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1.Wuhan National Laboratory for Optoelectronics and School of Physics, Huazhong University of Science and Technology, Wuhan, China
2.School of Electronic and Information Engineering, Hubei University of Science and Technology, Xianning, China
3.School of Optics and Electronic Information, Huazhong University of Science and Technology Wuhan, Wuhan, Hubei, China
4.Hubei Key Laboratory of Optical Information and Pattern Recognition, Wuhan Institute of Technology, Wuhan, China
Kai Wang (kale_wong@hust.edu.cn)
Furi Ling (lingfuri@mail.hust.edu.cn)
Peixiang Lu (lupeixiang@hust.edu.cn)
Received:26 November 2024,
Revised:2025-08-26,
Accepted:09 September 2025,
Published Online:09 October 2025,
Published:30 November 2025
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Yang, J. X. et al. Manipulating terahertz phonon-polariton in the ultrastrong coupling regime with bound states in the continuum. Light: Science & Applications, 14, 3747-3755 (2025).
Yang, J. X. et al. Manipulating terahertz phonon-polariton in the ultrastrong coupling regime with bound states in the continuum. Light: Science & Applications, 14, 3747-3755 (2025). DOI: 10.1038/s41377-025-02044-0.
The strong coupling between photons and phonons in polar materials gives rise to phonon-polaritons that encapsulate a wealth of physical information
offering crucial tools for the ultrafast terahertz sources and the topological engineering of terahertz light. However
it is still quite challenging to form and manipulate the terahertz phonon-polaritons under the ultrastrong coupling regime till now. In this work
we demonstrate the ultrastrong coupling between the phonon (at 0.95 THz) in a MAPbI
3
film and the metallic bound states in the continuum (BICs) in Au metasurfaces. The Rabi splitting can be continuously tuned from 28% to 48.4% of the phonon frequency by adjusting the parameters (size
shape and period) of Au metasurfaces
reaching the ultrastrong coupling regime. By introducing wavelet transform
the mode evolution information of the terahertz phonon-polariton is successfully extracted. It indicates that the phonon radiation intensity of the MAPbI
3
film is enhanced as the coupling strength is increased. This work not only establishes a new platform for terahertz devices but also opens new avenues for exploring the intricate dynamics of terahertz phonon-polaritons.
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