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1.Department of Physics, Politecnico di Milano, 20133 Milan, Italy
2.Université de Paris, CNRS, Laboratoire Matériaux et Phénomènes Quantiques, 75013 Paris, France
3.Université Paris-Saclay, CNRS, Centre de Nanosciences et de Nanotechnologies, 91120 Palaiseau, France
Michele Celebrano (michele.celebrano@polimi.it)
Marco Finazzi (marco.finazzi@polimi.it)
Received:31 December 2024,
Revised:2025-06-15,
Accepted:30 June 2025,
Published Online:15 September 2025,
Published:30 November 2025
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Luan, Y. G. et al. All-optical polarization encoding and modulation by nonlinear interferometry at the nanoscale. Light: Science & Applications, 14, 3471-3478 (2025).
Luan, Y. G. et al. All-optical polarization encoding and modulation by nonlinear interferometry at the nanoscale. Light: Science & Applications, 14, 3471-3478 (2025). DOI: 10.1038/s41377-025-01948-1.
Optical metasurfaces allow complex light manipulation within subwavelength thicknesses and are thus rapidly emerging as a key enabling technology for nanophotonics applications. The control over light polarization already provided a route towards ultracompact metasurface-based polarimetry devices. If translated to the nonlinear optical regime it may become a transformative tool for nonlinear imaging
optical holography
and sensing. Here
we report ultrafast all-optical polarization modulation of upconverted light by all-dielectric metasurfaces via nonlinear interferometry. By controlling the relative phase between a pump beam at
ω
and its frequency-doubled replica at 2
ω
we can set the phase relation between two frequency-degenerate upconversion processes at 3
ω
– sum-frequency generation and third-harmonic generation – stemming from an AlGaAs metasurface. By leveraging the opposite parity of the two nonlinear processes and adjusting their relative intensities
we achieve a modulation of the polarization state of the upconverted light between linear and circular states with a circular polarization degree of up to 83%. Remarkably
circularly polarized light of opposite handedness is symmetrically mapped in the Fourier space
at coincidence with the first diffraction orders of the metasurface. Furthermore
the handedness can be completely reversed within the same diffraction order by applying a phase delay of π. Our work adds an additional modulation layer beyond intensity to all-optical routing with precise phase control: polarization. The capability to encode and modulate simultaneously different polarization states in the
k
-space holds potential for chiral sensing and advanced imaging techniques.
Neshev, D. N. & Miroshnichenko, A. E. Enabling smart vision with metasurfaces. Nat. Photonics 17 , 26–35 (2023)..
Hu, J. et al. Diffractive optical computing in free space. Nat. Commun. 15 , 1525 (2024)..
Schulz, S. A. et al. Roadmap on photonic metasurfaces. Appl. Phys. Lett. 124 , 260701 (2024)..
Feng, Z. et al. Dual-band polarized upconversion photoluminescence enhanced by resonant dielectric metasurfaces. eLight 3 , 21 (2023)..
Zheng, Z. et al. Third-harmonic generation and imaging with resonant Si membrane metasurface. Opto-Electron. Adv 6 , 220174 (2023)..
Lalanne, P. et al. Design and fabrication of blazed binary diffractive elements with sampling periods smaller than the structural cutoff. J. Opt. Soc. Am. A 16 , 1143–1156 (1999)..
Chen, W. T., Zhu, A. Y. & Capasso, F. Flat optics with dispersion-engineered metasurfaces. Nat. Rev. Mater. 5 , 604–620 (2020)..
Sinelnik, A. et al. Ultrafast all-optical second harmonic wavefront shaping. Nat. Commun. 15 , 2507 (2024)..
Zheng, Z. et al. Planar narrow bandpass filter based on Si resonant metasurface. J. Appl. Phys. 130 , 053105 (2021)..
Zou, X. et al. Pixel-l evel Bayer-type colour router based on metasurfaces. Nat. Commun. 13 , 3288 (2022)..
Shcherbakov, M. R. et al. Ultrafast all-optical tuning of direct-gap semiconductor metasurfaces. Nat. Commun. 8 , 17 (2017)..
Maiuri, M. et al. Ultrafast all-optical metasurfaces: Challenges and new frontiers. ACS Photonics 11 , 2888–2905 (2024)..
Santiago-Cruz, T. et al. Photon pairs from resonant metasurfaces. Nano Lett. 21 , 4423–4429 (2021)..
Santiago-Cruz, T. et al. Resonant metasurfaces forgenerating complex quantum states. Science 377 , 991–995 (2022)..
Arbabi, A. et al. A. Dielectric metasurfaces for complete control of phase and polarization with subwavelength spatial resolution and high transmission. Nat. Nanotechnol. 10 , 937–943 (2015)..
Li, F. -J. et al. Metasurface polarization optics: From classical to quantum. Appl. Phys. Rev. 11 , 041332 (2024)..
Basiri, A. et al. Nature-inspired chiral metasurfaces for circular polarization detection and full-Stokes polarimetric measurements. Light Sci. Appl. 8 , 78 (2019)..
Rubin, N. A. et al. Matrix Fourier optics enables a compact full-Stokes polarization camera. Science 365 , eaax1839 (2019)..
Li, G., Zhang, S. & Zentgraf, T. Nonlinear photonic metasurfaces. Nat. Rev. Mater. 2 , 17010 (2017)..
Bonacina, L. et al. Harmonic generation at the nanoscale. J. Appl. Phys. 127 , 230901 (2020)..
Vabishchevich, P. & Kivshar, Y. Nonlinear photonics with metasurfaces. Photonics Res. 11 , B50–B62 (2023)..
Zhang, Y. et al. Chirality logic gates. Sci. Adv. 8 , eabq8246 (2022)..
Zhang, Y. et al. Coherent modulation of chiral nonlinear optics with crystal symmetry. Light Sci. Appl. 11 , 216 (2022)..
Finazzi, M. et al. Selection rules for second-harmonic generati on in nanoparticles. Phys. Rev. B 76 , 125414 (2007)..
Konishi, K., Kan, T. & Kuwata-Gonokami, M. Tunable and nonlinear metamaterials for controlling circular polarization. J. Appl. Phys. 127 , 230902 (2020)..
Konishi, K. et al. Polarization-controlled circular second-harmonic generation from metal hole arrays with threefold rotational symmetry. Phys. Rev. Lett. 112 , 135502 (2014)..
Chen, S. M. et al. Giant nonlinear optical activity of achiral origin in planar metasurfaces with quadratic and cubic nonlinearities. Adv. Mater. 28 , 2992–2999 (2016)..
Wang, H. et al. All-optical ultrafast polarization switching with nonlinear plasmonic metasurfaces. Sci. Adv 10 , eadk3882 (2024)..
Reineke, B. et al. Silicon metasurfaces for third harmonic geometric phase manipulation and multiplexed holography. Nano Lett. 19 , 6585–6591 (2019)..
Zhu, Z. et al. Nonlinear polarization imaging by parametric upconversion. Optica 9 , 1297–1302 (2022)..
Hendry, E. et al. Ultrasensitive detection and characterization of biomolecules using superchiral fields. Nat. Nanotechnol. 5 , 783–787 (2010)..
Ren, M. X. et al. Giant nonlinear optical activity in a plasmonic metamaterial. Nat. Commun. 3 , 833 (2012)..
Di Francescantonio, A. et al. Coherent control of the nonlinear emission of single plasmonic nanoantennas by dual‐beam pumping. Adv. Opt. Mater. 10 , 2200757 (2022)..
Di Francescantonio, A. et al. All-optical free-space routing of upconverted light by metasurfaces via nonlinear interferometry. Nat. Nanotechnol. 19 , 298–305 (2024)..
Abdelraouf, O. A. M. et al. Recent advances in tunable metasurfaces: Materials, design, and applications. ACS Nano 16 , 13339–13369 (2022)..
Cordaro, A. et al. Solving integral equations in free space with inverse-designed ultrathin optical metagratings. Nat. Nanotechnol. 18 , 365–372 (2023)..
Guo, C. et al. Photonic crystal slab Laplace operator f or image differentiation. Optica 5 , 251–256 (2018)..
Zhou, Y. et al. Flat optics for image differentiation. Nat. Photonics 14 , 316–323 (2020)..
de Ceglia, D. et al. Analog image processing with nonlinear nonlocal flat optics. Opt. Mater. Express 14 , 92–100 (2024)..
Rocco, D. et al. Tunable second harmonic generation by an all-dielectric diffractive metasurface embedded in liquid crystals. New J. Phys 24 , 045002 (2022)..
Sultanov, V. et al. Tunable entangled photon-pair generation in a liquid crystal. Nature 631 , 294–299 (2024)..
He, Z. et al. Electro-optically modulated nonlinear metasurfaces. Nano Lett. 24 , 14215–14221 (2024)..
Di Francescantonio, A. et al. Efficient GHz electro-optical modulation with a nonlocal lithium niobate metasurface in the linear and nonlinear regime. Nat Commun 16 , 7000 (2025)..
Celebrano, M. et al. Optical tunin g of dielectric nanoantennas for thermo-optically reconfigurable nonlinear metasurfaces. Opt. Lett 46 , 2453–2456 (2021)..
Sartorello, G. et al. Ultrafast optical modulation of second- and third-harmonic generation from cut-disk-based metasurfaces. ACS Photonics 3 , 1517–1522 (2016)..
Pogna, E. A. A. et al. Ultrafast, all optically reconfigurable, nonlinear nanoantenna. ACS Nano 15 , 11150–11157 (2021)..
Burla, M. et al. 500 GHz plasmonic Mach-Zehnder modulator enabling sub-THz microwave photonics. APL Photonics 4 , 056106 (2019)..
Carletti, L. et al. Enhanced second-harmonic generation from magnetic resonance in AlGaAs nanoantennas. Opt. Express 23 , 26544–26550 (2015)..
Gili, V. F. et al. Monolithic AlGaAs second-harmonic nanoantennas. Opt. Express 24 , 15965–15971 (2016)..
Camacho-Morales, R. et al. Nonlinear generation of vector beams from AlGaAs nanoantennas. Nano Lett. 16 , 7191–7197 (2016)..
Liu, S. et al. Resonantly enhanced second-harmonic generation using Ⅲ–Ⅴ semiconductor all-dielectric metasurfaces. Nano Lett. 16 , 5426–5432 (2016)..
Ghirardini, L. et al. Polarization properties of second-harmonic generation in AlGaAs optical nanoantennas. Opt. Lett 42 , 559–562 (2017)..
Schaefer, B. et al. Measuring the Stokes polarization parameters. Am. J. Phys. 75 , 163–168 (2007)..
Vogwell, J. et al. Ultrafast control over chiral sum-frequency generation. Sci. Adv. 9 , eadj1429 (2023)..
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