Quantum nonlocal effects in individual and interacting graphene nanoribbons
Original Articles|Updated:2024-09-26
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Quantum nonlocal effects in individual and interacting graphene nanoribbons
Quantum nonlocal effects in individual and interacting graphene nanoribbons
LSA2015年4卷第1期
Affiliations:
1.ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, 08860 Castelldefels (Barcelona), Spain
2.ICREA-Institució Catalana de Recerca i Estudis Avançats, Passeig Lluís Companys 23, 08010 Barcelona, Spain
Author bio:
Professor FJ García de Abajo, ICFO-Institut de Ciencies Fotoniques, Mediterranean Technology Park, 08860 Castelldefels (Barcelona), SpainE-mail: javier.garciadeabajo@icfo.es
Quantum nonlocal effects in individual and interacting graphene nanoribbons[J]. LSA, 2015,4(1).
Silveiro, I., Ortega, J. M. P. & de Abajo, F. J. G. Quantum nonlocal effects in individual and interacting graphene nanoribbons. Light: Science & Applications, 4, e241 (2015).
Quantum nonlocal effects in individual and interacting graphene nanoribbons[J]. LSA, 2015,4(1). DOI: 10.1038/lsa.2015.14.
Silveiro, I., Ortega, J. M. P. & de Abajo, F. J. G. Quantum nonlocal effects in individual and interacting graphene nanoribbons. Light: Science & Applications, 4, e241 (2015). DOI: 10.1038/lsa.2015.14.
Quantum nonlocal effects in individual and interacting graphene nanoribbons
We show that highly doped graphene ribbons can support surface plasmons at near-infrared frequencies when their width is in the nanometer range
leading to important nonlocal and finite quantum-size corrections
such as sizable blueshifts. The magnitude of these effects is assessed by comparing classical and quantum-mechanical models to describe graphene plasmons. More precisely
we examine individual and interacting 6–8 nm wide zigzag and armchair ribbons doped to 0.4–1.5 eV Fermi energies. We find a strong influence of nonlocal effects on the orientation of graphene edges
with plasmons in zigzag ribbons undergoing strong quenching when their energy is below the Fermi level. Nonlocality is also affecting the hybridization between ribbon plasmons in dimers and arrays for separations below a few nanometers. Remarkably
the removal of a single row of atomic bonds in a ribbon produces a strong plasmon frequency shift
whereas the removal of bonds along an array of rows separated by several nanometers in an extended sheet causes a dramatic increase in the absorption. Besides the fundamental interest of these results
our work supports the use of narrow ribbons to achieve electro-optical modulation in the near infrared.
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State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics, Sun Yat-sen University
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ICFO—Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology, Castelldefels (Barcelona)