Observation of transition from superfluorescence to polariton condensation in CsPbBr<sub>3</sub> quantum dots film

Danqun Mao; Linqi Chen; Zheng Sun; Min Zhang; Zhe-Yu Shi; Yongsheng Hu; Long Zhang; Jian Wu; Hongxing Dong; Wei Xie; Hongxing Xu

doi:10.1038/s41377-024-01378-5

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Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film

Original Articles

- Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film
- Light: Science & Applications Vol. 13, Issue 2, Pages: 316-324(2024)
- Affiliations：
  
  1.State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China
  2.Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, 201800 Shanghai, China
  3.Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, China
  4.Chongqing Key Laboratory of Precision Optics, Chongqing Institute of East China Normal University, Chongqing 401121, China
  5.CAS Center for Excellence in Ultra-intense Laser Science, Shanghai 201800, China
  6.School of Physics and Technology, Center for Nanoscience and Nanotechnology, Wuhan University, Wuhan 430072, China
- Author bio：
  
  Zheng Sun (zsun@lps.ecnu.edu.cn)
  Hongxing Dong (hongxingd@siom.ac.cn)
  Wei Xie (wxie@phy.ecnu.edu.cn)
- Funds：
- DOI：10.1038/s41377-024-01378-5
  CLC：
- Received：04 July 2023，
  
  Revised：19 December 2023，
  
  Accepted：2024-01-03，
  
  Published Online：30 January 2024，
  
  Published：29 February 2024
- Accepted：
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Mao, D. Q. et al. Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film. Light: Science & Applications, 13, 316-324 (2024).
DOI：

Mao, D. Q. et al. Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film. Light: Science & Applications, 13, 316-324 (2024). DOI： 10.1038/s41377-024-01378-5.

摘要

Abstract

The superfluorescence effect has received extensive attention due to the many-body physics of quantum correlation in dipole gas and the optical applications of ultrafast bright radiation field based on the cooperative quantum state. Here

we demonstrate not only to observe the superfluorescence effect but also to control the cooperative state of the excitons ensemble by externally applying a regulatory dimension of coupling light fields. A new quasi-particle called cooperative exciton-polariton is revealed in a light-matter hybrid structure of a perovskite quantum dot thin film spin-coated on a Distributed Bragg Reflector. Above the nonlinear threshold

polaritonic condensation occurs at a nonzero momentum state on the lower polariton branch owning to the vital role of the synchronized excitons. The phase transition from superfluorescence to polariton condensation exhibits typical signatures of a decrease of the linewidth

an increase of the macroscopic coherence as well as an accelerated radiation decay rate. These findings are promising for opening new potential applications for super-brightness and unconventional coherent light sources and could enable the exploitation of cooperative effects for quantum optics.

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references

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Observation of transition from superfluorescence to polariton condensation in CsPbBr3 quantum dots film

DOI：10.1038/s41377-024-01378-5

摘要

Abstract

关键词

Keywords

references

Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film