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1.Department of Physics, University of California, Berkeley, CA, USA
2.Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, USA
3.Department of Chemistry, University of California, Berkeley, CA, USA
4.Graduate Group in Applied Science and Technology, University of California, Berkeley, CA, USA
5.Department of Mechanical and Industrial Engineering, Northeastern University, Boston, MA, USA
6.Kavli Energy NanoScience Institute, Berkeley, CA, USA
Feng Wang (fengwang76@berkeley.edu)
Received:19 November 2024,
Revised:16 April 2025,
Accepted:17 April 2025,
Published Online:25 June 2025,
Published:31 August 2025
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Uzundal, C.B. et al. Efficient on-chip terahertz generation and detection with GaN photoconductive emitters. Light: Science & Applications, 14, 2327-2334 (2025).
Uzundal, C.B. et al. Efficient on-chip terahertz generation and detection with GaN photoconductive emitters. Light: Science & Applications, 14, 2327-2334 (2025). DOI: 10.1038/s41377-025-01870-6.
Photoconductive emitters for terahertz generation hold promise for highly efficient down-conversion of optical photons because it is not constrained by the Manley-Rowe relation. Existing terahertz photoconductive devices
however
faces limits in efficiency due to the semiconductor properties of commonly used GaAs materials. Here
we demonstrate that large bandgap semiconductor GaN
characterized by its high breakdown electric field
facilitates the highly efficient generation of terahertz waves in a coplanar stripline waveguide. Towards this goal
we investigated the excitonic contribution to the electro-optic response of GaN under static electric field both through experiments and first-principles calculations
revealing a robust excitonic Stark shift. Using this electro-optic effect
we developed a novel ultraviolet pump-probe spectroscopy for in-situ characterization of the terahertz electric field strength generated by the GaN photoconductive emitter. Our findings show that terahertz power scales quadratically with optical excitation power and applied electric field over a broad parameter range. We achieved an optical-to-terahertz conversion efficiency approaching 100% within the 0.03–1 THz bandwidth at the highest bias field (116 kV/cm) in our experiment. Further optimization of GaN-based terahertz generation devices could achieve even greater optical-to-terahertz conversion efficiencies.
Nagatsuma, T., Ducournau, G. & Renaud, C. C. Advances in terahertz communications accelerated by photonics. Nat. Photonics 10 , 371–379 (2016)..
Mittleman, D. M. Twenty years of terahertz imaging [Invited ] . Opt. Express 26 , 9417–9431 (2018)..
Yang, C. J. et al. Terahertz control of many-body dynamics in quantum materials. Nat. Rev. Mater. 8 , 518–532 (2023)..
Tonouchi, M. Cutting-edge terahertz technology. Nat. Photonics 1 , 97–105 (2007)..
Ulbricht, R. et al. Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy. Rev. Mod. Phys. 83 , 543–586 (2011)..
Li, X. et al. Terahertz field–induced ferroelectricity in quantum paraelectric SrTiO 3 . Science 364 , 1079–1082 (2019)..
Ferguson, B. & Zhang, X. C. Materials for terahertz science and technology. Nat. Mater. 1 , 26–33 (2002)..
Smith, P. R., Auston, D. H. & Nuss, M. C. Subpicosecond photoconducting dipole antennas. IEEE J. Quantum Electron. 24 , 255–260 (1988)..
Boyd, R. W. Nonlinear Optics . (Elsevier, 2008).
Lee, Y. S. Principles of Terahertz Science and Technology . (Springer, 2009).
Fülöp, J. A., Tzortzakis, S. & Kampfrath, T. Laser‐driven strong‐field terahertz sources. Adv. Optical Mater. 8 , 1900681 (2020)..
Shan, J. & Heinz, T. F. Terahertz radiation from semiconductors. in Ultrafast Dynamical Processes in Semiconductors (ed Tsen, K. T. ) (Springer, 2004), 1–56. https://doi.org/10.1007/978-3-540-44879-2_1 https://doi.org/10.1007/978-3-540-44879-2_1 ..
Hwang, H. Y. et al. A review of non-linear terahertz spectroscopy with ultrashort tabletop-laser pulses. J. Mod. Opt. 62 , 1447–1479 (2015)..
Jepsen, P. U., Jacobsen, R. H. & Keiding, S. R. Generation and detection of terahertz pulses from biased semiconductor antennas. J. Optical Soc. Am. B 13 , 2424–2436 (1996)..
Lepeshov, S. et al. Enhancement of terahertz photoconductive antenna operation by optical nanoantennas. Laser Photonics Rev. 11 , 1600199 (2017)..
Yang, S. H. et al. 7.5% Optical-to-terahertz conversion efficiency offered by photoconductive emitters with three-dimensional plasmonic contact electrodes. IEEE Trans. Terahertz Sci. Technol. 4 , 575–581 (2014)..
Yardimci, N. T. et al. A high-power broadband terahertz source enabled by three-dimensional light confinement in a plasmonic nanocavity. Sci. Rep. 7 , 4166 (2017)..
Jarrahi, M. Advanced photoconductive terahertz optoelectronics based on nano-antennas and nano-plasmonic light concentrators. IEEE Trans. Terahertz Sci. Technol. 5 , 391–397 (2015)..
Berry, C. W., Hashemi, M. R. & Jarrahi, M. Generation of high power pulsed terahertz radiation using a plasmonic photoconductive emitter array with logarithmic spiral antennas. Appl. Phys. Lett. 104 , 081122 (2014)..
Cai, Y. et al. Design and performance of singular electric field terahertz photoconducting antennas. Appl. Phys. Lett. 71 , 2076–2078 (1997)..
Berry, C. W. & Jarrahi, M. Terahertz generation using plasmonic photoconductive gratings. N. J. Phys. 14 , 105029 (2012)..
Luo, J. K. et al. The electrical breakdown properties of GaAs layers grown by molecular beam epitaxy at low temperature. Semiconductor Sci. Technol. 9 , 2199–2204 (1994)..
Morkoç, H. Handbook of Nitride Semiconductors and Devices: Materials Properties, Physics and Growth . (Wiley, 2008).
Houston, P. A. & Evans, A. G. R. Saturation velocity of electrons in GaAs. IEEE Trans. Electron Devices 23 , 584–586 (1976)..
Ropagnol, X. et al. Intense sub-terahertz radiation from wide-bandgap semiconductor based large-aperture photoconductive antennas pumped by UV lasers. N. J. Phys. 21 , 113042 (2019)..
Imafuji, O. et al. High power subterahertz electromagnetic wave radiation from GaN photoconductive switch. Appl. Phys. Lett. 91 , 071112 (2007)..
Neamen, D. A. Semiconductor Physics and Devices: Basic Principles (McGraw-Hill, 2012).
Dan, Y. P. et al. A photoconductor intrinsically has no gain. ACS Photonics 5 , 4111–4116 (2018)..
Chen, G. D. et al. Fundamental optica l transitions in GaN. Appl. Phys. Lett. 68 , 2784–2786 (1996)..
Liu, W. et al. Photovoltaic spectroscopic study of GaN epilayers and InGaN quantum well structures. J. Mater. Res. 14 , 2794–2798 (1999)..
Verma, D. et al. Local electric field measurement in GaN diodes by exciton Franz–Keldysh photocurrent spectroscopy. Appl. Phys. Lett. 116 , 202102 (2020)..
Oberhofer, A. E. et al. Planar gallium nitride ultraviolet optical modulator. Appl. Phys. Lett. 83 , 2748–2750 (2003)..
Kao, C. K. et al. Electroabsorption modulators based on bulk GaN films and GaN/AlGaN multiple quantum wells. J. Appl. Phys. 109 , 083102 (2011)..
Sakurai, J. J. & Napolitano, J. Modern Quantum Mechanics (Cambridge University Press, 2020). https://doi.org/10.1017/9781108587280 https://doi.org/10.1017/9781108587280 ..
Mendis, R. & Grischkowsky, D. Undistorted guided-wave propagation of subpicosecond terahertz pulses. Opt. Lett. 26 , 846–848 (2001)..
Simons, R. N. Coplanar Waveguide Circuits, Components, and Systems (Wiley, 2001). https://doi.org/10.1002/0471224758 https://doi.org/10.1002/0471224758 ..
Potts, A. M. et al. On-chip time-domain terahertz spectroscopy of superconducting films below the diffraction limit. Nano Lett. 23 , 3835–3841 (2023)..
Gallagher, P. et al. Quantum-critical conductivity of the Dirac fluid in graphene. Science 364 , 158–162 (2019)..
Zomega Terahertz https://www.opt-ron.com/images/zomega_catalogue_1401_lr.pdf https://www.opt-ron.com/images/zomega_catalogue_1401_lr.pdf (2024).
Udabe, A., Baraia-Etxaburu, I. & Diez, D. G. Gallium nitride power devices: a state of the art review. IEEE Access 11 , 48628–48650 (2023)..
Nomoto, K. et al. 1.7-kV and 0.55-mΩ⋅cm 2 GaN p-n diodes on bulk GaN substrates with avalanche capability. IEEE Electron Device Lett. 37 , 161–164 (2016)..
Woo, K. et al. From wide to ultrawide-bandgap semiconductors for high power and high frequency electronic devices. J. Phys. : Mater. 7 , 022003 (2024)..
Matthäus, G. et al. Microlens coupled interdigital photoconductive switch. Appl. Phys. Lett. 93 , 091110 (2008)..
Giannozzi, P. et al. QUANTUM ESPRESSO: a modular and open-source software project for quantum simulations of materials. J. Phys. : Condens. Matter 21 , 395502 (2009)..
Giannozzi, P. et al. Advanced capabilities for materials modelling with Quantum ESPRESSO. J. Phys. : Condens. Matter 29 , 465901 (2017)..
Deslippe, J. et al. BerkeleyGW: a massively parallel computer package for the calculation of the quasiparticle and optical properties of materials and nanostructures. Computer Phys. Commun. 183 , 1269–1289 (2012)..
Hybertsen, M. S. & Louie, S. G. Electron correlation in semiconductors and insulators: band gaps and quasiparticle energies. Phys. Rev. B 34 , 5390–5413 (1986)..
Chan, Y. H. et al. Giant exciton-e nhanced shift currents and direct current conduction with subbandgap photo excitations produced by many-electron interactions. Proc. Natl Acad. Sci. USA 118 , e1906938118 (2021)..
Hu, C. et al. Excitonic interactions and mechanism for ultrafast interlayer photoexcited response in van der Waals heterostructures. Phys. Rev. Lett. 131 , 236904 (2023)..
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