Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas

R. Margoth Córdova-Castro; Bart van Dam; Alberto Lauri; Stefan A. Maier; Riccardo Sapienza; Yannick De Wilde; Ignacio Izeddin; Valentina Krachmalnicoff

doi:10.1038/s41377-023-01349-2

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Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas

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- Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas
- Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas
- LSA 2024年13卷第1期页码：47-54
- Affiliations：
- Author bio：
  
  gignacio.izeddin@espci.fr
  hvalentina.krachmalnicoff@espci.fr
- Funds：
  
  Agence Nationale de la Recherche (French National Research Agency);RCUK | Engineering and Physical Sciences Research Council (EPSRC)
- DOI：10.1038/s41377-023-01349-2
  中图分类号：
- 收稿日期：2023-06-27，
  
  修回日期：2023-11-20，
  
  录用日期：2023-11-29，
  
  网络出版日期：2024-01-02，
  
  纸质出版日期：2024-12
- Accepted：
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Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas[J]. LSA, 2024,13(1):47-54.

R. Margoth Córdova-Castro, Bart van Dam, Alberto Lauri, et al. Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas[J]. Light: science & applications, 2024, 13(1): 47-54.
Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas[J]. LSA, 2024,13(1):47-54. DOI： 10.1038/s41377-023-01349-2.

R. Margoth Córdova-Castro, Bart van Dam, Alberto Lauri, et al. Single-emitter super-resolved imaging of radiative decay rate enhancement in dielectric gap nanoantennas[J]. Light: science & applications, 2024, 13(1): 47-54. DOI： 10.1038/s41377-023-01349-2.

摘要

Abstract

High refractive index dielectric nanoantennas strongly modify the decay rate via the Purcell effect through the design of radiative channels. Due to their dielectric nature

the field is mainly confined inside the nanostructure and in the gap

which is hard to probe with scanning probe techniques. Here we use single-molecule fluorescence lifetime imaging microscopy (smFLIM) to map the decay rate enhancement in dielectric GaP nanoantenna dimers with a median localization precision of 14 nm. We measure

in the gap of the nanoantenna

decay rates that are almost 30 times larger than on a glass substrate. By comparing experimental results with numerical simulations we show that this large enhancement is essentially radiative

contrary to the case of plasmonic nanoantennas

and therefore has great potential for applications such as quantum optics and biosensing.

Single-molecule fluorescence lifetime imaging microscopy (smFLIM) measures the radiative decay rate of single molecules in the near field of dielectric nanoantennas providing super-resolved information of the local density of states.

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references

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