
1.Department of Electronics and Nanoengineering, Aalto University, Espoo, Finland
2.QTF Centre of Excellence, Department of Applied Physics, Aalto University, Aalto, Finland
3.Department of Engineering and Natural Sciences, Tampere University, Tampere, Finland
4.State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing, China
Susobhan Das (susobhan.das@aalto.fi)
Zhipei Sun (zhipei.sun@aalto.fi)
Received:07 May 2024,
Revised:01 October 2024,
Accepted:2024-10-13,
Published Online:09 January 2025,
Published:28 February 2025
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Das, S. et al. Nanoscale thickness Octave-spanning coherent supercontinuum light generation. Light: Science & Applications, 14, 366-373 (2025).
Das, S. et al. Nanoscale thickness Octave-spanning coherent supercontinuum light generation. Light: Science & Applications, 14, 366-373 (2025). DOI: 10.1038/s41377-024-01660-6.
Coherent broadband light generation has attracted massive attention due to its numerous applications ranging from metrology
sensing
and imaging to communication. In general
spectral broadening is realized via third-order and higher-order nonlinear optical processes (e.g.
self-phase modulation
Raman transition
four-wave mixing
multiwave mixing)
which are typically weak and thus require a long interaction length and the phase matching condition to enhance the efficient nonlinear light-matter interaction for broad-spectrum generation. Here
for the first time
we report octave-spanning coherent light generation at the nanometer scale enabled by a phase-matching-free frequency down-conversion process. Up to octave-spanning coherent light generation with a −40dB spectral width covering from ~565 to 1906 nm is demonstrated in discreate manner via difference-frequency generation
a second-order nonlinear process in gallium selenide and niobium oxide diiodide crystals at the 100-nanometer scale. Compared with conventional coherent broadband light sources based on bulk materials
our demonstration is ~5 orders of magnitude thinner and requires ~3 orders of magnitude lower excitation power. Our results open a new way to possibly create compact
versatile and integrated ultra-broadband light sources.
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