Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames

Yogeshwar Nath Mishra; Peng Wang; Florian J. Bauer; Murthy S. Gudipati; Lihong V. Wang

doi:10.1038/s41377-024-01588-x

Go to Nature Website

Your Location：

Home >

Browse articles >

Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames

Original Articles

- Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames
- Light: Science & Applications Vol. 13, Issue 10, Pages: 2312-2320(2024)
- Affiliations：
  
  1.Caltech Optical Imaging Laboratory, Andrew and Peggy Cheng Department of Medical Engineering, Department of Electrical Engineering, California Institute of Technology, 1200 East California Boulevard, Mail Code 138-78, Pasadena, CA 91125, USA
  2.Science Division, Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Drive, Pasadena, CA 91109, USA
  3.Lehrstuhl für Technische Thermodynamik (LTT) and Erlangen Graduate School in Advanced Optical Technologies (SAOT), Universität Erlangen-Nürnberg, Erlangen 91058, Germany
- Author bio：
  
  Lihong V. Wang (LVW@caltech.edu)
- Funds：
- DOI：10.1038/s41377-024-01588-x
  CLC：
- Published：31 October 2024，
  
  Published Online：29 August 2024，
  
  Received：18 January 2024，
  
  Revised：13 August 2024，
  
  Accepted：15 August 2024
- Accepted：
Scan QR Code
Mishra, Y. N. et al. Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames. Light: Science & Applications, 13, 2312-2320 (2024).
DOI：

Mishra, Y. N. et al. Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames. Light: Science & Applications, 13, 2312-2320 (2024). DOI： 10.1038/s41377-024-01588-x.

摘要

Abstract

The creation of carbonaceous nanoparticles and their dynamics in hydrocarbon flames are still debated in environmental

combustion

and material sciences. In this study

we introduce single-pulse femtosecond laser sheet-compressed ultrafast photography (fsLS-CUP)

an ultrafast imaging technique specifically designed to shed light on and capture ultrafast dynamics stemming from interactions between femtosecond lasers and nanoparticles in flames in a single-shot. fsLS-CUP enables the first-time real-time billion frames-per-second (Gfps) simultaneous two-dimensional (2D) imaging of laser-induced fluorescence (LIF) and laser-induced heating (LIH) that are originated from polycyclic aromatic hydrocarbons (PAHs) and soot particles

respectively. Furthermore

fsLS-CUP provides the real-time spatiotemporal map of femtosecond laser-soot interaction as elastic light scattering (ELS) at an astonishing 250 Gfps. In contrast to existing single-shot ultrafast imaging approaches

which are limited to millions of frames per second only and require multiple laser pulses

our method employs only a single pulse and captures the entire dynamics of laser-induced signals at hundreds of Gfps. Using a single pulse does not change the optical properties of nanoparticles for a following pulse

thus allowing reliable spatiotemporal mapping. Moreover

we found that particle inception and growth are derived from precursors. In essence

as an imaging modality

fsLS-CUP offers ultrafast 2D diagnostics

contributing to the fundamental understanding of nanoparticle's inception and broader applications across different fields

such as material science and biomedical engineering.

关键词

Keywords

references

Arthur, J. R., Kapur, P. K.&Napier, D. H. Carbonaceous deposits from hydrocarbon diffusion flames.Nature169, 372–373 (1952)..

Zhang, R. Y. et al. Variability in morphology, hygroscopicity, and optical properties of soot aerosols during atmospheric processing.Proc. Natl Acad. Sci. USA105, 10291–10296 (2008)..

Seaton, A. et al. Particulate air pollution and acute health effects.Lancet345, 176–178 (1995)..

Khodabakhshi, S.,Fulvio, P. F.&Andreoli, E. Carbon black reborn: structure and chemistry for renewable energy harnessing.Carbon162, 604–649 (2020)..

Vander Wal, R. L., Jensen, K. A.&Choi, M. Y. Simultaneous laser-induced emission of soot and polycyclic aromatic hydrocarbons within a gas-jet diffusion flame.Combust. Flame109, 399–414 (1997)..

Will, S., Schraml, S.&Leipert, A. Comprehensive two-dimensional soot diagnostics based on laser-induced incandescence (LII).Symp. (Int.) Combust.26, 2277–2284 (1996)..

Kohse-Höinghaus, K. et al. Combustion at the focus: laser diagnostics and control.Proc. Combust. Inst.30, 89–123 (2005)..

Michelsen, H. A. et al. Laser-induced incandescence: particulate diagnostics for combustion, atmospheric, and industrial applications.Prog. Energy Combust. Sci.51, 2–48 (2015)..

Verdugo, I. et al. Candle flame soot sizing by planar time-resolved laser-induced incandescence.Sci. Rep.10, 11364 (2020)..

Michelsen, H. A. Laser-induced incandescence of flame-generated soot on a picosecond time scale.Appl. Phys. B83, 443–448 (2006)..

Lieske, L. A. et al. Portraits of soot molecules reveal pathways to large aromatics, five-/seven-membered rings, and inception through π-radical localization.ACS Nano17, 13563–13574 (2023)..

Chen, Y. et al. Single-camera, single-shot, time-resolved laser-induced incandescence decay imaging.Opt. Lett.43, 5363–5366 (2018)..

Meyer, T. R. et al. High-speed, three-dimensional tomographic laser-induced incandescence imaging of soot volume fraction in turbulent flames.Opt. Express24, 29547–29555 (2016)..

Gao, L. et al. Single-shot compressed ultrafast photography at one hundred billion frames per second.Nature516, 74–77 (2014)..

Wang, P., Liang, J. Y.&Wang, L. V. Single-shot ultrafast imaging attaining 70 trillion frames per second.Nat. Commun.11, 2091 (2020)..

Wang, P.&Wang, L. V. Single-shot reconfigurable femtosecond imaging of ultrafast optical dynamics.Adv. Sci.10, 2207222 (2023)..

Mishra, Y. N. et al. Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames.Light Sci. Appl.12, 47 (2023)..

Zhang, W. et al. Probing ultrafast dynamics of soot in situ in a laminar diffusion flame using a femtosecond near-infrared laser pump and multi-color Rayleigh scattering probe spectroscopy.Opt. Express30, 26182–26191 (2022)..

Bruno, A. et al. Detection of fluorescent nanoparticles in flame with femtosecond laser-induced fluorescence anisotropy.Opt. Express16, 5623–5632 (2008)..

Li, H. L. et al. Sensing combustion intermediates by femtosecond filament excitation.Opt. Lett.38, 1250–1252 (2013)..

Johansson, K. O. et al. Resonance-stabilized hydrocarbon-radical chain reactions may explain soot inception and growth.Science361, 997–1000 (2018)..

Chorey, D. et al. 3D mapping of polycyclic aromatic hydrocarbons, hydroxyl radicals, and soot volume fraction in sooting flames using FRAME technique.Appl. Phys. B127, 147 (2021)..

Bejaoui, S. et al. Laser induced fluorescence spectroscopy of aromatic species produced in atmospheric sooting flames using UV and visible excitation wavelengths.Combust. Flame161, 2479–2491 (2014)..

Bauer, F. J. et al. In situ characterisation of absorbing species in stationary premixed flat flames using UV–Vis absorption spectroscopy.Appl. Phys. B127, 115 (2021)..

Will, S., Schraml, S.&Leipertz, A. Two-dimensional soot-particle sizing by time-resolved laser-induced incandescence.Opt. Lett.20, 2342–2344 (1995)..

Joret, M. et al. Spectral and angular analysis of non-linear optical response for soot exposed to femtosecond laser light. Proceedings of the European Combustion Meeting 2023. Rouen, 2023.https://normandie-univ.hal.science/hal-04085442https://normandie-univ.hal.science/hal-04085442

Sorensen, C. M. Light scattering by fractal aggregates: a review.Aerosol Sci. Technol.35, 648–687 (2001)..

Charalampopoulos, T. T.&Chang, H. Agglomerate parameters and fractal dimension of soot using light scattering—effects on surface growth.Combust. Flame87, 89–99 (1991)..

Charalampopoulos, T. T.&Felske, J. D. Refractive indices of soot particles deduced from in-situ laser light scattering measurements.Combust. Flame68, 283–294 (1987)..

Mannazhi, M., Bergqvist, S.&Bengtsson, P. E. Laser-induced fluorescence for studying the influence of potassium and sodium salts on PAH formation in sooting premixed flames.Appl. Phys. B128, 68 (2022)..

Zang, H. W. et al. Ultrafast swelling and shrinking of soot in alkanol–air flames induced by femtosecond laser filamentation.Combust. Flame212, 345–351 (2020)..

Wang, P.&Wang, L. V. Compressed ultrafast photography. inCoded Optical Imaging(ed Liang, J. Y.) 453-480 (Cham, Springer, 2024).

Arce, G. R. et al. Compressive coded aperture spectral imaging: an introduction.IEEE Signal Process. Mag.31, 105–115 (2014)..

Lu, Y. et al. Compressed ultrafast spectral-temporal photography.Phys. Rev. Lett.122, 193904 (2019)..

Fang, M. Y. et al. Streak tube imaging lidar with kilohertz laser pulses and few-photons detection capability.Opt. Express32, 19042–19056 (2024)..

Török, S. et al. Influence of rapid laser heating on differently matured soot with double-pulse laser-induced incandescence.Aerosol Sci. Technol.56, 488–501 (2022)..

Martin, J. W., Salamanca, M.&Kraft, M. Soot inception: carbonaceous nanoparticle formation in flames.Prog. Energy Combust. Sci.88, 100956 (2022)..

Bruno, A., de Lisio, C.&Minutolo, P. Time resolved fluorescence polarization anisotropy of carbonaceous particles produced in combustion systems.Opt. Express13, 5393–5408 (2005)..

Pitz, W. J. et al. Development of An Experimental Database and Chemical Kinetic Models for Surrogate Gasoline Fuels. (SAE International, 2007).

Eigentler, F.&Gerlinger, P. A detailed PAH and soot model for complex fuels in CFD applications.Flow., Turbulence Combust.109, 225–251 (2022)..

Kashif, M. et al. Sooting tendencies of primary reference fuels in atmospheric laminar diffusion flames burning into vitiated air.Combust. Flame161, 1575–1586 (2014)..

Liang, J. Y. et al. Single-shot stereo-polarimetric compressed ultrafast photography for light-speed observation of high-dimensional optical transients with picosecond resolution.Nat. Commun.11, 5252 (2020)..

Zang, H. W. et al. Robust and ultralow-energy-threshold ignition of a lean mixture by an ultrashort-pulsed laser in the filamentation regime.Light Sci. Appl.10, 49 (2021)..

Helmchen, F.&Denk, W. Deep tissue two-photon microscopy.Nat. Methods2, 932–940 (2005)..

Guan, M. L. et al. Polarization modulation with optical lock-in detection reveals universal fluorescence anisotropy of subcellular structures in live cells.Light Sci. Appl.11, 4 (2022)..

Huisken, J. et al. Optical sectioning deep inside live embryos by selective plane illumination microscopy.Science305, 1007–1009 (2004)..

Views

Downloads

CSCD

Alert me when the article has been cited

Submit

Tools

Publicity Resources

No data

Related Author

No data

Related Institution

No data

⁰