3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis

Diana Pereira; Torsten Wieduwilt; Walter Hauswald; Matthias Zeisberger; Marta S. Ferreira; Markus A. Schmidt

doi:10.1038/s41377-025-01827-9

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3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis

Original Articles

- 3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis
- 3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis
- LSA 2025年14卷第7期页码：2019-2029
- Affiliations：
  
  1.Leibniz Institute of Photonic Technology, Jena, Germany
  2.i3N & Physics Department, University of Aveiro, Campus de Santiago, Aveiro, Portugal
  3.Abbe Center of Photonics and Faculty of Physics, Friedrich Schiller University Jena, Jena, Germany
  4.Otto Schott Institute of Materials Research (OSIM), Friedrich Schiller University Jena, Jena, Germany
- Author bio：
  
  Markus A. Schmidt (markus-alexander.schmidt@uni-jena.de)
- Funds：
- DOI：10.1038/s41377-025-01827-9
  中图分类号：
- 收稿日期：2024-08-22，
  
  修回日期：2025-02-18，
  
  录用日期：2025-03-13，
  
  网络出版日期：2025-05-15，
  
  纸质出版日期：2025-07-31
- Accepted：
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3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis[J]. LSA, 2025,14(7):2019-2029.

Pereira, D. et al. 3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis. Light: Science & Applications, 14, 2019-2029 (2025).
3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis[J]. LSA, 2025,14(7):2019-2029. DOI： 10.1038/s41377-025-01827-9.

Pereira, D. et al. 3D nanoprinted fiber-interfaced hollow-core waveguides for high-accuracy nanoparticle tracking analysis. Light: Science & Applications, 14, 2019-2029 (2025). DOI： 10.1038/s41377-025-01827-9.

摘要

Abstract

The integration of functional components into flexible photonic environments is a critical area of research in integrated photonics and is essential for high-precision sensing. This work presents a novel concept of interfacing square-core hollow-core waveguides with commercially available optical fibers using 3D nanoprinting

and demonstrates its practical relevance through a nanoscience-based characterization technique. In detail

this innovative concept results in a monolithic

fully fiber-integrated device with key advantages such as alignment-free operation

high-purity fundamental mode excitation

full polarization control

and a unique handling flexibility. For the first time

the application potential of a fiber-interfaced waveguide in nanoscale analysis is demonstrated by performing nanoparticle-tracking-analysis experiments. These experiments involve the tracking and analysis of individual gold nanospheres diffusing in the hollow core waveguide

enabled by nearly aberration-free imaging

extended observation times

and homogeneous light-line illumination. The study comprehensively covers design strategy

experimental implementation

key principles

optical characterization

and practical applications. The fiber-interfaced hollow-core waveguide concept offers significant potential for applications in bioanalytics

environmental sciences

quantum technologies

optical manipulation

and life sciences. It also paves the way for the development of novel all-fiber devices that exploit enhanced light-matter interaction in a monolithic form suitable for flexible and remote applications.

关键词

Keywords

references

Peng, C. et al. Optical waveguide refractive index sensor for biochemical sensing. Appl. Sci. 13 , 3829 (2023)..

Mu, B. Y. et al. Review on liquid-core waveguide technology and its application for spectroscopic analysis. Microchem. J. 199 , 109935 (2024)..

Fokoua, E. N. et al. Loss in hollow-core optical fibers: mechanisms, scaling rules, and limits. Adv. Opt. Photonics 15 , 1–85 (2023)..

Poletti, F., Petrovich, M. N. & Richardson, D. J. Hollow-core photonic bandgap fibers: technology and applications. Nanophotonics 2 , 315–340 (2013)..

Sakr, H. et al. Hollow core optical fibres with comparable attenuation to silica fibres between 600 and 1100nm. Nat. Commun. 11 , 6030 (2020)..

Russell, P. S. J. et al. Hollow-core photonic crystal fibres for gas-based nonlinear optics. Nat. Photonics 8 , 278–286 (2014)..

Nissen, M. et al. UV Absorption spectroscopy in water-filled antiresonant hollow core fibers for pharmaceutical detection. Sensors 18 , 478 (2018)..

Epple, G. et al. Rydberg atoms in hollow-core photonic crystal fibres. Nat. Commun. 5 , 4132 (2014)..

Yin, D. et al. Integrated ARROW waveguides with hollow cores. Opt. Express 12 , 2710–2715 (2004)..

Yang, W. G. et al. Atomic spectroscopy on a chip. Nat. Photonics 1 , 331–335 (2007)..

Bürger, J. et al. Ultrahigh-aspect-ratio light cages: fabrication limits and tolerances of free-standing 3D nanoprinted waveguides. Opt. Mater. Express 11 , 1046–1057 (2021)..

Davidson-Marquis, F. et al. Coherent interaction of atoms with a beam of light confined in a light cage. Light Sci. Appl. 10 , 137 (2021)..

Jain, C. et al. Hollow core light cage: trapping light behind bars. ACS Photonics 6 , 649–658 (2019)..

Granzow, N. et al. Bandgap guidance in hybrid chalcogenide-silica photonic crystal fibers. Opt. Lett. 36 , 2432–2434 (2011)..

Kim, J. et al. The optofluidic light cage-on-chip integrated spectroscopy using an antiresonance hollow core waveguide. Anal. Chem. 93 , 752–760 (2021)..

Kim, J. et al. Locally structured on-chip optofluidic hollow-core light cages for single nanoparticle tracking. ACS Sens. 7 , 2951–2959 (2022)..

Bürger, J. et al. 3D-nanoprinted antiresonant hollow-core microgap waveguide: an on-chip platform for integrated photonic devices and sensors. ACS Photonics 9 , 3012–3024 (2022)..

Kim, J. et al. 3D-nanoprinted on-chip antiresonant waveguide with hollow core and microgaps for integrated optofluidic spectroscopy. Opt. Express 31 , 2833–2845 (2023)..

Huang, W. Q. et al. Fiber-interfaced hollow-core light cage: a platform for on-fiber-integrated waveguides. Opt. Lett. 49 , 3194–3197 (2024)..

Bertoncini, A. & Liberale, C. 3D printed waveguides based on photonic crystal fiber designs for complex fiber-end photonic devices. Optica 7 , 1487–1494 (2020)..

Michalet, X. & Berglund, A. J. Optimal diffusion coefficient estimation in single-particle tracking. Phys. Rev. E 85 , 061916 (2012)..

Navarro Sanchez, M. E. et al. Rabies vaccine characterization by nanoparticle tracking analysis. Sci. Rep. 10 , 8149 (2020)..

Chan, M. Y. et al. Particle sizing of nanoparticle adjuvant formulations by dynamic light scattering (DLS) and nanoparticle tracking analysis (NTA). Methods Mol. Biol. 1494 , 239–252 (2017)..

Nathan, L&Daniel, S. Single virion tracking microscopy for the study of virus entry processes in live cells and biomimetic platforms. in Physical Virology: Virus Structure and Mechanics (ed Greber, U. F. ) (Cham: Springer, 2019), 13-43.

Gondikas, A. et al. Nanomaterial fate in seawater: a rapid sink or intermittent stabilization? Front. Environ. Sci. 8 , 151 (2020)..

Thanh, N. T. K., Maclean, N. & Mahi ddine, S. Mechanisms of nucleation and growth of nanoparticles in solution. Chem. Rev. 114 , 7610–7630 (2014)..

Förster, R. et al. Tracking and analyzing the brownian motion of nano-objects inside hollow core fibers. ACS Sens. 5 , 879–886 (2020)..

Nissen, M. et al. Nanoparticle tracking in single-antiresonant-element fiber for high-precision size distribution analysis of mono- and polydisperse samples. Small 18 , 2202024 (2022)..

Yin, D. L. et al. Planar optofluidic chip for single particle detection, manipulation, and analysis. Lab Chip 7 , 1171–1175 (2007)..

Zeisberger, M. & Schmidt, M. A. Analytic model for the complex effective index of the leaky modes of tube-type anti-resonant hollow core fibers. Sci. Rep. 7 , 11761 (2017)..

Jang, B. et al. Light guidance in photonic band gap guiding dual-ring light cages implemented by direct laser writing. Opt. Lett. 44 , 4016–4019 (2019)..

Pereira, D. et al. Spatially controlled phase modulation - selective higher-order mode excitation in 3D nanoprint ed on-chip hollow-core waveguides. ACS Photonics 11 , 3178–3186 (2024)..

Kim, J. et al. On-chip fluorescence detection using photonic bandgap guiding optofluidic hollow-core light cage. APL Photonics 7 , 106103 (2022)..

Gui, F. J. et al. Ultralong tracking of fast-diffusing nano-objects inside nanofluidic channel−enhanced microstructured optical fiber. Adv. Photonics Res. 2 , 2100032 (2021)..

Jiang, S. Q. et al. Three-dimensional spatiotemporal tracking of nano-objects diffusing in water-filled optofluidic microstructured fiber. Nanophotonics 9 , 4545–4554 (2020)..

Špačková, B. et al. Label-free nanofluidic scattering microscopy of size and mass of single diffusing molecules and nanoparticles. Nat. Methods 19 , 751–758 (2022)..

Washburn, A. L. & Bailey, R. C. Photonics-on-a-chip: recent advances in integrated waveguides as enabling detection elements for real-world, lab-on-a-chip biosensing applications. Analyst 136 , 227–236 (2011)..

Barreto, D. N. et al. From light pipes to substrate-integra ted hollow waveguides for gas sensing: a review. ACS Meas. Sci. Au 1 , 97–109 (2021)..

Giraud-Carrier, M. et al. Perforated hollow-core optical waveguides for on-chip atomic spectroscopy and gas sensing. Appl. Phys. Lett. 108 , 131105 (2016)..

Rowland, J. et al. High-bandwidth warm-atom quantum memory using hollow-core photonic crystal fibers. Phys. Rev. Appl. 21 , 014048 (2024)..

Measor, P. et al. Hollow-core waveguide characterization by optically induced particle transport. Opt. Lett. 33 , 672–674 (2008)..

Liu, D. J. et al. High sensitivity liquid level sensor for microfluidic applications using a hollow core fiber structure. Sens. Actuators A: Phys. 332 , 113134 (2021)..

Debord, B. et al. Hollow-core fiber technology: the rising of "gas photonics". Fibers 7 , 16 (2019)..

Yao, C. Y. et al. Silica hollow-core negative curvature fibers enable ultrasensitive mid-infrared absorption spectroscopy. J. Light. Technol. 38 , 2067–2072 (2020)..

Ding, H. N. et al. Review on all-fiber online raman sensor with hollow core microstructured optical fiber. Photonics 9 , 134 (2022)..

Cubillas, A. M. et al. Photochemistry in a soft-glass single-ring hollow-core photonic crystal fibre. Analyst 142 , 925–929 (2017)..

Momota, M. R. & Hasan, M. R. Hollow-core silver coated photonic crystal fiber plasmonic sensor. Opt. Mater. 76 , 287–294 (2018)..

Khosravi, M., Qi, X. & Schmidt, M. A. Interfacing high numerical aperture metalenses with thermally expanded core fibers via 3D nanoprinting for advanced meta-fiber operation. Opt. Express 32 , 28206–28214 (2024)..

Ren, H. R. et al. An achromatic metafiber for focusing and imaging across the entire telecommunication range. Nat. Commun. 13 , 4183 (2022)..

Yeh, C.&Shimabukuro, F. I. The Essence of Dielectric Waveguides. (New York: Springer, 2008), https://doi.org/10.1007/978-0-387-49799-0.

Deng, A. et al . Analyzing mode index mismatch and field overlap for light guidance in negative-curvature fibers. Opt. Express 28 , 27974–27988 (2020)..

Lee, H. W. et al. Optofluidic refractive-index sensor in step-index fiber with parallel hollow micro-channel. Opt. Express 19 , 8200–8207 (2011)..

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