1.State Key Laboratory of Luminescent Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangzhou, China
2.School of Optoelectronic Engineering, Guangdong Polytechnic Normal University, Guangzhou, China
3.School of Physics and Optoelectronics, South China University of Technology, Guangzhou, China
4.School of Materials Science and Engineering, Zhejiang University, Hangzhou, China
5.State Key Laboratory of Modern Optical Instrumentation, College of Optical Science and Engineering, Zhejiang University, Hangzhou, China
Guoping Dong (dgp@scut.edu.cn)
收稿:2025-10-21,
修回:2025-11-30,
录用:2025-12-07,
网络首发:2026-01-26,
纸质出版:2026-03-31
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Shengda Ye, Jianhao Chen, Jiayue He, 等. A monolithic microcavity laser with simultaneous upconversion and frequency-doubled lasing via crystal-in-glass engineering[J]. Light: Science & Applications, 2026,15(3):973-983.
Ye, S. D. et al. A monolithic microcavity laser with simultaneous upconversion and frequency-doubled lasing via crystal-in-glass engineering. Light: Science & Applications, 15, 973-983 (2026).
Shengda Ye, Jianhao Chen, Jiayue He, 等. A monolithic microcavity laser with simultaneous upconversion and frequency-doubled lasing via crystal-in-glass engineering[J]. Light: Science & Applications, 2026,15(3):973-983. DOI: 10.1038/s41377-025-02162-9.
Ye, S. D. et al. A monolithic microcavity laser with simultaneous upconversion and frequency-doubled lasing via crystal-in-glass engineering. Light: Science & Applications, 15, 973-983 (2026). DOI: 10.1038/s41377-025-02162-9.
This work demonstrates a novel crystal-in-glass composite structure for multifunctional micro-nano light sources in integrated photonics. Based on a Er
3+
/Yb
3+
-codoped glass-ceramic (GC) whispering gallery mode (WGM) microcavity incorporating Ba
2
TiGe
2
O
8
(BTG) crystals
this microcavity enables dual-mode responses combining upconversion (UC) and frequency-doubled lasing. Made from a low-phonon-energy germanate glass matrix codoped with Er
3+
/Yb
3+
for UC gain
the microcavity is crystallized to form BTG microcrystals for second harmonic generation (SHG). By leveraging the high-quality factor (Q ≈ 5.7 × 10
4
) and small mode volume
we achieve green (550 nm) and red (660 nm) UC lasing in a 30-μm-diameter microcavity with low thresholds of 13.31 μW and 12.97 μW
respectively. Benefitted from the random quasi-phase-matching (RQPM) mechanism in BTG GC
the microcavity also demonstrates an ultrabroadband frequency-doubling response from 900 to 1200 nm. By combining tapered fiber near-field coupling and femtosecond free-space pumping
we achieve simultaneous output of green/red UC lasing and frequency-doubled lasing within a single microcavity. We believe this work offers insights into hybrid material design and cooperative optical field manipulation for tunable lasers and on-chip nonlinear photonic systems.
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