Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles

Nicolò Accanto; Jana B Nieder; Lukasz Piatkowski; Marta Castro-Lopez; Francesco Pastorelli; Daan Brinks; Niek F van Hulst

doi:10.1038/lsa.2014.24

Go to Nature Website

Your Location：

Home >

Browse articles >

Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles

Original Articles

- Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles
- Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles
- LSA 2014年3卷第1期
- Affiliations：
  
  1.ICFO—Institut de Ciencies Fotoniques, 08860 Castelldefels (Barcelona), Spain
  2.Institut Fresnel, CNRS UMR7249, Aix-Marseille University, 13397 Marseille, France
  3.ICREA—Institució Catalana de Recerca i Estudis Avançats (ICREA), 08010 Barcelona, Spain
- Author bio：
  
  Dr NF van Hulst, ICFO—Institut de Ciencies Fotoniques, Mediterranean Technology Park, 08860 Castelldefels (Barcelona), Spain E-mail: Niek.vanHulst@ICFO.eu
- Funds：
- DOI：10.1038/lsa.2014.24
  中图分类号：
- 纸质出版日期：2014-03，
  
  网络出版日期：2014-01-31，
  
  收稿日期：2013-07-12，
  
  修回日期：2013-10-01，
  
  录用日期：2013-10-18
- Accepted：
Scan QR Code
Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles[J]. LSA, 2014,3(1).

Accanto, N. et al. Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles. Light: Science & Applications, 3, e143 (2014).
Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles[J]. LSA, 2014,3(1). DOI： 10.1038/lsa.2014.24.

Accanto, N. et al. Phase control of femtosecond pulses on the nanoscale using second harmonic nanoparticles. Light: Science & Applications, 3, e143 (2014). DOI： 10.1038/lsa.2014.24.

摘要

Abstract

Investigations of ultrafast processes occurring on the nanoscale require a combination of femtosecond pulses and nanometer spatial resolution. However

controlling femtosecond pulses with nanometer accuracy is very challenging

as the limitations imposed both by dispersive optics on the time duration of a pulse and by the spatial diffraction limit on the focusing of light must be overcome simultaneously. In this paper

we provide a universal method that allows full femtosecond pulse control in subdiffraction-limited areas. We achieve this aim by exploiting the intrinsic coherence of the second harmonic emission from a single nonlinear nanoparticle of deep subwavelength dimensions. The method is proven to be highly sensitive

easy to use

quick

robust and versatile. This approach allows measurements of minimal phase distortions and the delivery of tunable higher harmonic light in a nanometric volume. Moreover

the method is shown to be compatible with a wide range of particle sizes

shapes and materials

allowing easy optimization for any given sample. This method will facilitate the investigation of light–matter interactions on the femtosecond–nanometer level in various areas of scientific study.

关键词

Keywords

diffraction limitFourier limitmultiphoton intrapulse interference phase scannanoparticlenanophotonicsphase controlsecond harmonic generationultrafast

references

Brinks D, Stefani FD, Kulzer F, Hildner R, Taminiau THet al. Visualizing and controlling vibrational wave packets of single molecules.Nature2010;465: 905–908..

Hildner R, Brinks D, Nieder JB, Cogdell RJ, van Hulst NF. Quantum coherent energy transfer over varying pathways in single light-harvesting complexes.Science2013;340: 1448–1451..

Masia F, Accanto N, Langbein W, Borri P. Spin-flip limited exciton dephasing in CdSe/ZnS colloidal quantum dots.Phys Rev Lett2012;108: 087401..

Anderson A, Deryckx KS, Xu XG, Steinmeyer G, Raschke MB. Few-femtosecond plasmon dephasing of a single metallic nanostructure from optical response function reconstruction by interferometric frequency resolved optical gating.Nano Lett2010;10: 2519–2524..

Aeschlimann M, Brixner T, Fischer A, Kramer C, Melchior Pet al. Coherent two-dimensional nanoscopy.Science2011;333: 1723–1726..

Biagioni P, Brida D, Huang JS, Kern J, Duò Let al. Dynamics of four-photon photoluminescence in gold nanoantennas.Nano Lett2012;12: 2941–2947..

Stockman MI. Ultrafast nanoplasmonics under coherent control.New J Phys2008;10: 025031..

Fuchs U, Zeitner U, Tünnermann A. Ultra-short pulse propagation in complex optical systems.Opt Express2005;13: 3852–3861..

Trebino R. Measuring the seemingly immeasurable.Nat Photon2011;5: 189–192..

Iaconis C, Walmsley IA. Spectral phase interferometry for direct electric-field reconstruction of ultrashort optical pulses.Opt Lett1998;23: 792–794..

Coello Y, Lozovoy VV, Gunaratne TC, Xu B, Borukhovich Iet al. Interference without an interferometer: a different approach to measuring, compressing, and shaping ultrashort laser pulses.J Opt Soc Am B2008;25: A140–A150..

Xu B, Gunn JM, Cruz JM, Lozovoy VV, Dantus M. Quantitative investigation of the multiphoton intrapulse interference phase scan method for simultaneous phase measurement and compensation of femtosecond laser pulses.J Opt Soc Am B2006;23: 750–759..

Le Xuan L, Zhou C, Slablab A, Chauvat D, Tard Cet al. Photostable second-harmonic generation from a single KTiOPO4nanocrystal for nonlinear microscopy.Small2008;4: 1332–1336..

Extermann J, Bonacina L, Courvoisier F, Kiselev D, Mugnier Yet al. Nano-FROG: frequency resolved optical gating by a nanometric object.Opt Express2008;16: 10405–10411..

Li H, Zhang Z, Xu Q, Shi K, Jia Yet al. Characterizing ultrashort optical pulses using second-order nonlinear nanoprobes.Appl Phys Lett2010;97: 261108..

Wnuk P, Xuan LL, Slablab A, Tard C, Perruchas Set al. Coherent nonlinear emission from a single KTP nanoparticle with broadband femtosecond pulses.Opt Express2009;17: 4652–4658..

Aulbach J, Gjonaj B, Johnson P, Lagendijk A. Spatiotemporal focusing in opaque scattering media by wave front shaping with nonlinear feedback.Opt Express2012;20: 29237–29251..

Bäumner R, Bonacina L, Enderlein J, Extermann J, Fricke-Begemann Tet al. Evanescent-field-induced second harmonic generation by noncentrosymmetric nanoparticles.Opt Express2010;18: 23218–23225..

Berweger S, Atkin JM, Xu XG, Olmon RL, Raschke MB. Femtosecond nanofocusing with full optical waveform control.Nano Lett2011;11: 4309–4313..

Neumann L, Pang Y, Houyou A, Juan ML, Gordon Ret al. Extraordinary optical transmission brightens near-field fiber probe.Nano Lett2011;11: 355–360..

Staedler D, Magouroux T, Hadji R, Joulaud C, Extermann Jet al. Harmonic nanocrystals for biolabeling: a survey of optical properties and biocompatibility.ACS Nano2012;6: 2542–2549..

Bidault S, Polman A. Water-based assembly and purification of plasmon-coupled gold nanoparticle dimers and trimers.Int J Opt2012;2012: 387274..

Brinks D, Hildner R, Stefani FD, van Hulst NF. Beating spatio-temporal coupling: implications for pulse shaping and coherent control experiments.Opt Express2011;19: 26486–26499..

McCabe DJ, Austin DR, Tajalli A, Weber S, Walmsley IAet al. Space–time coupling of shaped ultrafast ultraviolet pulses from an acousto-optic programmable dispersive filter.J Opt Soc Am B2011;28: 58–64..

Pestov D, Lozovoy VV, Dantus M. Multiple Independent Comb Shaping (MICS): phase-only generation of optical pulse sequences.Opt Express2009;17: 14351–14361..

Butet J, Duboisset J, Bachelier G, Russier-Antoine I, Benichou Eet al. Optical second harmonic generation of single metallic nanoparticles embedded in a homogeneous medium.Nano Lett2010;10: 1717–1721..

Slablab A, Le Xuan L, Zielinski M, de Wilde Y, Jacques Vet al. Second-harmonic generation from coupled plasmon modes in a single dimer of gold nanospheres.Opt Express2012;20: 220–227..

Castro-Lopez M, Brinks D, Sapienza R, van Hulst NF. Aluminum for nonlinear plasmonics: resonance-driven polarized luminescence of Al, Ag, and Au nanoantennas.Nano Lett2011;11: 4674–4678..

Ghenuche P, Cherukulappurath S, Taminiau TH, van Hulst NF, Quidant R. Spectroscopic mode mapping of resonant plasmon nanoantennas.Phys Rev Lett2008;101: 116805..

Deng HD, Li GC, Dai QF, Ouyang M, Lan Set al. Size dependent competition between second harmonic generation and two-photon luminescence observed in gold nanoparticles.Nanotechnology2013;24: 075201..

Novotny L, van Hulst N. Antennas for light.Nat Photon2011;5: 83–90..

Brinks D, Castro-Lopez M, Hildner R, van Hulst NF. Plasmonic antennas as design elements for coherent ultrafast nanophotonics.Proc Natl Acad Sci USA2013;110: 18386–18390. doi: 10.1073/pnas.1308652110..

浏览量

Downloads

CSCD

文章被引用时，请邮件提醒。

Submit

工具集

关联资源

An ultrafast reconfigurable nanophotonic switch using wavefront shaping of light in a nonlinear nanomaterial

Spiniform phase-encoded metagratings entangling arbitrary rational-order orbital angular momentum

Microwatts continuous-wave pumped second harmonic generation in few- and mono-layer GaSe

Double-layer graphene for enhanced tunable infrared plasmonics

Rapid and robust control of single quantum dots