Dispersion engineering by rotational symmetry breaking in an optical microcavity

Jian-Zheng Ren; Li-Jie Li; Rui-Qi Zhang; Zhi-Yan Wang; Qi-Tao Cao; Yun-Feng Xiao

doi:10.1038/s41377-025-02169-2

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Dispersion engineering by rotational symmetry breaking in an optical microcavity

Original Articles

- Dispersion engineering by rotational symmetry breaking in an optical microcavity
- Dispersion engineering by rotational symmetry breaking in an optical microcavity
- Light: Science & Applications 2026年15卷第3期页码：895-902
- Affiliations：
  
  1.State Key Laboratory for Mesoscopic Physics, Frontiers Science Center for Nano-optoelectronics, New Cornerstone Science Labotatory, School of Physics, Peking University, Beijing 100871, China
  2.Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China
- Author bio：
  
  Qi-Tao Cao (caoqt@pku.edu.cn)
  Yun-Feng Xiao (yfxiao@pku.edu.cn)
- Funds：
- DOI：10.1038/s41377-025-02169-2
  中图分类号：
- 收稿：2025-12-03，
  
  录用：2025-12-13，
  
  网络首发：2026-01-22，
  
  纸质出版：2026-03-31
- Accepted：
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Jian-Zheng Ren, Li-Jie Li, Rui-Qi Zhang, 等. Dispersion engineering by rotational symmetry breaking in an optical microcavity[J]. Light: Science & Applications, 2026,15(3):895-902.

Ren, J. Z. et al. Dispersion engineering by rotational symmetry breaking in an optical microcavity. Light: Science & Applications, 15, 895-902 (2026).
Jian-Zheng Ren, Li-Jie Li, Rui-Qi Zhang, 等. Dispersion engineering by rotational symmetry breaking in an optical microcavity[J]. Light: Science & Applications, 2026,15(3):895-902. DOI： 10.1038/s41377-025-02169-2.

Ren, J. Z. et al. Dispersion engineering by rotational symmetry breaking in an optical microcavity. Light: Science & Applications, 15, 895-902 (2026). DOI： 10.1038/s41377-025-02169-2.

摘要

Abstract

Dispersion engineering is pivotal for nonlinear optics

yet it often faces challenges posed by material and structural limitations. Here

we establish rotational symmetry breaking as the guiding principle for dispersion engineering in optical microcavities. Through boundary deformation

multi-branch global dispersion emerges in island modes

and local dispersion is controlled via resonance-assisted tunneling between quasi-whispering gallery modes. Enabled by the global dispersion

the optical parametric oscillation is predicted in blue-violet light spectrum with high efficiency (> 55%) and large frequency separation (> 180 THz). Using the local dispersion engineering

the doubly-resonant enhancement of second-harmonic generation is regulated by the resonance-assisted tunneling.

关键词

Keywords

references

Strickland,D. & Mourou, G. Compression of amplified chirped optical pulses. Opt. Commun. 55 , 447 (1985)..

Reeves, W. et al. Transformation and control of ultra-short pulses in dispersion-engineered photonic crystal fibres. Nature 424 , 511 (2003)..

Ouyang, Y.-H., Luan, H.-Y., Zhao, Z.-W., Mao, W.-Z. & Ma, R.-M. Singular dielectric nanolaser with atomic-scale field localization. Nature 632 , 287 (2024)..

Wang, S. et al. A broadband achromatic metalens in the visible. Nat. Nanotechnol. 13 , 227 (2018)..

Song, W. et al. Dispersionless coupling among optical waveguides by artificial gauge field. Phys. Rev. Lett. 129 , 053901 (2022)..

Huang, C. et al. A conformal mapping approach to broadband nonlinear optics on chip. Nat. Photonics 18 , 471–477 (2024)..

Wu, T.-H. et al. Visible-to-ultraviolet frequency comb generation in lithium niobate nanophotonic waveguides. Nat. Photonics 18 , 218 (2024)..

Giordmaine, J. A. & Miller, R. C. Tunable coherent parametric oscillation in LiNbO 3 at optical frequencies, . Phys. Rev. Lett. 14 , 973 (1965)..

Stone, J. R. et al. Wavelength-accurate nonlinear conversion through wavenumber selectivity in photonic crystal resonators. Nat. Photonics 18 , 192 (2024)..

Kwiat, P. G. et al. New high-intensity source of polarization-entangled photon pairs. Phys. Rev. Lett. 75 , 4337 (1995)..

Mittal, S., Goldschmidt, E. A. & Hafezi, M. A topological source of quantum light. Nature 561 , 502 (2018)..

Wang, Z. et al. Large-scale cluster quantum microcombs. Light Sci. Appl. 14 , 164 (2025)..

Fejer, M. M., Magel, G., Jundt, D. H. & Byer, R. L. Quasi-phase-matched second harmonic generation: tuning and tolerances. IEEE J. Quantum Electron. 28 , 2631 (1992)..

Markos, C., Travers, J. C., Abdolvand, A., Eggleton, B. J. & Bang, O. Hybrid photonic-crystal fiber. Rev. Mod. Phys. 89 , 045003 (2017)..

Dudley, J. M., Genty, G. & Coen, S. Supercontinuum generation in photonic crystal fiber. Rev. Mod. Phys. 78 , 1135 (2006)..

Vahala, K. J. Optical microcavities. Nature 424 , 839 (2003)..

Cao, H. & Wiersig, J. Dielectric microcavities: Model systems for wave chaos and non-Hermitian physics. Rev. Mod. Phys. 87 , 61 (2015)..

Xiao, Y.-F., Zou, C.-L., Gong, Q. & Yang, L. Ultra-High-Q Optical Microcavities (World Scientific, 2020).

Zhang, X. et al. Symmetry-breaking-induced nonlinear optics at a microcavity surface. Nat. Photonics 13 , 21 (2019)..

Lu, J., Li, M., Zou, C.-L., Al Sayem, A. & Tang, H. X. Toward 1% single-photon anharmonicity with periodically poled lithium niobate microring resonators. Optica 7 , 1654 (2020)..

Clementi, M. et al. A chip-scale second-harmonic source via self-injection-locked all-optical poling. Light Sci. Appl. 12 , 296 (2023)..

Breunig, I. Three-wave mixing in whispering gallery resonators. Laser Photonics Rev. 10 , 569 (2016)..

Lu, X., Moille, G., Rao, A., Westly, D. A. & Srinivasan, K. On-chip optical parametric oscillation into the visible: generating red, orange, yellow, and green from a near-infrared pump. Optica 7 , 1417 (2020)..

Sayson, N. L. B. et al. Octave-spanning tunable parametric oscillation in crystalline Kerr microresonators. Nat. Photonics 13 , 701 (2019)..

Sun, Y. et al. Advancing on-chip Kerr optical parametric oscillation towards coherent applications covering the green gap. Light Sci. Appl. 13 , 201 (2024)..

Lai, Y.-H., Lu, Y.-K., Suh, M.-G., Yuan, Z. & Vahala, K. Observation of the exceptional-point-enhanced Sagnac effect. Nature 576 , 65 (2019)..

Wang, M. et al. Taming brillouin optomechanics using supermode microresonators. Phys. Rev. X 14 , 011056 (2024)..

Wang, C. et al. High-Q microresonators on 4H-silicon-carbide-on-insulator platform for nonlinear photonics. Light Sci. Appl. 10 , 139 (2021)..

Herr, T. et al. Universal formation dynamics and noise of Kerr-frequency combs in microresonators. Nat. Photonics 6 , 480 (2012)..

Kippenberg, T. J., Gaeta, A. L., Lipson, M. & Gorodetsky, M. L. Dissipative Kerr solitons in optical microresonators. Science 361 , eaan8083 (2018)..

Sohn, D. B., Kim, S. & Bahl, G. Time-reversal symmetry breaking with acoustic pumping of nanophotonic circuits. Nat. Photonics 12 , 91 (2018)..

Henke, J.-W. et al. Integrated photonics enables continuous-beam electron phase modulation. Nature 600 , 653 (2021)..

Yang, Y. et al. Free-electron interaction with nonlinear optical states in microresonators. Science 383 , 168 (2024)..

Byrnes, T., Kim, N. Y. & Yamamoto, Y. Exciton–polariton condensates. Nat. Phys. 10 , 803 (2014)..

Brodier, O., Schlagheck, P. & Ullmo, D. Resonance-assisted tunneling in near-integrable systems. Phys. Rev. Lett. 87 , 064101 (2001)..

Jiang, X. et al. Chaos-assisted broadband momentum transformation in optical microresonators. Science 358 , 344 (2017)..

Jiang, X. et al. Coherent control of chaotic optical microcavity with reflectionless scattering modes. Nat. Phys. 20 , 109 (2024)..

Ge, Z. et al. Direct visualization of relativistic quantum scars in graphene quantum dots. Nature 635 , 841 (2024)..

Zhang, Y., Xu, C., Zhao, Z., Su, Y. & Guo, X. Miniaturized chaos-assisted spectrometer. Light Sci. Appl. 14 , 331 (2025)..

Sun, W. et al. A chip-integrated comb-based microwave oscillator. Light Sci. Appl. 14 , 179 (2025)..

Song, Y., Hu, Y., Lončar, M. & Yang, K. Hybrid Kerr-electro-optic frequency combs on thin-film lithium niobate. Light Sci. Appl. 14 , 270 (2025)..

Song, Y., Hu, Y., Zhu, X., Yang, K. & Lončar, M. Octave-spanning Kerr soliton frequency combs in dispersion-and dissipation-engineered lithium niobate microresonators. Light Sci. Appl. 13 , 225 (2024)..

Farajollahi, S. et al. Multimode perturbation modeling for cavity polygon and star modes. Phys. Rev. A 108 , 033520 (2023)..

Wiersig, J. Perturbative approach to optical mic rodisks with a local boundary deformation. Phys. Rev. A 85 , 063838 (2012)..

Yi, C.-H., Kullig, J. & Wiersig, J. Pair of exceptional points in a microdisk cavity under an extremely weak deformation. Phys. Rev. Lett. 120 , 093902 (2018)..

Fritzsch, F., Ketzmerick, R. & Bäcker, A. Resonance-assisted tunneling in deformed optical microdisks with a mixed phase space. Phys. Rev. E 100 , 042219 (2019)..

Anderson, M. H. et al. Dissipative solitons and switching waves in dispersion-modulated Kerr cavities. Phys. Rev. X 13 , 011040 (2023)..

Moille, G. et al. Versatile optical frequency division with Kerr-induced synchronization at tunable microcomb synthetic dispersive waves. Nat. Photonics 1 , 36–43 (2024)..

Bruch, A. W. et al. Pockels soliton microcomb. Nat. Photonics 15 , 21 (2021)..

Sun, Y. et al. Room-temperature continuous-wave electrically injected InGaN-based laser directly grown on Si. Nat. Photonics 10 , 595 (2016)..

Li, B. et al. High-coherence hybrid-integrated 780 nm source by self-injection-locked second-harmonic generation in a high-Q silicon-nitride resonator. Optica 10 , 1241 (2023)..

Chauhan, N. et al. Ultra-low loss visible light waveguides for integrated atomic, molecular, and quantum photonics. Opt. Express 30 , 6960 (2022)..

Perez, E. F. et al. High-performance Kerr microresonator optical parametric oscillator on a silicon chip. Nat. Commun. 14 , 242 (2023)..

Corato-Zanarella, M., Ji, X., Mohanty, A. & Lipson, M. Absorption and scattering limits of silicon nitride integrated photonics in the visible spectrum. Opt. Express 32 , 5718 (2024)..

Black, J. A. et al. Optical-parametric oscillation in photonic-crystal ring resonators. Optica 9 , 1183 (2022)..

Chen, H.-J. et al. Chaos-assisted two-octave-spanning microcombs. Nat. Commun. 11 , 2336 (2020)..

Lesko, D. M. et al. A six-octave optical frequency comb from a scalable few-cycle erb ium fibre laser. Nat. Photonics 15 , 281 (2021)..

Zhang, C. et al. Frequency ratio of the 229m Th nuclear iso- meric transition and the 87 Sr atomic clock. Nature 633 , 63 (2024)..

Yi, C.-H., Kullig, J., Kim, C.-M. & Wiersig, J. Frequency splittings in deformed optical microdisk cavities. Phys. Rev. A 96 , 023848 (2017)..

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