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Department of Physics, Ben-Gurion University of the Negev, Beer-Sheva, Israel
Eugene Frumker (efrumker@bgu.ac.il)
Received:23 September 2024,
Revised:27 January 2025,
Accepted:04 March 2025,
Published Online:21 April 2025,
Published:30 June 2025
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Shlomo, N. & Frumker, E. In situ characterization of laser-induced strong field ionization phenomena. Light: Science & Applications, 14, 1673-1686 (2025).
Shlomo, N. & Frumker, E. In situ characterization of laser-induced strong field ionization phenomena. Light: Science & Applications, 14, 1673-1686 (2025). DOI: 10.1038/s41377-025-01808-y.
Accurately characterizing the intensity and duration of strong-field femtosecond pulses within the interaction volume is crucial for attosecond science. However
this remains a major bottleneck
limiting accuracy of the strong-field
and in particular
high harmonic generation experiments. We present a novel scheme for the in situ measurement and control of spatially resolved strong-field femtosecond pulse intensity and duration within the interaction focal region. Our approach combines conjugate focal imaging with in situ ion measurements using gas densities pertinent to attosecond science experiments. Independent measurements in helium and argon
accompanied by a fitting to a strong-field ionization dynamic model
yield accurate and consistent results across a wide range of gas densities and underscores the significance of double ionization
as well as barrier suppression ionization. Direct spatially resolved characterization of the driving laser is a critical step towards resolving the averaging problem in the interaction volume
paving the way for more accurate and reliable attosecond experiments.
Corkum, P. B. Plasma perspective on strong field multiphoton ionization. Phys. Rev. Lett. 71 , 1994–1997 (1993)..
Frumker, E. et al. Probing polar molecules with high harmonic spectroscopy. Phys. Rev. Lett. 109 , 233904 (2012)..
Eckle, P. et al. Attosecond ionization and tunneling delay time measurements in helium. Science 322 , 1525–1529 (2008)..
Sainadh, U. S. etal. Attosecond angular streaking and tunnelling time in atomic hydrogen. Nature 568 , 75–77 (2019)..
Eppink, A. T. J. B. & Parker, D. H. Velocity map imaging of ions and electrons using electrostatic lenses: application in photoelectron and photofragment ion imaging of molecular oxygen. Rev. Sci. Instrum. 68 , 3477–3484 (1997)..
Ullrich, J. et al. Recoil-ion and electron momentum spectroscopy: reaction-microscopes. Rep. Prog. Phys. 66 , 1463–1545 (2003)..
Akagi, H. et al. Laser tunnel ionization from multiple orbitals in HCL. Science 325 , 1364–1367 (2009)..
Weber, T. et al. Correlated electron emission in multiphoton double ionization. Nature 405 , 658–661 (2000)..
Tajima, T. & Dawson, J. M. Laser electron accelerator. Phys. Rev. Lett. 43 , 267–270 (1979)..
Malka, V. et al. Electron acceleration by a wake field forced by an intense ultrashort laser pulse. Science 298 , 1596–1600 (2002)..
Peralta, E. A. et al. Demonstration of electron acceleration in a laser-driven dielectric microstructure. Nature 503 , 91–94 (2013)..
Breuer, J. & Hommelhoff, P. Laser-based acceleration of nonrelativistic electrons at a dielectric structure. Phys. Rev. Lett. 111 , 134803 (2013)..
Shiloh, R. et al. Electron phase-space control in photo nic chip-based particle acceleration. Nature 597 , 498–502 (2021)..
L'Huillier, A. et al. Multiply charged ions induced by multiphoton absorption processes in rare-gas atoms at 1.064µm. J. Phys. B: At. Mol. Phys. 16 , 1363–1381 (1983)..
Alnaser, A. S. et al. Laser-peak-intensity calibration using recoil-ion momentum imaging. Phys. Rev. A 70 , 023413 (2004)..
Lai, Y. H. et al. Experimental investigation of strong-field-ionization theories for laser fields from visible to midinfrared frequencies. Phys. Rev. A 96 , 063417 (2017)..
Smeenk, C. et al. Precise in-situ measurement of laser pulse intensity using strong field ionization. Opt. Express 19 , 9336–9344 (2011)..
Itatani, J. et al. Tomographic imaging of molecular orbitals. Nature 432 , 867–871 (2004)..
Frumker, E. et al. Oriented rotational wave-packet dynamics studies via high harmonic generation. Phys. Rev. Lett. 109 , 113901 (2012)..
Frumker, E. et al. Frequency-resolved high-harmonic wavefront characterization. Opt. Lett. 34 , 3026–3028 (2009)..
L'Huillier, A. et al. High-order harmonic-generation cutoff. Phys. Rev. A 48 , R3433–R3436 (1993)..
Kramida, A. et al. NIST Atomic Spectra Database (ver. 5.12) . https://physics.nist.gov/asd https://physics.nist.gov/asd (2024)..
Shiner, A. D. et al. Wavelength scaling of high harmonic generation efficiency. Phys. Rev. Lett. 103 , 073902 (2009)..
Tchulov, O. et al. Laser induced strong-field ionization gas jet tomography. Sci. Rep. 7 , 6905 (2017)..
Franken, P. A. et al. Generation of optical harmonics. Phys. Rev. Lett. 7 , 118–119 (1961)..
Armstrong, J. A. et al. Interactionsbetween light waves in a nonlinear dielectric. Phys. Rev. 127 , 1918–1939 (1962)..
Boyd, R. W. Nonlinear Optics 3rd edn (Academic Press, 2008).
Terhune, R. W., Maker, P. D. & Savage, C. M. Optical harmonic generation in calcite. Phys. Rev. Lett. 8 , 404–406 (1962)..
Harris, S. E., Oshman, M. K. & Byer, R. L. Observation of tunable optical parametric fluorescence. Phys. Rev. Lett. 18 , 732–734 (1967)..
Shimizu, F. Frequency broadening in liquids by a short light pulse. Phys. Rev. Lett. 19 , 1097–1100 (1967)..
Alfano, R. R. & Shapiro, S. L. Observation of self-phase modulation and small-scale filaments in crystals and glasses. Phys. Rev. Lett. 24 , 592–594 (1970)..
Alfano, R. R. & Shapiro, S. L. Emission in the region 4000 to 7000 å via four-photon coupling in glass. Phys. Rev. Lett. 24 , 584–587 (1970)..
Keldysh, L. V. Ionization in the field of a strong electromagnetic wave. J. Exp. Theor. Phys. 20 , 1307–1314 (1965)..
Perelomov, A. M., Popov, V. S. & Terent'ev, M. V. Ionization of atoms in an alternating electric field. J. Exp. Theor. Phys. 23 , 924 (1966)..
Ammosov, M. V., Delone, N. B. & Krainov, V. P. Tunnel ionization of complex atoms and of atomic ions in an alternating electromagnetic field. J. Exp. Theor. Phys. 64 , 1191 (1986)..
Landau, L. D. & Lifshitz, E. M. Quantum Mechanics: Non-Relativistic Theory 3rd edn, Vol. 3 (Butterworth-Heinemann, 1981).
Perelomov, A. M., Popov, V. S. & Terentev, M. V. Ionization of atoms in an alternating electric field: Ⅱ. J. Exp. Theor. Phys. 24 , 207 (1967)..
Perelomov, A. M. & Popov, V. S. Ionization of atoms in an alternating electrical field: Ⅲ. J. Exp. Theor. Phys. 25 , 336 (1967)..
Reiss, H. R. Effect of an intense electromagnetic field on a Weakly bound system. Phys. Rev. A 22 , 1786–1813 (1980)..
Yudin, G. L. & Ivanov, M. Y. Nonadiabatic tunnel ionization: Looking inside a laser cycle. Phys. Rev. A 64 , 013409 (2001)..
Becker, A. et al. Total ionization rates and ion yields of atoms at nonperturbative laser intensities. Phys. Rev. A 64 , 023408 (2001)..
Tong, X. M., Zhao, Z. X. & Lin, C. D. Theory of molecular tunneling ionization. Phys. Rev. A 66 , 033402 (2002)..
Popruzhenko, S. V. et al. Strong field ionization rate for arbitrary laser frequencies. Phys. Rev. Lett. 101 , 193003 (2008)..
Zhao, S. F. et al. Analytical model for calibrating laser intensity in strong-field-ionization experiments. Phys. Rev. A 93 , 023413 (2016)..
Larochelle, S. F. J., Talebpour, A. & Chin, S. L. Coulomb effect in multiphoton ionization of rare-gas atoms. J. Phys. B: At., Mol. Opt. Phys. 31 , 1215–1224 (1998)..
Cornaggia, C. & Hering, P. Nonsequential double ionization of small molecules induced by a femtosecond laser field. Phys. Rev. A 62 , 023403 (2000)..
Wu, J. et al. Multiorbital tunneling ionization of the co molecule. Phys. Rev. Lett. 108 , 183001 (2012)..
Lloyd, D. T., O'Keeffe, K. & Hooker, S. M. Comparison of strong-field ionization models in the wavelength-scaling of high harmonic generation. Opt. Express 27 , 6925–6935 (2019)..
Ilkov, F. A., Decker, J. E. & Chin, S. L. Ionization of atoms in the tunnelling regime with experimental evidence using hg atoms. J. Phys. B At. Mol. Opt. Phys. 25 , 4005–4020 (1992)..
Kopold, R. et al. Routes to nonsequential double ionization. Phys. Rev. Lett. 85 , 3781–3784 (2000)..
Feuerstein, B. et al. Separation of recollision mechanisms in nonsequential strong field double ionization of Ar: the role of excitation tunneling. Phys. Rev. Lett. 87 , 043003 (2001)..
Bergues, B. et al. Attosecond tracing of correlated electron-emission in non-sequential double ionization. Nat. Commun. 3 , 813 (2012)..
Diels, J. C. & Rudolph, W. Ultrashort Laser Pulse Phenomena 2nd edn (Elsevier, 2006).
Delone, N. B. & Krainov, V. P. Energy and angular electron spectra for the tunnel ionization of atoms by strong low-frequency radiation. J. Opt. Soc. Am. B Opt. Phys. 8 , 1207–1211 (1991)..
Ivanov, M. Y., Spanner, M. & Smirnova, O. Anatomy of strong field ionization. J. Mod. Opt. 52 , 165–184 (2005)..
Tawara, H. & Kato, T. Total and partial ionization cross sections of atoms and ions by electron impact. At. Data Nucl. Data Tables 36 , 167–353 (1987)..
De Jesus, V. L. B. et al. Atomic structure dependence of nonsequential double ionization of He, Ne and Ar in strong laser pulses. J. Phys. B At. Mol. Opt. Phys. 37 , L161–L167 (2004)..
Delone, N. B. & Krainov, V. P. Tunneling and barrier-suppression ionization of atoms and ions in a laser radiation field. Phys. Uspekhi 41 , 469–485 (1998)..
Zhang, Q. B., Lan, P. F. & Lu, P. X. Empirical formula for over-barrier strong-field ionization. Phys. Rev. A 90 , 043410 (2014)..
Zhou, J. P. et al. Amplification of 26-fs, 2-TW pulses near the gain-narrowing limit in Ti: sapphire. Opt. Lett. 20 , 64–66 (1995)..
Bor, Z. & Horváth, Z. L. Distortion of femtosecond pulses in lenses. Wave optical description. Opt. Commun. 94 , 249–258 (1992)..
Porras, M. A. Characterization of the electric field of focused pulsed Gaussian beams for phase-sensitive interactions with matter. Opt. Lett. 34 , 1546–1548 (2009)..
Attia, I. & Frumker, E. Space-time coupling of the carrier-envelope phase in ultrafast optical pulses. Opt. Express 30 , 12420–12426 (2022)..
Raizer, Y. P. Gas Discharge Physics , Vol. 1 (Springer, 1991).
Fitzpatrick, R. Plasma Physics: An Introduction 2nd edn. (CRC Press, 2022).
Grafström, S. et al. Fast laser beam position control with submicroradian precision. Opt. Commun. 65 , 121–126 (1988)..
Jones, D. J. et al. Carrier-envelope phase control of femtosecond mode-locked lasers and direct optical frequency synthesis. Science 288 , 635–639 (2000)..
Frumker, E. et al. Order-dependent structure of high harmonic wavefronts. Opt. Express 20 , 13870–13877 (2012)..
Vozzi, C. et al. Generalized molecular orbital tomography. Nat. Phys. 7 , 822–826 (2011)..
Li, W. et al. Time-resolved dynamics in N 2 O 4 probed using high harmonic generation. Science 322 , 1207–1211 (2008)..
Smirnova, O. et al. High harmonic interferometry of multi-electron dynamics in molecules. Nature 460 , 972–977 (2009)..
Drescher, M. et al. Time-resolved atomic inner-shell spectroscopy. Nature 419 , 803–807 (2002)..
Tong, X. M. & Lin, C. D. Empirical formula for static field ionization rates of atoms and molecules by lasers in the barrier-suppression regime. J. Phys. B At. Mol. Opt. Phys. 38 , 2593–2600 (2005)..
Walker, B. et al. Precision measurement of strong field double ionization of helium. Phys. Rev. Lett. 73 , 1227–1230 (1994)..
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