Observation of transition from superfluorescence to polariton condensation in CsPbBr<sub>3</sub> quantum dots film

Danqun Mao; Linqi Chen; Zheng Sun; Min Zhang; Zhe-Yu Shi; Yongsheng Hu; Long Zhang; Jian Wu; Hongxing Dong; Wei Xie; Hongxing Xu

doi:10.1038/s41377-024-01378-5

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Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film

Original Articles

- Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film
- Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film
- LSA 2024年13卷第2期页码：316-324
- Affiliations：
  
  1.State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China
  2.Key Laboratory of Materials for High-Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, 201800 Shanghai, China
  3.Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, China
  4.Chongqing Key Laboratory of Precision Optics, Chongqing Institute of East China Normal University, Chongqing 401121, China
  5.CAS Center for Excellence in Ultra-intense Laser Science, Shanghai 201800, China
  6.School of Physics and Technology, Center for Nanoscience and Nanotechnology, Wuhan University, Wuhan 430072, China
- Author bio：
  
  Zheng Sun (zsun@lps.ecnu.edu.cn)
  Hongxing Dong (hongxingd@siom.ac.cn)
  Wei Xie (wxie@phy.ecnu.edu.cn)
- Funds：
- DOI：10.1038/s41377-024-01378-5
  中图分类号：
- 收稿日期：2023-07-04，
  
  修回日期：2023-12-19，
  
  录用日期：2024-01-03，
  
  网络出版日期：2024-01-30，
  
  纸质出版日期：2024-02-29
- Accepted：
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Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film[J]. LSA, 2024,13(2):316-324.

Mao, D. Q. et al. Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film. Light: Science & Applications, 13, 316-324 (2024).
Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film[J]. LSA, 2024,13(2):316-324. DOI： 10.1038/s41377-024-01378-5.

Mao, D. Q. et al. Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film. Light: Science & Applications, 13, 316-324 (2024). DOI： 10.1038/s41377-024-01378-5.

摘要

Abstract

The superfluorescence effect has received extensive attention due to the many-body physics of quantum correlation in dipole gas and the optical applications of ultrafast bright radiation field based on the cooperative quantum state. Here

we demonstrate not only to observe the superfluorescence effect but also to control the cooperative state of the excitons ensemble by externally applying a regulatory dimension of coupling light fields. A new quasi-particle called cooperative exciton-polariton is revealed in a light-matter hybrid structure of a perovskite quantum dot thin film spin-coated on a Distributed Bragg Reflector. Above the nonlinear threshold

polaritonic condensation occurs at a nonzero momentum state on the lower polariton branch owning to the vital role of the synchronized excitons. The phase transition from superfluorescence to polariton condensation exhibits typical signatures of a decrease of the linewidth

an increase of the macroscopic coherence as well as an accelerated radiation decay rate. These findings are promising for opening new potential applications for super-brightness and unconventional coherent light sources and could enable the exploitation of cooperative effects for quantum optics.

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references

Bonifacio, R. & Lugiato, L. A. Cooperative radiation processes in two-level systems: superfluorescence. Phys. Rev. A 11 , 1507–1521 (1975)..

Cong, K. K. et al. Dicke superradiance in solids [Invited ] . J. Opt. Soc. Am. B 33 , C80–C101 (2016)..

Dicke, R. H. Coherence in spontaneous radiation processes. Phys. Rev. 93 , 99–110 (1 954)..

Dai, D. C. & Monkman, A. P. Observation of superfluorescence from a quantum ensemble of coherent excitons in a ZnTe crystal: Evidence for spontaneous Bose-Einstein condensation of excitons. Phys. Rev. B 84 , 115206 (2011)..

Malcuit, M. S. et al. Transition from superfluorescence to amplified spontaneous emission. Phys. Rev. Lett. 59 , 1189–1192 (1987)..

Skribanowitz, N. et al. Observation of Dicke superradiance in optically pumped HF gas. Phys. Rev. Lett. 30 , 309–312 (1973)..

Chu, L., Zhang, L. X. & Ding, L. M. Superfluorescence from halide perovskite nanocrystal superlattices. J. Semicond. 43 , 100202 (2022)..

Cherniukh, I. et al. Perovskite-type superlattices from lead halide perovskite nanocubes. Nature 593 , 535–542 (2021)..

Zhou, C. et al. Cooperative excitonic quantum ensemble in perovskite-assembly superlattice microcavities. Nat. Commun. 11 , 329 (2020)..

Rainò, G. et al. Superfluorescence from lead halide perovskite quantum dot superlattices. Nature 563 , 671–675 (2018)..

Biliroglu, M. et al. Room-temperature superfluorescence in hybrid perovskites and its origins. Nat. Photon. 16 , 324–329 (2022)..

Chen, J. et al. Perovskite quantum dot lasers. InfoMat 2 , 170–183 (2020)..

Zhang, L. et al. Photonic-crystal exciton-polaritons in monolayer semiconductors. Nat. Commun. 9 , 713 (2018)..

Fieramosca, A. et al. Two-dimensional hybrid perovskites sustaining strong polariton interactions at room temperature. Sci. Adv. 5 , eaav9967 (2019)..

Shang, Q. Y. et al. Role of the exciton-polariton in a continuous-wave optically pumped CsPbBr 3 perovskite Laser. Nano Lett. 20 , 6636–6643 (2020)..

Song, J. P. et al. Continuous‐wave pumped perovskite lasers with device area below 1 μm2. Adv. Mater. 35 , 2302170 (2023)..

Huang, C. Y. et al. CsPbBr 3 perovskite quantum dot vertical cavity lasers with low threshold and high stability. ACS Photon. 4 , 2281–2289 (2017)..

Su, X. Q. et al. Surface vertical multi-emission laser with distributed Bragg reflector feedback from CsPbI 3 quantum dots. Nano. Mater. 13 , 1669 (2023)..

Zhang, H. B. et al. Stable continuous-wave lasing from discrete cesium lead bromide quantum dots embedded in a microcavity. Nano. Horiz. 8 , 1403–1410 (2023)..

Wang, Y. et al. Solution‐processed low threshold vertical cavity surface emitting lasers from all‐inorganic perovskite nanocrystals. Adv. Funct. Mater. 27 , 1605088 (2017)..

Yen, M. C. et al. Tamm-plasmon exciton-polaritons in single-monolayered CsPbBr 3 quantum dots at room temperature. Adv. Opt. Mater. 11 , 2202326 (2023)..

Kasprzak, J. et al. Bose–Einstein condensation of exciton polaritons. Nature 443 , 409–414 (2006)..

Byrnes, T., Kim, N. Y. & Yamamoto, Y. Exciton–polariton condensates. Nat. Phys. 10 , 803–813 (2014)..

Ramezani, M. et al. Plasmon-exciton-polariton lasing. Optica 4 , 31–37 (2017)..

Balili, R. et al. Bose-einstein condensation of microcavity polaritons in a trap. Science 316 , 1007–1010 (2007)..

Su, R. et al. Observation of exciton polariton condensation in a perovskite lattice at room temperature. Nat. Phys. 16 , 301–306 (2020)..

Wang, C. Y. et al. Engineering giant Rabi splitting via strong coupling between localized and propagating Plasmon modes on metal surface lattices: observation of √f scaling rule. Nano Lett. 21 , 605–611 (2021)..

Wang, B., Zeng, X. Z. & Li, Z. Y. Quantum versus optical interaction contribution to giant spectral splitting in a strongly coupled Plasmon-molecules system. Photon. Res. 8 , 343–351 (2020)..

Khitrova, G. et al. Vacuum Rabi splitting in semiconductors. Nat. Phys. 2 , 81–90 (2006)..

Debnath, S. et al. Demonstration of a small programmable quantum computer with atomic qubits. Nature 536 , 63–66 (2016)..

Chertkov, E. et al. Holographic dynamics simulations with a trapped-ion quantum computer. Nat. Phys. 18 , 1074–1079 (2022)..

Kavokin, A. et al. Polariton condensates for classical and quantum computing. Nat. Rev. Phys. 4 , 435–451 (2022)..

Chen, H. Q. et al. Room-temperature polariton lasing in GaN microrods with large Rabi splitting. Opt. Expr. 30 , 16794–16801 (2022)..

Zhang, L. et al. Recent developments on polariton lasers. Prog. Quant. Electron. 83 , 100399 (2022)..

Du, W. N. et al. Strong exciton-photon coupling and lasing behavior in all-inorganic CsPbBr 3 micro/nanowire Fabry-Perot cavity. ACS Photon. 5 , 2051–2059 (2018)..

Su, R. et al. Room-temperature polariton lasing in all-inorganic perovskite nanoplatelets. Nano Lett. 17 , 3982–3988 (2017 )..

Chen, F. et al. Optically controlled femtosecond polariton switch at room temperature. Phys. Rev. Lett. 129 , 057402 (2022)..

Feng, J. G. et al. All-optical switching based on interacting exciton polaritons in self-assembled perovskite microwires. Sci. Adv. 7 , eabj6627 (2021)..

Moilanen, A. J. et al. Mode switching dynamics in organic polariton lasing. Phys. Rev. B 106 , 195403 (2022)..

Ye, Y. et al. Monolayer excitonic laser. Nat. Photon. 9 , 733–737 (2015)..

Su, R. et al. Perovskite semiconductors for room-temperature exciton-polaritonics. Nat. Mater. 20 , 1315–1324 (2021)..

Kena-Cohen, S. & Forrest, S. R. Room-temperature polariton lasing in an organic single-crystal microcavity. Nat. Photon. 4 , 371–375 (2010)..

Wang, X. et al. Observation of Bragg polaritons in monolayer tungsten disulphide. Nano Res. 15 , 1479–14 85 (2022)..

Askitopoulos, A. et al. Bragg polaritons: strong coupling and amplification in an unfolded microcavity. Phys. Rev. Lett. 106 , 076401 (2011)..

Dong, H. et al. Metal halide perovskite for next-generation optoelectronics: progresses and prospects. eLight 3 , 3 (2023)..

Li, C. et al. Arbitrarily structured quantum emission with a multifunctional metalens. eLight 3 , 19 (2023)..

Delfanazari, K. et al. Integrated, portable, tunable, and coherent terahertz sources and sensitive detectors based on layered superconductors. Proc. IEEE 108 , 721–734 (2020)..

Najda, S. P. et al. GaN laser diodes for quantum sensors, clocks, systems and computing. Quantum Information Science, Sensing, and Computation XI 109–406 (SPIE, 2019).

Savona, V. et al. Quantum well excitons in semiconductor microcavities: unified treatment of weak and strong coupling regimes. Solid State Commun. 93 , 733–739 (1995)..

Ates, S. et al. Post-selected indistinguishable photons from the resonance fluorescence of a single quantum dot in a microcavity. Phys. Rev. Lett. 103 , 167402 (2009)..

Press, D. et al. Photon antibunching from a single quantum-dot-microcavity system in the strong coupling regime. Phys. Rev. Lett. 98 , 117402 (2007)..

Hennessy, K. et al. Quantum nature of a strongly coupled single quantum dot–cavity system. Nature 445 , 896–899 (2007)..

Ohadi, H. et al. Nontrivial phase coupling in polariton multiplets. Phys. Rev. X 6 , 031032 (2016)..

Wouters, M., Carusotto, I. & Ciuti, C. Spatial and spectral shape of inhomogeneous nonequilibrium exciton-polariton condensates. Phys. Rev. B 77 , 115340 (2008)..

Protesescu, L. et al. Nanocrystals of cesium lead halide perovskites (CsPbX 3 , X = Cl, Br, and I): novel optoelectronic materials showing bright emission with wide color gamut. Nano Lett. 15 , 3692–3696 (2015)..

Fetter, A. L. & Walecka, J. D. Quant um theory of many-particle systems. Phys. Today 25 (11), 54–55 (1972)..

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Observation of transition from superfluorescence to polariton condensation in CsPbBr3 quantum dots film

Observation of transition from superfluorescence to polariton condensation in CsPbBr3 quantum dots film

DOI：10.1038/s41377-024-01378-5

摘要

Abstract

关键词

Keywords

references

Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film

Observation of transition from superfluorescence to polariton condensation in CsPbBr₃ quantum dots film