1.Department of Physics, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano, Italy
2.IFN-CNR, Piazza Leonardo da Vinci 32, 20133 Milano, Italy
3.Grupo de Investigación en Aplicaciones del Láser y Fotónica, Departamento de Física Aplicada, Universidad de Salamanca, E-37008 Salamanca, Spain
4.Unidad de Excelencia en Luz y Materia Estructuradas (LUMES), Universidad de Salamanca, Salamanca, Spain
5.Laboratorium für Physikalische Chemie, ETH Zürich, 8093 Zürich, Switzerland
6.Department of Physics, Lund University, Lund, Sweden
Mauro Nisoli (mauro.nisoli@polimi.it)
Carlos Hernández-García (carloshergar@usal.es)
Rocío Borrego-Varillas (rocio.borregovarillas@cnr.it)
Published:31 October 2024,
Published Online:20 August 2024,
Received:14 March 2024,
Revised:31 July 2024,
Accepted:04 August 2024
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Vismarra, F. et al. Isolated attosecond pulse generation in a semi-infinite gas cell driven by time-gated phase matching. Light: Science & Applications, 13, 2192-2200 (2024).
Vismarra, F. et al. Isolated attosecond pulse generation in a semi-infinite gas cell driven by time-gated phase matching. Light: Science & Applications, 13, 2192-2200 (2024). DOI: 10.1038/s41377-024-01564-5.
Isolated attosecond pulse (IAP) generation usually involves the use of short-medium gas cells operated at high pressures. In contrast
long-medium schemes at low pressures are commonly perceived as inherently unsuitable for IAP generation due to the nonlinear phenomena that challenge favourable phase-matching conditions. Here we provide clear experimental evidence on the generation of isolated extreme-ultraviolet attosecond pulses in a semi-infinite gas cell
demonstrating the use of extended-medium geometries for effective production of IAPs. To gain a deeper understanding we develop a simulation method for high-order harmonic generation (HHG)
which combines nonlinear propagation with macroscopic HHG solving the 3D time-dependent Schrödinger equation at the single-atom level. Our simulations reveal that the nonlinear spatio-temporal reshaping of the driving field
observed in the experiment as a bright plasma channel
acts as a self-regulating mechanism boosting the phase-matching conditions for the generation of IAPs.
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