Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities

Emmanouil G. Mavrotsoupakis; Leonidas Mouchliadis; Junhui Cao; Minoas C. Chairetis; Marios E. Triantafyllou-Rundell; Eleni C. P. Macropulos; Giannis G. Paschos; Apostolos Pantousas; Huaying Liu; Alexey V. Kavokin; Hamid Ohadi; Constantinos C. Stoumpos; Pavlos G. Savvidis

doi:10.1038/s41377-025-01852-8

Your Location：

Home >

Browse articles >

Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities

Original Articles

- Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities
- Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities
- LSA 2025年14卷第8期页码：2163-2172
- Affiliations：
  
  1.Institute of Electronic Structure and Laser, Foundation for Research and Technology-Hellas, Heraklion 71110 Crete, Greece
  2.Department of Materials Science and Engineering, University of Crete, Heraklion, Crete 70013, Greece
  3.Key Laboratory for Quantum Materials of Zhejiang Province, Department of Physics, Westlake University, Hangzhou, People's Republic of China
  4.Westlake University, 600 Dunyu Rd, Xihu District, Hangzhou, Zhejiang 310030, People's Republic of China
  5.Center for Quantum Science & Technologies, FORTH-QuTech, Crete 70013 Heraklion, Greece
  6.Abrikosov Center for Theoretical Physics, MIPT, Dolgoprudny, Moscow Region 141701, Russia
  7.Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology, School of Physics Science and Engineering, Tongji University, Shanghai 200092, China
  8.SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, UK
  9.Photonics of Crystals Laboratory, Saint Petersburg State University, Ulyanovskaya d.1, St. Petersburg 198504, Russia
- Author bio：
  
  Pavlos G. Savvidis (p.savvidis@westlake.edu.cn)
- Funds：
- DOI：10.1038/s41377-025-01852-8
  中图分类号：
- 收稿日期：2024-11-06，
  
  修回日期：2025-03-13，
  
  录用日期：2025-03-26，
  
  网络出版日期：2025-05-29，
  
  纸质出版日期：2025-08-31
- Accepted：
Scan QR Code
Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities[J]. LSA, 2025,14(8):2163-2172.

Mavrotsoupakis, E. G. et al. Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities. Light: Science & Applications, 14, 2163-2172 (2025).
Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities[J]. LSA, 2025,14(8):2163-2172. DOI： 10.1038/s41377-025-01852-8.

Mavrotsoupakis, E. G. et al. Unveiling asymmetric topological photonic states in anisotropic 2D perovskite microcavities. Light: Science & Applications, 14, 2163-2172 (2025). DOI： 10.1038/s41377-025-01852-8.

摘要

Abstract

Photonic Rashba-Dresselhaus coupling in anisotropic microcavities offers a compelling platform for realizing unconventional topological states with non-zero Berry curvature. In this study

we explore a self-assembled two-dimensional hybrid structure composed of anisotropically oriented organic/inorganic halide perovskite layers confined within a microcavity. The strong optical anisotropies of these perovskite systems

driven by significant refractive index contrasts and robust excitonic resonances at room temperature

enable the emergence of synthetic magnetic fields that mediate photonic and polaritonic interactions. The interplay between polarization-dependent modes and spatial inversion symmetry breaking gives rise to strong photonic Rashba-Dresselhaus spin-orbit coupling

leading to distinct modifications in band topology and energy dispersions. These effects result in the formation of unconventional topological features

including non-zero Berry curvature and off-axis diabolical points

within the photonic and polaritonic bands at room temperature. Our findings reveal the critical role of optical and geometric anisotropies in engineering synthetic gauge fields for light

providing a versatile approach for designing photonic systems with novel topological properties. By leveraging the unique properties of halide perovskites and their ability to support both room-temperature excitons and large birefringence

this work advances the development of polaritonic platforms for applications in topological photonics and spinoptronics.

关键词

Keywords

references

Aidelsburger, M., Nascimbene, S. & Goldman, N. Artificial gauge fields in materials and engineered systems. Comptes Rendus Phys. 19 , 394–432 (2018)..

Rashba, E. I. & Sheka, V. I. Symmetry of energy bands in crystals of wurtzite type II. Symmetry of bands with spin-orbit interaction included. N. J. Phys. 17 , 62–76 (2015)..

Dresselhaus, G. Spin-orbit coupling effects in zinc blende structures. Phys. Rev. 100 , 580–586 (1955)..

Hasan, M. Z. & Kane, C. L. Colloquium: topological insulators. Rev. Mod. Phys. 82 , 3045–3067 (2010)..

Manchon, A., Koo, H. C., Nitta, J., Frolov, S. M. & Duine, R. A. New perspectives for Rashba spin-orbit coupling. Nat. Mater. 14 , 871–882 (2015)..

Dyakonov, M. I. & Perel, V. I. Current-induced spin orientation of electrons in semiconductors. Phys. Lett. A 35 , 459–460 (1971)..

Sinova, J., Valenzuela, S. O., Wunderlich, J., Back, C. H. & Jungwirth, T. Spin Hall effects. Rev. Mod. Phys. 87 , 1213–1260 (2015)..

Kane, C. L. & Mele, E. J. Quantum spin Hall effect in graphene. Phys. Rev. Lett. 95 , 226801 (2005)..

Bernevig, B. A., Hughes, T. L. & Zhang, S.-C. Quantum spin Hall effect and topological phase transition inHgTe quantum wells. Science 314 , 1757–1761 (2006)..

König, M. et al. Quantum spin Hall insulator state in HgTe quantum wells. Science 318 , 766–7 70 (2007)..

Berry, M. V. Quantal phase factors accompanying adiabatic changes. Proc. R. Soc. Lond. Ser. A 392 , 45–57 (1984)..

Simon, B. Holonomy, the quantumadiabatic theorem, and Berry's phase. Phys. Rev. Lett. 51 , 2167–2170 (1983)..

Lu, L. & Joannopoulos, J. D. & Soljačić, M. Topological photonics. Nat. Photonics 8 , 821–829 (2014)..

Onoda, M., Murakami, S. & Nagaosa, N. Hall effect of light. Phys. Rev. Lett. 93 , 083901 (2004)..

Bliokh, K. Y., Smirnova, D. & Nori, F. Quantum spin Hall effect of light. Science 348 , 1448–1451 (2015)..

Khanikaev, A. B. & Shvets, G. Two-dimensional topological photonics. Nat. Photonics 11 , 763–773 (2017)..

Hey, D. & Li, E. Advances in synthetic gauge fields for light through dynamic modulation. R. Soc. Open Sci. 5 , 172447 (2018)..

Ozawa, T. et al. Topological photonics. Rev. Mod. Phys. 91 , 015006 (2019)..

Segev, M. & Bandres, M. A. Topological photonics: where do we go from here? Nanophotonics 10 , 425–434 (2021)..

Liew, T. C. H., Shelykh, I. A. & Malpuech, G. Polaritonic devices. Phys. E: Low.-Dimens. Syst. Nanostruct. 43 , 1543–1568 (2011)..

Sanvitto, D. & Kéna-Cohen, S. The road towards polaritonic devices. Nat. Mater. 15 , 1061–1073 (2016)..

Kavokin, A. V., Baumberg, J. J., Malpuech, G. & Laussy, F. P. Microcavities (Oxford University Press, 2017).

Kavokin, A., Malpuech, G. & Glazov, M. Optical spin Hall effect. Phys. Rev. Lett. 95 , 136601 (2005)..

Leyder, C. et al. Observation of the optical spin Hall effect. Nat. Phys. 3 , 628–631 (2007)..

Lim, H. T., Togan, E., Kroner, M., Miguel-Sanchez, J. & Imamoğlu, A. Electrically tunable artificial gauge potential for polaritons. Nat. Commun. 8 , 14540 (2017)..

Gianfrate, A. et al. Measurement of the quantum geometric tensor and of the anomalous Hall drift. Nature 578 , 381–385 (2020)..

St-Jean, P. et al. Lasing in topological edge states of a one-dimensional lattice. Nat. Photonics 11 , 651–656 (2017)..

Whittaker, C. E. et al. Optical analogue of Dresselhaus spin–orbit interaction in photonic graphene. Nat. Photonics 15 , 193–196 (2021)..

Klembt, S. et al. Exciton-polariton topological insulator. Nature 562 , 552–556 (2018)..

Lekenta, K. et al. Tunable optical spin Hall effect in a liquid crystal microcavity. Light Sci. Appl. 7 , 74 (2018)..

Rechcińska, K. et al. Engineering spin-orbit synthetic Hamiltonians in liquid-crystal optical cavities. Science 366 , 727–730 (2019)..

Muszyński, M. et al. Realizing persistent-spin-Helix lasing in the regime of Rashba-Dresselhaus spin-orbit coupling in a dye-filled liquid-crystal optical microcavity. Phys. Rev. Appl. 17 , 014041 (2022)..

Ren, J. et al. Realization of exciton-mediated optical spin-orbit interaction in organic microcrystalline resonators. Laser Photonics Rev. 16 , 2100090 (2022)..

Kędziora, M. et al. Predesigned perovskite crystal waveguides for room-temperature exciton-polariton condensation and edge lasing. Nat. Mater. 23 , 1515–1522 (2024)..

Tao, R. et al. Halide perovskites enable polaritonic XY spin Hamiltonian at room temperature. Nat. Mater. 21 , 761–766 (2022)..

Peng, K., Li, W., Berloff, N. G., Zhang, X. & Bao, W. Room temperature polaritonic soft-spin XY Hamiltonian in organic–inorganic halide perovskites. Nanophotonics 13 , 2651–2658 (2024)..

Peng, K. et al. Topological valley Hall polariton condensation. Nat. Nanotechnol. 19 , 1283–1289 (2024)..

Łempicka-Mirek, K. et al. Electrically tunable Berry curvature and strong light-matter coupling in liquid crystal microcavities with 2D perovskite. Sci. Adv. 8 , eabq9952 (2022)..

Polimeno, L. et al. Experimental investigation of a non-Abelian gauge field in 2D perovskite photonic platform. Optica 8 , 1442–1447 (2021)..

Polimeno, L. et al. Tuning of the Berry curvature in 2D perovskite polaritons. Nat. Nanotechnol. 16 , 1435 (2021)..

Spencer, M. S. et al. Spin-orbit–coupled exciton-polariton condensates in lead halide perovskites. Sci. Adv. 7 , eabe9950 (2021)..

Li, Y. et al. Manipulating polariton condensates by Rashba-Dresselhaus coupling at room temperature. Nat. Commun. 13 , 3785 (2022)..

Moriyama, Y. et al. Polarization superposition of room-temperature polariton condensation. Commun. Mater. 4 , 110 (2023)..

Liang, J. et al. Polariton spin Hall effect in a Rashba–Dresselhaus regime at room temperature. Nat. Photonics 18 , 357–362 (2024)..

Sedov, E. S., Glazov, M. M., Lagoudakis, P. G. & Kavokin, A. V. Light-matter coupling and spin-orbit interaction of polariton modes in liquid crystal optical microcavities. Phys. Rev. Res. 6 , 023220 (2024)..

Stoumpos, C. C. et al. Ruddlesden–Popper hybrid lead iodide perovskite 2D homologous semiconductors. Chem. Mater. 28 , 2852–2867 (2016)..

Blancon, J. C., Even, J., Stoumpos, C. C., Kanatzidis, M. G. & Mohite, A. D. Semiconductor physics of organic–inorganic 2D halide perovskites. Nat. Nanotechnol. 15 , 969–985 (2020)..

Mitzi, D. B., Chondroudis, K. & Kagan, C. R. Organic-inorganic electronics. IBM J. Res. Dev. 45 , 29–45 (2001)..

Mao, L., Stoumpos, C. C. & Kanatzidis, M. G. Two-dimensional hybrid halide perovskites principles and promises. J. Am. Chem. Soc. 141 , 1171–1190 (2019)..

Fu, Y. et al. Metal halide perovskite nanostructures for optoelectronic applications and the study of physical properties. Nat. Rev. Mater. 4 , 169–188 (2019)..

Soe, C. M. M. et al. Structural and thermodynamic limits of layer thickness in 2D halide perovskites. Proc. Natl Acad. Sci. USA 116 , 58–66 (2019)..

Guo, P. et al. Hyperbolic dispersion arising from anisotropic excitons in two-dimensional perovskites. Phys. Rev. Lett. 121 , 127401 (2018)..

Karzig, T., Bardyn, C.-E., Lindner, N. H. & Refael, G. Topological polaritons. Phys. Rev. X 5 , 031001 (2015)..

Blancon, J.-C. et al. Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites. Science 355 , 1288–1292 (2017)..

Säynätjoki, A. et al. Ultra-strong nonlinear optical processes and trigonal warping in MoS 2 layers. Nat. Commun. 8 , 893 (2017)..

Bladwell, S. S. R. Valley separation via trigonal warping. Phys. Rev. B 101 , 045404 (2020)..

Kavokin, A. et al. Polariton condensates for classical and quantum computing. Nat. Rev. Phys. 4 , 435–451 (2022)..

Fang, K., Yu, Z. & Fan, S. Realizing effective magnetic field for photons by controlling the phase of dynamic modulation. Nat. Photonics 6 , 782–787 (2012)..

Bahari, B. et al. Nonreciprocal lasing in topological cavities of arbitrary geometries. Science 358 , 636–640 (2017)..

浏览量

Downloads

CSCD

文章被引用时，请邮件提醒。

Submit

工具集

关联资源

暂无数据