1.State Key Laboratory of Materials for Integrated Circuits and Key Laboratory of Terahertz Solid State Technology, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China
2.Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China
3.Chongqing Key Laboratory of Precision Optics, Chongqing Institute of East China Normal University, Chongqing 401120, China
4.State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200241, China
5.Institute of Engineering, Tokyo University of Agriculture and Technology, Koganei-shi 184-8588 Tokyo, Japan
Heping Zeng (hpzeng@phy.ecnu.edu.cn)
Hua Li (hua.li@mail.sim.ac.cn)
收稿日期:2024-07-21,
修回日期:2025-02-12,
录用日期:2025-03-08,
网络出版日期:2025-03-31,
纸质出版日期:2025-04-30
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Farey tree locking of terahertz quantum cascade laser frequency combs[J]. LSA, 2025,14(4):1156-1168.
Liu, G. B. et al. Farey tree locking of terahertz quantum cascade laser frequency combs. Light: Science & Applications, 14, 1156-1168 (2025).
Farey tree locking of terahertz quantum cascade laser frequency combs[J]. LSA, 2025,14(4):1156-1168. DOI: 10.1038/s41377-025-01819-9.
Liu, G. B. et al. Farey tree locking of terahertz quantum cascade laser frequency combs. Light: Science & Applications, 14, 1156-1168 (2025). DOI: 10.1038/s41377-025-01819-9.
Frequency combs show various applications in molecular fingerprinting
imaging
communications
and so on. In the terahertz frequency range
semiconductor-based quantum cascade lasers (QCLs) are ideal platforms for realizing the frequency comb operation. Although self-started frequency comb operation can be obtained in free-running terahertz QCLs due to the four-wave mixing locking effects
resonant/off-resonant microwave injection
phase locking
and femtosecond laser based locking techniques have been widely used to broaden and stabilize terahertz QCL combs. These active locking methods indeed show significant effects on the frequency stabilization of terahertz QCL combs
but they simultaneously have drawbacks
such as introducing large phase noise and requiring complex optical coupling and/or electrical circuits. Here
we demonstrate Farey tree locking of terahertz QCL frequency combs under microwave injection. The frequency competition between the Farey fraction frequency and the cavity round-trip frequency results in the frequency locking of terahertz QCL combs
and the Farey fraction frequencies can be accurately anticipated based on the downward trend of the Farey tree hierarchy. Furthermore
dual-comb experimental results show that the phase noise of the dual-comb spectral lines is significantly reduced by employing the Farey tree locking method. These results pave the way to deploying compact and low phase noise terahertz frequency comb sources.
Udem, T., Holzwarth, R. & Hänsch, T. W. Optical frequency metrology. Nature 416 , 233–237 (2002)..
Diddams, S. A., Hollberg, L. & Mbele, V. Molecular fingerprinting with the resolved modes of a femtosecond laser frequency comb. Nature 445 , 627–630 (2007)..
Ideguchi, T. et al. Coherent Raman spectro-imaging with laser frequency combs. Nature 502 , 355–358 (2013)..
Marin-Palomo, P. et al. Microresonator-based solitons for massively parallel coherent optical communi cations. Nature 546 , 274–279 (2017)..
Yang, Q. F. et al. Efficient microresonator frequency combs. eLight 4 , 18 (2024)..
Yao, B. C. et al. Interdisciplinary advances in microcombs: bridging physics and information technology. eLight 4 , 19 (2024)..
Faist, J. etal. Quantum cascade laser. Science 264 , 553–556 (1994)..
Köhler, R. et al. Terahertz semiconductor-heterostructure laser. Nature 417 , 156–159 (2002)..
Zhuo, N., Liu, F. Q. & Wang, Z. G. Quantum cascade lasers: from sketch to mainstream in the mid and far infrared. J. Semicond. 41 , 010301 (2020)..
Li, R. S. et al. High brightness terahertz quantum cascade laser with near-diffraction-limited Gaussian beam. Light Sci. Appl. 13 , 193 (2024)..
Burghoff, D. et al. Terahertz laser frequency combs. Nat. Photonics 8 , 462–467 (2014)..
Zhou, K. et al. Ridge width effect on comb operation in terahertz quantum cascade lasers. Appl. Phys. Lett. 114 , 191106 (2019)..
Wang, F. H. et al. Short terahertz pulse generation from a dispersion compensated modelocked semiconductor laser. Laser Photonics Rev. 11 , 1700013 (2017)..
Bowers, J. E. et al. Actively mode-locked semiconductor lasers. IEEE J. Quantum Electron. 25 , 1426–1439 (1989)..
Gellie, P. et al. Injection-locking of terahertz quantum cascade lasers up to 35GHz using RF amplitude modulation. Opt. Express 18 , 20799–20816 (2010)..
Wan, W. J. et al. Homogeneous spectral spanning of terahertz semiconductor lasers with radio frequency modulation. Sci. Rep. 7 , 44109 (2017)..
Hillbrand, J. et al. Coherent injection locking of quantum casc ade laser frequency combs. Nat. Photonics 13 , 101–104 (2019)..
Li, Z. P. et al. On-chip dual-comb source based on terahertz quantum cascade lasers under microwave double injection. Phys. Rev. Appl. 12 , 044068 (2019)..
Forrer, A. et al. Photon-driven broadband emission and frequency comb RF injection locking in THz quantum cascade lasers. ACS Photonics 7 , 784–791 (2020)..
Liao, X. Y. et al. Broadband terahertz quantum cascade laser dual-comb sources under off-resonant microwave injection. Adv. Photonics Res. 3 , 2100361 (2022)..
Consolino, L. et al. Fully phase-stabilized quantum cascade laser frequency comb. Nat. Commun. 10 , 2938 (2019)..
Guan, W. et al. Relative phase locking of a terahertz laser system configured with a frequency comb and a single-mode laser. Adv. Photonics Nexus 2 , 026006 (2023)..
Oustinov, D. et al. Phase seeding of a terahertz quantum casc ade laser. Nat. Commun. 1 , 69 (2010)..
Barbieri, S. et al. Coherent sampling of active mode-locked terahertz quantum cascade lasers and frequency synthesis. Nat. Photonics 5 , 306–313 (2011)..
Winful, H. G., Chen, Y. C. & Liu, J. M. Frequency locking, quasiperiodicity, and chaos in modulated self-pulsing semiconductor lasers. Appl. Phys. Lett. 48 , 616–618 (1986)..
Freeman, J. R. et al. Injection locking of a terahertz quantum cascade laser to a telecommunications wavelength frequency comb. Optica 4 , 1059–1064 (2017)..
Bak, P. The devil's staircase. Phys. Today 39 , 38–45 (1986)..
Baums, D., Elsässer, W. & Göbel, E. O. Farey tree and devil's staircase of a modulated external-cavity semiconductor laser. Phys. Rev. Lett. 63 , 155–158 (1989)..
Xu, Y. Q. et al. Harmonic and rational harmonic driving of microresonator soliton frequency combs. Optica 7 , 940–946 (2020)..
Wu, X. Q. et al. Farey tree and devil's staircase of frequency-locked breathers in ultrafast lasers. Nat. Commun. 13 , 5784 (2022)..
Riepl, J. et al. Field-resolved high-order sub-cycle nonlinearities in a terahertz semiconductor laser. Light Sci. Appl. 10 , 246 (2021)..
Ecke, R. E., Farmer, J. D. & Umberger, D. K. Scaling of the Arnold tongues. Nonlinearity 2 , 175–196 (1989)..
Sacher, J. et al. Intensity instabilities of semiconductor lasers under current modulation, external light injection, and delayed feedback. Phys. Rev. A 45 , 1893–1905 (1992)..
Li, H. et al. Dynamics of ultra-broadband terahertz quantum cascade lasers for comb operation. Opt. Express 23 , 33270–33294 (2015)..
Li, H. et al. Toward compact and real-time terahertz dual-comb spectroscopy employing a self-detection scheme. ACS Photonics 7 , 49–56 (2020)..
Villares, G. et al. On-chip dual-comb based on quantum cascade laser frequency combs. Appl. Phys. Lett. 107 , 251104 (2015)..
Rösch, M. et al. On-chip, self-detected terahertz dual-comb source. Appl. Phys. Lett. 108 , 171104 (2016)..
Hentschel, H. G. E. & Procaccia, I. The infinite number of generalized dimensions of fractals and strange attractors. Phys. D: Nonlinear Phenom. 8 , 435–444 (1983)..
Jensen, M. H., Bak, P. & Bohr, T. Complete devil's staircase, fractal dimension, and universality of mode- locking structure in the circle map. Phys. Rev. Lett. 50 , 1637–1639 (1983)..
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