A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection

Kui-Chao Liu; Zhen-Yi Zhang; Chong-Xin Shan; Zhi-Qing Feng; Jia-Su Li; Chun-Lei Song; Ya-Nan Bao; Xiao-Hui Qi; Bin Dong

doi:10.1038/lsa.2016.136

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A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection

Original Articles

- A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection
- A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection
- LSA 2016年5卷第3期
- Affiliations：
  
  1.Key Laboratory of New Energy and Rare Earth Resource Utilization of State Ethnic Affairs Commission, Dalian Nationalities University, 18 Liaohe West Road, Dalian 116600, China
  2.State Key Laboratory of Luminescence and Applications, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, Changchun 130033, China
  3.School of Physics and Engineering, Zhengzhou University, Zhengzhou 450001, China
- Author bio：
  
  ZY Zhang, Email: zhangzy@dlnu.edu.cn
  B Dong, Email: dong@dlnu.edu.cn
- Funds：
- DOI：10.1038/lsa.2016.136
  中图分类号：
- 纸质出版日期：2016-09，
  
  网络出版日期：2016-03-21，
  
  收稿日期：2015-11-02，
  
  修回日期：2016-03-06，
  
  录用日期：2016-03-10
- Accepted：
Scan QR Code
A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection[J]. LSA, 2016,5(3).

Liu, K. C. et al. A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection. Light: Science & Applications, 5, e16136 (2016).
A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection[J]. LSA, 2016,5(3). DOI： 10.1038/lsa.2016.136.

Liu, K. C. et al. A flexible and superhydrophobic upconversion-luminescence membrane as an ultrasensitive fluorescence sensor for single droplet detection. Light: Science & Applications, 5, e16136 (2016). DOI： 10.1038/lsa.2016.136.

摘要

Abstract

A Ln

-doped (Yb

or Yb

co-doped) NaYF

nanoparticle/polystyrene hybrid fibrous membrane (HFM) was fabricated using an electrospinning technique. The HFM shows upconversion luminescence (UCL)

flexibility

superhydrophobicity and processability. The UCL membrane can be used as a fluorescence sensor to detect bioinformation from a single water droplet (~10 μl). Based on the fluorescence resonance energy transfer

the detection limits of this sensor can reach 1 and 10 ppb for the biomolecule

avidin

and the dye molecule

Rhodamine B

respectively

which are superior to most of the fluorescence sensors reported in previous works. After the f

luorescence detection

the target droplet was easily removed without residues on the UCL membrane surface due to its superhydrophobic property

which exhibits an excellent recyclability that cannot be achieved by traditional liquid-based detection systems.

关键词

Keywords

electrospinningfibrous membranefluorescence resonance energy transferfluorescence sensorsuperhydrophobic surfaceupconversion luminescence

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