Carrier dynamic identification enables wavelength and intensity sensitivity in perovskite photodetectors

Liangliang Min; Yicheng Zhou; Haoxuan Sun; Linqi Guo; Meng Wang; Fengren Cao; Wei Tian; Liang Li

doi:10.1038/s41377-024-01636-6

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Carrier dynamic identification enables wavelength and intensity sensitivity in perovskite photodetectors

Original Articles

- Carrier dynamic identification enables wavelength and intensity sensitivity in perovskite photodetectors
- Light: Science & Applications Vol. 13, Issue 11, Pages: 2824-2834(2024)
- Affiliations：
  
  1.School of Physical Science and Technology, Jiangsu Key Laboratory of Frontier Material Physics and Devices, Center for Energy Conversion Materials & Physics (CECMP), Soochow University, Suzhou, China
  2.College of Physical Science and Technology & Microelectronics Industry Research Institute, Yangzhou University, Yangzhou, China
- Author bio：
  
  Haoxuan Sun (hxsun@suda.edu.cn)
  Wei Tian (wtian@suda.edu.cn)
  Liang Li (lli@suda.edu.cn)
- Funds：
- DOI：10.1038/s41377-024-01636-6
  CLC：
- Received：14 June 2024，
  
  Revised：10 September 2024，
  
  Accepted：2024-09-11，
  
  Published Online：29 September 2024，
  
  Published：30 November 2024
- Accepted：
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Min, L. L. et al. Carrier dynamic identification enables wavelength and intensity sensitivity in perovskite photodetectors. Light: Science & Applications, 13, 2824-2834 (2024).
DOI：

Min, L. L. et al. Carrier dynamic identification enables wavelength and intensity sensitivity in perovskite photodetectors. Light: Science & Applications, 13, 2824-2834 (2024). DOI： 10.1038/s41377-024-01636-6.

摘要

Abstract

Deciphering the composite information within a light field through a single photodetector

without optical and mechanical structures

is challenging. The difficulty lies in extracting multi-dimensional optical information from a single dimension of photocurrent. Emerging photodetectors based on information reconstruction have potential

yet they only extract information contained in the photoresponse current amplitude (responsivity matrix)

neglecting the hidden information in response edges driven by carrier dynamics. Herein

by adjusting the thickness of the absorption layer and the interface electric field strength in the perovskite photodiode

we extend the transport and relaxation time of carriers excited by photons of different wavelengths

maximizing the spectrum richness of the edge waveform in the light-dark transition process. For the first time

without the need for extra optical and electrical components

the reconstruction of two-dimensional information of light intensity and wavelength has been achieved. With the integration of machine learning algorithms into waveform data analysis

a wide operation spectrum range of 350–750 nm is available with a 100% accuracy rate. The restoration error has been lowered to less than 0.1% for light intensity. This work offers valuable insights for advancing perovskite applications in areas such as wavelength identification and spectrum imaging.

关键词

Keywords

references

Zhou, Y. et al. Self-powered perovskite photon-counting detectors. Nature 616 , 712–718 (2023)..

de Arquer, F. P. G. et al. Solution-processed semiconductors for next-generation photodetectors. Nat. Rev. Mater. 2 , 16100 (2017)..

Liu, Z. X. et al. Narrowband near-infrared photodetector enabled by dual functional internal-filter-induced selective charge collection. Adv. Optical Mater. 9 , 2100288 (2021)..

Tsai, W. L. et al. Band tunable microcavity perovskite artificial human photoreceptors. Adv. Mater. 31 , 1900231 (2019)..

Lu, J. H. et al. Perovskite photosensors integrated with silver resonant-cavity color filters display color perception beyond that of the human eye. Adv. Funct. Mater. 30 , 2002503 (2020)..

Hou, H. Y. et al. Recent progress of polarization-sensitive perovskite photodetectors. Adv. Funct. Mater. 32 , 2209324 (2022)..

Wang, X. B. et al. Polarization-sensitive halide perovskites for polarized luminescence and detection: recent advances and perspectives. Adv. Mater. 33 , 2003615 (2021)..

Cai, G. Y. et al. Compact angle-resolved metasurface spectrometer. Nat. Mater. 23 , 71–78 (2024)..

Stewart, J. W. et al. Ultrafast pyroelectric photodetection with on-chip spectral filters. Nat. Mater. 19 , 158–162 (2020)..

Faraji-Dana, M. et al. Compact folded metasurface spectrometer. Nat. Commun. 9 , 4196 (2018)..

Uddin, G. et al. Broadband miniaturized spectrometers with a van der Waals tunnel diode. Nat. Commun. 15 , 571 (2024)..

Wu, G. et al. Miniaturized spectrometer with intrinsic long-term image memory. Nat. Commun. 15 , 676 (2024)..

Guo, L. Q. et al. A single-dot perovskite spectrometer. Adv. Mater. 34 , 2200221 (2022)..

Zhu, X. X. et al. Broadband perovskite quantum dot spectrometer beyond human visual resolution. Light Sci. Appl. 9 , 73 (2020)..

Yang, Z. Y. et al. Single-nanowire spectrometers. Science 365 , 1017–1020 (2019)..

Sun, H. X. et al. In situ formed gradient bandgap-tunable perovskite for ultrahigh-speed color/spectrum-sensitive photodetectors via electron-donor control. Adv. Mater. 32 , 1908108 (2020)..

Zhao, Y. J. et al. Multifunctional perovskite photodetectors: from molecular-scale crystal structure design to micro/nano-scale morphology manipulation. Nano-Micro Lett. 15 , 187 (2023)..

Cheng, R. S. et al. Broadband on-chip single-photon spectrometer. Nat. Commun. 10 , 4104 (2019)..

Wang, J. et al. Self-driven perovskite narrowband photodetectors with tunable spectral responses. Adv. Mater. 33 , 2005557 (2021)..

Yuan, S. F. et al. A wavelength-scale black phosphorus spectrometer. Nat. Photonics 15 , 601–607 (2021)..

Wang, J. Y. et al. Single-pixel p-graded-n junction spectrometers. Nat. Commun. 15 , 1773 (2024)..

Ouyang, B. S. et al. Dual-polarity response in self-powered ZnO NWs/Sb 2 Se 3 film heterojunction photodetector array for optical communication. Nano Energy 68 , 104312 (2020)..

Yu, X. Q. et al. Directed self-assembly of viologen-based 2D semiconductors with intrinsic UV-SWIR photoresponse after photo/thermo activation. Nat. Commun. 11 , 1179 (2020)..

Min, L. L. et al. Pyroelectric-accelerated perovskite photodetector for picosecond light detection and ranging. Adv. Mater. 36 , 2400279 (2024)..

Xiao, Z. W., Song, Z. N. & Yan, Y. F. From lead halide perovskites to lead-free metal halide perovskites and perovskite derivatives. Adv. Mater. 31 , 1803792 (2019)..

Ricciardulli, A. G. et al. Emerging perovskite monolayers. Nat. Mater. 20 , 1325–1336 (2021)..

Yang, F. et al. Upscaling solution-processed perovskite photovoltaics. Adv. Energy Mater. 11 , 2101973 (2021)..

Ganesh, N. et al. Wavelength-dependent charge carrier dynamics for single pixel color sensing using graded perovskite structures. Nano Lett. 19 , 6577–6584 (2019)..

Dong, X. Y. et al. Quantum confinement breaking: orbital coupling in 2D ruddlesden–popper perovskites enables efficient solar cells. Adv. Energy Mater. 13 , 2301006 (2023)..

Min, L. L. et al. 2D ruddlesden–popper perovskite with ordered phase distribution for high- performance self-powered photodetectors. Adv. Mater. 33 , 2101714 (2021)..

Yang, Y. et al. Defect suppression in oriented 2D perovskite solar cells with efficiency over 18% via rerouting crystallization pathway. Adv. Energy Mater. 11 , 2002966 (2021)..

Min, L. et al. Frequency–selective perovskite photodetector for anti-interference optical communications. Nat. Commun. 15 , 2066 (2024)..

Yan, Y. J. et al. Benefiting from spontaneously generated 2D/3D bulk–heterojunctions in Ruddlesden−Popper perovskite by incorporation of S–bearing spacer cation. Adv. Sci. 6 , 1900548 (2019)..

Shi, J. S. et al. Fluorinated low-dimensional ruddlesden–popper perovskite solar cells with over 17% power conversion efficiency and improved stability. Adv. Mater. 31 , 1901673 (2019)..

Zhang, Y. et al. Fusing nanowires into thin films: fabrication of graded-heterojunction perovskite solar cells with enhanced performance. Adv. Energy Mater. 9 , 1900243 (2019)..

Wang, R. et al. Caffeine improves the performance and thermal stability of pero vskite solar cells. Joule 3 , 1464–1477 (2019)..

Zhou, N. et al. The spacer cations interplay for efficient and stable layered 2D perovskite solar cells. Adv. Energy Mater. 10 , 1901566 (2020)..

Ebadi, F. et al. Origin of apparent light-enhanced and negative capacitance in perovskite solar cells. Nat. Commun. 10 , 1574 (2019)..

Kalam, A. et al. Interpretation of resistance, capacitance, defect density, and activation energy levels in single-crystalline MAPbI 3 . J. Phys. Chem. C 124 , 3496–3502 (2020)..

Tan, S. et al. Constructing an interfacial gradient heterostructure enables efficient CsPbI 3 perovskite solar cells and printed minimodules. Adv. Mater. 35 , 2301879 (2023)..

Merdasa, A. et al. Impact of excess lead iodide on the recombination kinetics in metal halide perovskites. ACS Energy Lett. 4 , 1370–1378 (2019)..

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