturing of spatial resolution approaching quantum limit. Light: Science & Applications, 13, 421-428 (2024).
Wang, X. J. et al. Laser manufacturing of spatial resolution approaching quantum limit. Light: Science & Applications, 13, 421-428 (2024). DOI: 10.1038/s41377-023-01354-5.
Atomic and close-to-atom scale manufacturing is a promising avenue toward single-photon emitters
single-electron transistors
single-atom memory
and quantum-bit devices for future communication
computation
and sensing applications. Laser manufacturing is outstanding to this end for ease of beam manipulation
batch production
and no requirement for photomasks. It is
however
suffering from optical diffraction limits. Herein
we report a spatial resolution improved to the quantum limit by exploiting a threshold tracing and lock-in method
whereby the two-order gap between atomic point defect complexes and optical diffraction limit is surpassed
and a feature size of <5 nm is realized. The underlying physics is that the uncertainty of local atom thermal motion dominates electron excitation
rather than the power density slope of the incident laser. We show that the colour centre yield in hexagonal boron nitride is transformed from stochastic to deterministic
and the emission from individual sites becomes polychromatic to monochromatic. As a result
single colour centres in the regular array are deterministically created with a unity yield and high positional accuracy
serving as a step forward for integrated quantum technological applications.
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