High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance

Yeonjeong Koo; Dong Kyo Oh; Jungho Mun; Artem N. Abramov; Mikhail Tyugaev; Yong Bin Kim; Inki Kim; Tae Ho Kim; Sera Yang; Yeseul Kim; Jonghwan Kim; Vasily Kravtsov; Junsuk Rho; Kyoung-Duck Park

doi:10.1038/s41377-025-01873-3

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High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance

Original Articles

- High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance
- High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance
- LSA 2025年14卷第8期页码：2263-2271
- Affiliations：
  
  1.Department of Physics, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
  2.Department of Mechanical Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
  3.Department of Electrical and Computer Engineering, Purdue University, West Lafayette, IN 47907, USA
  4.School of Physics and Engineering, ITMO University, Saint Petersburg 197101, Russia
  5.Department of Biophysics, Institute of Quantum Biophysics, Sungkyunkwan University, Seoul 16419, Republic of Korea
  6.Department of Intelligent Precision Healthcare Convergence, Sungkyunkwan University, Seoul 16419, Republic of Korea
  7.Department of Material Science and Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
  8.Center for Van der Waals Quantum Solids, Institute for Basic Science (IBS), Daejeon 37673, Republic of Korea
  9.Institute for Convergence Research and Education in Advanced Technology, Yonsei University, Seoul 03722, Republic of Korea
  10.Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
  11.Department of Electrical Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
  12.POSCO-POSTECH-RIST Convergence Research Center for Flat Optics and Metaphotonics, Pohang 37673, Republic of Korea
  13.National Institute of Nanomaterials Technology (NINT), Pohang 37673, Republic of Korea
  14.Department of Semiconductor Engineering, Pohang University of Science and Technology (POSTECH), Pohang 37673, Republic of Korea
- Author bio：
  
  Vasily Kravtsov (vasily.kravtsov@metalab.ifmo.ru)
  Junsuk Rho (jsrho@postech.ac.kr)
  Kyoung-Duck Park (parklab@postech.ac.kr)
- Funds：
- DOI：10.1038/s41377-025-01873-3
  中图分类号：
- 收稿日期：2024-12-18，
  
  修回日期：2025-03-30，
  
  录用日期：2025-04-22，
  
  网络出版日期：2025-06-20，
  
  纸质出版日期：2025-08-31
- Accepted：
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High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance[J]. LSA, 2025,14(8):2263-2271.

Koo, Y. et al. High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance. Light: Science & Applications, 14, 2263-2271 (2025).
High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance[J]. LSA, 2025,14(8):2263-2271. DOI： 10.1038/s41377-025-01873-3.

Koo, Y. et al. High momentum two-dimensional propagation of emitted photoluminescence coupled with surface lattice resonance. Light: Science & Applications, 14, 2263-2271 (2025). DOI： 10.1038/s41377-025-01873-3.

摘要

Abstract

Dramatic fluorescence enhancement in two-dimensional (2D) van der Waals materials (vdWMs) coupled to plasmonic nanostructures has the potential to enable ultrathin

flexible

and high-brightness illumination devices. However

addressing the limitation of locally scattered small plasmon-enhanced areas remains challenging. Here

we present a 2D plasmonic enhancement of photoluminescence (PL) spanning nearly 800 μm

enabled by surface lattice resonance (SLR) in a 2D vdWM-Au slot lattice hybrid. The Au slot lattice is designed and fabricated using Babinet's principle and Rayleigh's anomaly to maximize radiative decay rate and induce non-local photo-excitation in a MoSe

monolayer. For emitted PL coupled with SLR

enhanced by up

to 32-fold

we investigate its in-plane directivity and long-range propagation using angle- and space-resolved spectroscopic PL measurements. Our experiment reveals that a nearly 800 μm

2D luminescent sheet can be achieved regardless of the size of the MoSe

crystal

even with a sub-μm

flake. This work provides a new type of ultrabright

large-area 2D luminescent material

suitable for a range of optical illumination

communication

and sensing devices.

关键词

Keywords

references

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