Cavity-enhanced photoacoustic dual-comb spectroscopy

Zhen Wang; Qinxue Nie; Haojia Sun; Qiang Wang; Simone Borri; Paolo De Natale; Wei Ren

doi:10.1038/s41377-023-01353-6

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Cavity-enhanced photoacoustic dual-comb spectroscopy

Original Articles

- Cavity-enhanced photoacoustic dual-comb spectroscopy
- Cavity-enhanced photoacoustic dual-comb spectroscopy
- LSA 2024年13卷第4期页码：610-618
- Affiliations：
  
  1.Department of Mechanical and Automation Engineering, The Chinese University of Hong Kong, New Territories, Hong Kong SAR, China
  2.State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences, 130033 Changchun, China
  3.CNR-INO—Istituto Nazionale di Ottica, and LENS—European Laboratory for Nonlinear Spectroscopy, 50019 Sesto Fiorentino, Italy
- Author bio：
  
  Zhen Wang (wangzhen@link.cuhk.edu.hk)
  Qiang Wang (wangqiang@ciomp.ac.cn)
  Wei Ren (renwei@mae.cuhk.edu.hk)
- Funds：
- DOI：10.1038/s41377-023-01353-6
  中图分类号：
- 收稿日期：2023-08-01，
  
  修回日期：2023-12-01，
  
  录用日期：2023-12-07，
  
  网络出版日期：2024-01-05，
  
  纸质出版日期：2024-04-30
- Accepted：
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Cavity-enhanced photoacoustic dual-comb spectroscopy[J]. LSA, 2024,13(4):610-618.

Wang, Z. et al. Cavity-enhanced photoacoustic dual-comb spectroscopy. Light: Science & Applications, 13, 610-618 (2024).
Cavity-enhanced photoacoustic dual-comb spectroscopy[J]. LSA, 2024,13(4):610-618. DOI： 10.1038/s41377-023-01353-6.

Wang, Z. et al. Cavity-enhanced photoacoustic dual-comb spectroscopy. Light: Science & Applications, 13, 610-618 (2024). DOI： 10.1038/s41377-023-01353-6.

摘要

Abstract

Photoacoustic dual-comb spectroscopy (DCS)

converting spectral information in the optical frequency domain to the audio frequency domain via multi-heterodyne beating

enables background-free spectral measurements with high resolution and broad bandwidth. However

the detection sensitivity remains limited due to the low power of individual comb lines and the lack of broadband acoustic resonator

s. Here

we develop cavity-enhanced photoacoustic DCS

which overcomes these limitations by using a high-finesse optical cavity for the power amplification of dual-frequency combs and a broadband acoustic resonator with a flat-top frequency response. We demonstrate high-resolution spectroscopic measurements of trace amounts of C

and CO in the entire telecommunications C-band. The method shows a minimum detection limit of 0.6 ppb C

at the measurement time of 100 s

corresponding to the noise equivalent absorption coefficient of 7 × 10

−10

−1

. The proposed cavity-enhanced photoacoustic DCS may open new avenues for ultrasensitive

high-resolution

and multi-species gas detection with widespread applications.

关键词

Keywords

references

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