Multi-parameter control of photodetection in van der Waals magnet CrSBr

Shiqi Yang; Zhigang Song; Yuchen Gao; Leyan Huang; Xinyue Huang; Pingfan Gu; Wenjing Liu; Zuxin Chen; Yu Ye

doi:10.1038/s41377-024-01737-2

Go to Nature Website

Your Location：

Home >

Browse articles >

Multi-parameter control of photodetection in van der Waals magnet CrSBr

Original Articles

- Multi-parameter control of photodetection in van der Waals magnet CrSBr
- Multi-parameter control of photodetection in van der Waals magnet CrSBr
- LSA 2025年14卷第3期页码：713-720
- Affiliations：
  
  1.State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, China
  2.John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA
  3.Academy for Advanced Interdisciplinary Studies, Peking University, Beijing 100871, China
  4.School of Semiconductor Science and Technology, South China Normal University, Foshan 528225, China
  5.Collaborative Innovation Centre of Quantum Matter, Beijing 100871, China
  6.Yangtze Delta Institute of Optoelectronics, Peking University, Nantong 226010 Jiangsu, China
  7.Liaoning Academy of Materials, Shenyang 110167, China
- Author bio：
  
  Yu Ye (ye_yu@pku.edu.cn)
- Funds：
- DOI：10.1038/s41377-024-01737-2
  中图分类号：
- 收稿日期：2024-10-10，
  
  修回日期：2024-12-09，
  
  录用日期：2024-12-27，
  
  网络出版日期：2025-02-03，
  
  纸质出版日期：2025-03-31
- Accepted：
Scan QR Code
Multi-parameter control of photodetection in van der Waals magnet CrSBr[J]. LSA, 2025,14(3):713-720.

Yang, S. Q. et al. Multi-parameter control of photodetection in van der Waals magnet CrSBr. Light: Science & Applications, 14, 713-720 (2025).
Multi-parameter control of photodetection in van der Waals magnet CrSBr[J]. LSA, 2025,14(3):713-720. DOI： 10.1038/s41377-024-01737-2.

Yang, S. Q. et al. Multi-parameter control of photodetection in van der Waals magnet CrSBr. Light: Science & Applications, 14, 713-720 (2025). DOI： 10.1038/s41377-024-01737-2.

摘要

Abstract

Photodetectors equipped with multi-parameter control hold the potential to deliver exceptional performance in a wide range of scenarios

paving the way for developing novel spin-opto-electronic devices. Nevertheless

the integration of such capabilities within a single device is challenging due to the necessity of harmonizing multiple materials with varying degrees of freedom. In this study

we introduce the van der Waals magnet CrSBr

featuring inherent anisotropy and distinctive spin-electronic coupling

to this realm. The linear dichroic ratio of the photocurrent in CrSBr tunneling device can reach ~60 at 1.65 K

and the photoresponse experiences a significant boost with increasing magnetic field. Additionally

the unique spin-charge coupling engenders a photon energy-dependent photocurrent that is modulated by an external field and is validated by first-principle calculations. Our findings elucidate the effective multi-parameter control of photodetection based on vdWs magnet CrSBr

highlighting its potential applications in cutting-edge optoelectronic devices and as a highly sensitive probe medium.

关键词

Keywords

references

de Vasconcellos, S. M. et al. Coherent control of a single exciton qubit by optoelectronic manipulation. Nat. Photonics 4 , 545–548 (2010)..

Mak, K. F., Xiao, D. & Shan, J. Light–valley interactions in 2D semiconductors. Nat. Photonics 12 , 451–460 (2018)..

Lyons, T. P. et al. Giant effective Zeeman splitting in a monolayer semiconductor realized by spin-selective strong light–matter coupling. Nat. Photonics 16 , 632–636 (2022)..

Yang, C. L. et al. Spectral dependence of spin photocurrent and current-induced spin polarization in an InGaAs/InAlAs two-dimensional electron gas. Phys. Rev. Lett. 96 , 186605 (2006)..

Gottscholl, A. et al. Spin defects in hBN as promising temperature, pressure and magnetic fie ld quantum sensors. Nat. Commun. 12 , 4480 (2021)..

Zhang, T. et al. A monolithically sculpted van der Waals nano-opto-electro-mechanical coupler. Light Sci. Appl. 11 , 48 (2022)..

Sheng, Z. G. et al. Magneto-tunable photocurrent in manganite-based heterojunctions. Nat. Commun. 5 , 4584 (2014)..

Matsubara, M. et al. Polarization-controlled tunable directional spin-driven photocurrents in a magnetic metamaterial with threefold rotational symmetry. Nat. Commun. 13 , 6708 (2022)..

Singh, S. & Khare, N. Low field magneto-tunable photocurrent in CoFe 2 O 4 nanostructure films for enhanced photoelectrochemical properties. Sci. Rep. 8 , 6522 (2018)..

McIver, J. W. et al. Control over topological insulator photocurrents with light polarization. Nat. Nanotechnol. 7 , 96–100 (2012)..

Semonin, O. E. et al. Peak external photocurrent quantum efficiency exceeding 100% via MEG in a quantum dot solar cell. Science 334 , 1530–1533 (2011)..

Yu, W. J. et al. Highly efficient gate-tunable photocurrent generation in vertical heterostructures of layered materials. Nat. Nanotechnol. 8 , 952–958 (2013)..

Gill, R., Zayats, M. & Willner, I. Semiconductor quantum dots for bioanalysis. Angew. Chem. Int. Ed. 47 , 7602–7625 (2008)..

Yuan, H. T. et al. Polarization-sensitive broadband photodetector using a black phosphorus vertical p–n junction. Nat. Nanotechnol. 10 , 707–713 (2015)..

Song, T. C. et al. Spin photovoltaic effect in magnetic van der Waals heterostructures. Sci. Adv. 7 , eabg8094 (2021)..

Cheng, X. et al. Light helicity detector based on 2D magnetic semiconductor CrI3. Nat. Commun. 12 , 6874 (2021)..

Göse, O., Paul, W. & Kahle, H. Magnetic properties of CrSBr. J. Magn. Magn. Mater. 92 , 129–136 (1990)..

Yang, K. et al. Triaxial magnetic anisotropy in the two-dimensional ferromagnetic semiconductor CrSBr. Phys. Rev. B 104 , 1444 16 (2021)..

Telford, E. J. et al. Layered antiferromagnetism induces large negative magnetoresistance in the van der Waals semiconductor CrSBr. Adv. Mater. 32 , 2003240 (2020)..

Lee, K. et al. Magnetic order and symmetry in the 2D semiconductor CrSBr. Nano Lett. 21 , 3511–3517 (2021)..

Wilson, N. P. et al. Interlayer electronic coupling on demand in a 2D magnetic semiconductor. Nat. Mater. 20 , 1657–1662 (2021)..

Wang, T. T. et al. Magnetically-dressed CrSBr exciton-polaritons in ultrastrong coupling regime. Nat. Commun. 14 , 5966 (2023)..

Dirnberger, F. et al. Magneto-optics in a van der Waals magnet tuned by self-hybridized polaritons. Nature 620 , 533–537 (2023)..

Bae, Y. J. et al. Exciton-coupled coherent magnons in a 2D semiconductor. Nature 609 , 282–286 (2022)..

Diederich, G. M. et al. Tunable interaction between excitons and hybridized magnons in a layered semicond uctor. Nat. Nanotechnol. 18 , 23–28 (2023)..

Cenker, J. et al. Reversible strain-induced magnetic phase transition in a van der Waals magnet. Nat. Nanotechnol. 17 , 256–261 (2022)..

Pawbake, A. et al. Magneto-optical sensing of the Pres 8 sure driven magnetic ground states in bulk CrSBr. Nano Lett. 23 , 9587–9593 (2023)..

Song, T. C. et al. Giant tunneling magnetoresistance in spin-filter van der Waals heterostructures. Science 360 , 1214–1218 (2018)..

Wang, Z. et al. Very large tunneling magnetoresistance in layered magnetic semiconductor CrI3. Nat. Commun. 9 , 2516 (2018)..

Klein, D. R. et al. Probing magnetism in 2D van der Waals crystalline insulators via electron tunneling. Science 360 , 1218–1222 (2018)..

Yang, D. Y. et al. Spontaneous-polarization-induced photovoltaic effect in rhombohedrally stacked MoS 2 . Nat. Photonics 16 , 469–474 (2022)..

Yu, W. J. et al. Unusually efficient photocurrent extraction in monolayer van der Waals heterostructure by tunnelling through discretized barriers. Nat. Commun. 7 , 13278 (2016)..

Li, L. F. et al. Plasmon excited ultrahot carriers and negative differential photoresponse in a vertical graphene van der Waals heterostructure. Nano Lett. 19 , 3295–3304 (2019)..

Klein, J. et al. The bulk van der Waals layered magnet CrSBr is a quasi-1D material. ACS Nano 17 , 5316–5328 (2023)..

Wang, C. et al. A family of high-temperature ferromagnetic monolayers with locked spin-dichroism-mobility anisotropy: MnNX and CrCX (X= Cl, Br, I; C= S, Se, Te). Sci. Bull. 64 , 293–300 (2019)..

Klein, J. et al. Sensing the local magnetic environment through optically active defects in a layered magnetic semiconductor. ACS Nano 17 , 288–299 (2023)..

Liu, C. H. et al. Graphene photodetectors with ultra-broadband and high responsivity at room temperature. Nat. Nanotechnol. 9 , 273–278 (2014)..

Yin, Z. Y. et al. Single-l ayer MoS 2 phototransistors. ACS Nano 6 , 74–80 (2012)..

Buscema, M. et al. Photocurrent generation with two-dimensional van der Waals semiconductors. Chem. Soc. Rev. 44 , 3691–3718 (2015)..

Zhou, Z. Q. et al. Perpendicular optical reversal of the linear dichroism and polarized photodetection in 2D GeAs. ACS Nano 12 , 12416–12423 (2018)..

Zhang, E. Z. et al. Tunable ambipolar polarization-sensitive photodetectors based on high-anisotropy ReSe2 nanosheets. ACS Nano 10 , 8067–8077 (2016)..

Zhang, Z. D. et al. Anisotropic photoresponse of layered 2D SnS-based near infrared photodetectors. J. Mater. Chem. C. 5 , 11288–11293 (2017)..

Ran, W. H. et al. Integrated polarization-sensitive amplification system for digital information transmission. Nat. Commun. 12 , 6476 (2021)..

Wang, X. T. et al. Short-wave near-infrared linear dichroism of two-dimensional germanium selenide. J. Am. Chem. Soc. 139 , 14976–14982 (2017)..

Tian, Z. et al. Two-dimensional SnS: a phosphorene analogue with strong in-plane electronic anisotropy. ACS Nano 11 , 2219–2226 (2017)..

Chen, W. L. et al. Strong in-plane optoelectronic anisotropy and polarization sensitivity in low-symmetry 2D violet phosphorus. Nano Lett. 23 , 10821–10831 (2023)..

浏览量

Downloads

CSCD

文章被引用时，请邮件提醒。

Submit

工具集

关联资源

暂无数据