Deterministic quantum light emitters in DNA origami–engineered molecule–MoS<sub>2</sub> hybrids

Zhijie Li; Shen Zhao; Iuliia Melchakova; Elisabeth Erber; Christoph Sikeler; Kenji Watanabe; Takashi Taniguchi; Tim Liedl; Alexander Högele; Anvar S. Baimuratov; Irina V. Martynenko

doi:10.1038/s41377-026-02204-w

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Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids

Original Articles

- Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids
- Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids
- Light: Science & Applications 2026年15卷第6期页码：1837-1847
- Affiliations：
  
  1.Faculty of Physics and Center for NanoScience (CeNS), Ludwig-Maximilians-Universität München, Geschwister-Scholl-Platz 1, 80539 Munich, Germany
  2.National Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, Nanjing University, Nanjing 210023, China
  3.School of Physics and Engineering, ITMO University, St. Petersburg 197101, Russia
  4.Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
  5.Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
  6.Munich Center for Quantum Science and Technology (MCQST), Schellingstraße 4, 80799 München, Germany
  7.Center for Engineering Physics, Skolkovo Institute of Science and Technology, Bolshoy Boulevard, 30, bld. 1, Moscow 121205, Russia
- Author bio：
  
  Shen Zhao (szhao@nju.edu.cn)
  Anvar S. Baimuratov (a.baimuratov@skoltech.ru)
  Irina V. Martynenko (i.martynenko@skoltech.ru)
- Funds：
- DOI：10.1038/s41377-026-02204-w
  中图分类号：
- 收稿：2025-08-01，
  
  修回：2026-01-18，
  
  录用：2026-01-21，
  
  网络首发：2026-03-09，
  
  纸质出版：2026-06-30
- Accepted：
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Zhijie Li, Shen Zhao, Iuliia Melchakova, 等. Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids[J]. Light: Science & Applications, 2026,15(6):1837-1847. DOI: 10.1038/s41377-026-02204-w.

Li, Z. J. et al. Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids. Light: Science & Applications, 15, 1837-1847 (2026). DOI: 10.1038/s41377-026-02204-w.
Zhijie Li, Shen Zhao, Iuliia Melchakova, 等. Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids[J]. Light: Science & Applications, 2026,15(6):1837-1847. DOI: 10.1038/s41377-026-02204-w. DOI：

Li, Z. J. et al. Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids. Light: Science & Applications, 15, 1837-1847 (2026). DOI: 10.1038/s41377-026-02204-w. DOI：

摘要

Abstract

The functionalization of atomically-thin transition metal dichalcogenides (TMDs) with organic molecules is a promising approach for realizing nanoscale optoelectronic devices with tailored functionalities

such as quantum light gener

ation or

junctions. However

achieving precise control over the molecules' positioning on the 2D material remains a significant challenge. Here

we overcome the limitations of solution- and vapor-deposition methods and use a DNA origami placement technique to spatially arrange thiol molecules on a chip surface at the single-molecule level with high assembly yields. We successfully integrated MoS

monolayers with micron-scale thiol–origami patterns

creating quantum-emitting sites from thiol-induced localized excitons in MoS

. Our work lays a foundation for the chemical control of quantum emitters in atomically-thin semiconductors and enables the design and production of ultracompact 2D devices for quantum technologies.

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references

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Deterministic quantum light emitters in DNA origami–engineered molecule–MoS2 hybrids

Deterministic quantum light emitters in DNA origami–engineered molecule–MoS2 hybrids

DOI：10.1038/s41377-026-02204-w

摘要

Abstract

关键词

Keywords

references

Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids

Deterministic quantum light emitters in DNA origami–engineered molecule–MoS₂ hybrids