1.Department of Physics, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
2.School of Physics and Engineering, ITMO University, Saint Petersburg 197101, Russia
Kyoung-Duck Park (parklab@postech.ac.kr)
收稿日期:2023-08-28,
修回日期:2023-11-26,
录用日期:2024-01-10,
网络出版日期:2024-01-25,
纸质出版日期:2024-02-29
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Dynamical control of nanoscale light-matter interactions in low-dimensional quantum materials[J]. LSA, 2024,13(2):236-253.
Koo, Y. et al. Dynamical control of nanoscale light-matter interactions in low-dimensional quantum materials. Light: Science & Applications, 13, 236-253 (2024).
Dynamical control of nanoscale light-matter interactions in low-dimensional quantum materials[J]. LSA, 2024,13(2):236-253. DOI: 10.1038/s41377-024-01380-x.
Koo, Y. et al. Dynamical control of nanoscale light-matter interactions in low-dimensional quantum materials. Light: Science & Applications, 13, 236-253 (2024). DOI: 10.1038/s41377-024-01380-x.
Tip-enhanced nano-spectroscopy and -imaging have significantly advanced our understanding of low-dimensional quantum materials and their interactions with light
providing a rich insight into the underlying physics at their natural length scale. Recently
various functionalities of the plasmonic tip expand the capabilities of the nanoscopy
enabling dynamic manipulation of light-matter interactions at the nanoscale. In this review
we focus on a new paradigm of the nanoscopy
shifting from the conventional role of imaging and spectroscopy to the dynamical control approach of the tip-induced light-matter interactions. We present three different approaches of tip-induced control of light-matter interactions
such as cavity-gap control
pressure control
and near-field polarization control. Specifically
we discuss the nanoscale modifications of radiative emissions for various emitters from weak to strong coupling regime
achieved by the precise engineering of the cavity-gap. Furthermore
we introduce recent works on light-matter interactions controlled by tip-pressure and near-field polarization
especially tunability of the bandgap
crystal structure
photoluminescence quantum yield
exciton density
and energy transfer in a wide range of quantum materials. We envision that this comprehensive review not only contributes to a deeper understanding of the physics of nanoscale light-matter interactions but also offers a valuable resource to nanophotonics
plasmonics
and materials science for future technological advancements.
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