Department of Electrical and Electronic Engineering, Southern University of Science and Technology, Shenzhen 518055, China
Shuming Chen (chen.sm@sustech.edu.cn)
收稿日期:2024-10-28,
修回日期:2025-03-11,
录用日期:2025-03-17,
网络出版日期:2025-04-25,
纸质出版日期:2025-06-30
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Face-to-face integrated tandem quantum-dot LEDs with high performance and multifunctionality[J]. LSA, 2025,14(6):1739-1748.
Li, H. T., Wang, J. M. & Chen, S. M. Face-to-face integrated tandem quantum-dot LEDs with high performance and multifunctionality. Light: Science & Applications, 14, 1739-1748 (2025).
Face-to-face integrated tandem quantum-dot LEDs with high performance and multifunctionality[J]. LSA, 2025,14(6):1739-1748. DOI: 10.1038/s41377-025-01835-9.
Li, H. T., Wang, J. M. & Chen, S. M. Face-to-face integrated tandem quantum-dot LEDs with high performance and multifunctionality. Light: Science & Applications, 14, 1739-1748 (2025). DOI: 10.1038/s41377-025-01835-9.
The realization of solution-processed tandem quantum-dot LEDs (QLEDs) remains a technical challenge due to the limitations of inefficient interconnect layer and the damage caused by multiple solution processes. Here
we develop a high performance tandem QLED by face-to-face integrating a top-emitting QLED with a transp
arent QLED. The top and bottom units can be addressed independently
thereby enabling the tandem QLED to operate in series
parallel
and color-tunable modes for multifunctionality. In series mode
QLEDs demonstrate an ultra-low turn-on voltage of 3.3 V and a record-breaking external quantum efficiency of 60.7%. In parallel mode
QLEDs achieve an impressive brightness of over 4.8 × 10
6
cd m
-2
. In color-tunable mode
the color
brightness
and color temperature can all be adjusted with a color tuning range of 114% NSTC. Moreover
both series and parallel connections contribute to an improved stability
resulting in a T
95
lifetime of nearly 30
000 h at 1000 cd m
-2
which is an improvement of approximately 2.8 times over control devices. Our work offers a feasible solution for achieving multifunctional tandem QLEDs with the advantages of solution processed
high efficiency
high brightness
long lifetime and full color tunability for various light source applications.
Dai, X. et al. Solution-processed, high-performance light-emitting diodes based on quantum dots. Nature 515 , 96–99 (2014)..
Mashford, B. S. et al. High-efficiency quantum-dot light-emitting devices with enhanced charge injection. Nat. Photonics 7 , 407–412 (2013)..
Zhang, H., Su, Q. & Chen, S. Quantum-dot and organic hybrid tandem light-emitting diodes with multi-functionality of full-color-tunability and white-light-emission. Nat. Commun. 11 , 2826 (2020)..
Dai, X., Deng, Y., Peng, X. & Jin, Y. Quantum-dot light-emitting diodes for large-area displays: towardsthe dawn of commercialization. Adv. Mater. 29 , 1607022 (2017)..
Shen, H. et al. Visible quantum dot light-emitting diodes with simultaneous high brightness and efficiency. Nat. Photonics 13 , 192–197 (2019)..
Chen, Z. et al. Color revolution: prospects and challenges of quantum-dot light-emitting diode display technologies. Small Methods 8 , 2300359 (2024)..
Song, J. et al. Over 30% external quantum efficiency light-emitting diodes by engineering quantum dot-assisted energy level match for hole transport layer. Adv. Funct. Mater. 29 , 1808377 (2019)..
Xu, H. et al. Dipole-dipole-interaction-assisted self-assembly of quantum dots for highly efficient light-emitting diodes. Nat. Photonics 515 , 96 (2024)..
Li, H., Tian, F. & Chen, S. Approaching the theoretical efficiency limit of quantum-dot light-emitting diodes via synergistic optimization. Nano Res. 16 , 10156–10163 (2023)..
Li, H., Zhou, S. & Chen, S. Highly efficient top-emitting quantum-dot light-emitting diodes with record-breaking external quantum efficiency of over 44.5. Laser Photonics Rev 17 , 407 (2023)..
Zhang, H., Chen, S. & Sun, X. W. Efficient red/green/blue tandem quantum-dot light-emitting diodes with external quantum efficiency exceeding 21. ACS Nano 12 , 697–704 (2018)..
Wu, Q. et al. Efficient tandem quantum-dot LEDs enabled by an inorganic semiconductor-metal-dielectric interconnecting layer stack. Adv. Mater. 34 , 2108150 (2022)..
Yuan, C., Chen, Z., Tian, F. & Chen, S. Very stable and efficient tandem quantum-dot light-emitting diodes enabled by IZO-base d interconnecting layers. Nano Lett. 24 , 7541–7547 (2024)..
Zhou, T. et al. High-performance tandem quantum-dot light-emitting diodes based on bulk-heterojunction-like charge-generation layers. Adv. Mater. 36 , 2313888 (2024)..
Jiang, C. et al. Fully solution-processed tandem white quantum-dot light-emitting diode with an external quantum efficiency exceeding 25. ACS Nano 12 , 6040–6049 (2018)..
Zhang, H., Sun, X. & Chen, S. Over 100 cd A −1 efficient quantum dot light-emitting diodes with inverted tandem structure. Adv. Funct. Mater. 27 , 1700610 (2017)..
Zhang, H., Wang, S., Sun, X. & Chen, S. All solution-processed white quantum-dot light-emitting diodes with three-unit tandem structure. J. Soc. Inf. Disp. 25 , 143–150 (2017)..
Jang, E. & Jang, H. Review: quantum dot light-emitting diodes. Chem. Rev. 123 , 4663–4692 (2023)..
Chen, Z., Qin, Z., Su, S. & Chen, S. The influence of H 2 O and O 2 on the optoelectronic properties of inverted quantum-dot lig ht-emitting diodes. Nano Res. 14 , 4140–4145 (2021)..
Ding, S. et al. Impact of the resistive switching effects in ZnMgO electron transport layer on the aging characteristics of quantum dot light-emitting diodes. Appl. Phys. Lett. 117 , 96 (2020)..
Yoshida, K. et al. Electrically driven organic laser using integrated OLED pumping. Nature 621 , 746–752 (2023)..
Kwon, T. H. et al. Quantum dot-based three-stack tandem near-infrared-to-visible optoelectric upconversion devices. ACS Nano 18 , 21957–21965 (2024)..
Jeon, Y. et al. Parallel-stacked flexible organic light-emitting diodes for wearable photodynamic therapeutics and color-tunable optoelectronics. ACS Nano 14 , 15688–15699 (2020)..
Chen, H. et al. Quantum dot light emitting devices for photomedical applications. J. Soc. Inf. Disp. 25 , 177–184 (2017)..
Yuan, C., Tian, F. & Chen, S. ZnSeTe blue top-emitting QLEDs with color saturation near Rec. 2020 standards and efficiency over 18.16. Nano Res. 16 , 5517–55 24 (2023)..
Furno, M., Meerheim, R., Hofmann, S., Lüssem, B. & Leo, K. Efficiency and rate of spontaneous emission in organic electroluminescent devices. Phys. Rev. B 85 , 115205 (2012)..
Choi, S. et al. Thin-film transistor-driven vertically stacked full-color organic light-emitting diodes for high-resolution active-matrix displays. Nat. Commun. 11 , 2732 (2020)..
Su, Q., Zhang, H., Xia, F., Sun, X. W. & Chen, S. 73-4: tandem red quantum-dot light-emitting diodes with external quantum efficiency over 34. SID Symp. Dig. Tech. Pap. 49 , 977–980 (2018)..
Gao, Y. et al. Minimizing heat generation in quantum dot light-emitting diodes by increasing quasi-Fermi-level splitting. Nat. Nanotechnol. 18 , 1168–1174 (2023)..
Bae, W. K. et al. Controlling the influence of Auger recombination on the performance of quantum-dot light-emitting diodes. Nat. Commun. 4 , 2661 (2013)..
Moon, H., Lee, C., Lee, W., Kim, J. & Chae, H. Stability of quantum dots, quantum dot films, and quantum dot light-emitting diodes for display appl ications. Adv. Mater. 31 , 1804294 (2019)..
Sun, Y. et al. Investigation on thermally induced efficiency roll-off: toward efficient and ultrabright quantum-dot light-emitting diodes. ACS Nano 13 , 11433–11442 (2019)..
Lee, T. et al. Bright and stable quantum dot light-emitting diodes. Adv. Mater. 34 , 2106276 (2022)..
Zhu, X., Wang, Y. & Ji, W. Unraveling the turn-on limitation of quantum-dot electroluminescence via a stepwise-increasing voltage measurement. Phys. Rev. Appl. 19 , 024010 (2023)..
Fang, Y. et al. Highly efficient red quantum dot light-emitting diodes by balancing charge injection and transport. ACS Appl. Mater. Interfaces 14 , 21263–21269 (2022)..
Rhee, S. et al. Tailoring the electronic landscape of quantum dot light-emitting diodes for high brightness and stable operation. ACS Nano 14 , 17496–17504 (2020)..
Lim, J., Park, Y.-S., Wu, K., Yun, H. J. & Klimov, V. I. Droop-free colloidal quantum dot light-emitting diodes. Nano Lett 18 , 6645–6653 (2018)..
Lee, K.-H. et al. Highly efficient, color-reproducible full-color electroluminescent devices based on red/green/blue quantum dot-mixed multilayer. ACS Nano 9 , 10941–10949 (2015)..
Hames, B. C., Mora-Seró, I. & Sánchez, R. S. Device performance and light characteristics stability of quantum-dot-based white-light-emitting diodes. Nano Res. 11 , 1575–1588 (2018)..
Anikeeva, P. O., Halpert, J. E., Bawendi, M. G. & Bulović, V. Electroluminescence from a mixed red-green-blue colloidal quantum dot monolayer. Nano Lett. 7 , 2196–2200 (2007)..
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