Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures

Shuki Enomoto; Tomoya Tagami; Yusuke Ueda; Yuta Moriyama; Kentaro Fujiwara; Shun Takahashi; Kenichi Yamashita

doi:10.1038/s41377-021-00701-8

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Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures

Articles

- Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures
- Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures
- LSA 2022年11卷第1期页码：79-86
- Affiliations：
  
  Faculty of Electrical Engineering and Electronics, Kyoto Institute of Technology, Matsugasaki, Sakyo-ku, Kyoto, 606-8585, Japan
- Author bio：
  
  Kenichi Yamashita (yamasita@kit.ac.jp)
- Funds：
- DOI：10.1038/s41377-021-00701-8
  中图分类号：
- 纸质出版日期：2022-01-31，
  
  网络出版日期：2022-01-02，
  
  收稿日期：2021-07-08，
  
  修回日期：2021-11-28，
  
  录用日期：2021-12-19
- Accepted：
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Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures[J]. LSA, 2022,11(1):79-86.

Enomoto, S. et al. Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures. Light: Science & Applications, 11, 79-86 (2022).
Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures[J]. LSA, 2022,11(1):79-86. DOI： 10.1038/s41377-021-00701-8.

Enomoto, S. et al. Drastic transitions of excited state and coupling regime in all-inorganic perovskite microcavities characterized by exciton/plasmon hybrid natures. Light: Science & Applications, 11, 79-86 (2022). DOI： 10.1038/s41377-021-00701-8.

摘要

Abstract

Lead-halide perovskites are highly promising for various optoelectronic applications

including laser devices. However

fundamental photophysics explaining the coherent-light emission from this material system is so intricate and often the subject of debate. Here

we systematically investigate photoluminescence properties of all-inorganic perovskite microcavity at room temperature and discuss the excited state and the light–matter coupling regime depending on excitation density. Angle-resolved photoluminescence clearly exhibits that the microcavity system shows a transition from weak coupling regime to strong coupling regime

revealing the increase in correlated electron–hole pairs. With pumping fluence above the threshold

the photoluminescence signal shows a lasing behavior with bosonic condensation characteristics

accompanied by long-range phase coherence. The excitation density required for the lasing behavior

however

is found to exceed the Mott density

excluding the exciton as the excited state. These results demonstrate that the polaritonic Bardeen–Cooper–Schrieffer state originates the strong coupling formation and the lasing behavior.

关键词

Keywords

references

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