
1.Department of Physics, King's College London, Strand, London, WC2R 2LS, UK
2.Department of Electronic Engineering, Queen Mary University of London, London, UK
3.School of Electrical Engineering, Tel Aviv University, Ramat Aviv, Tel Aviv, 69978, Israel
4.ITMO University, St. Petersburg, 197101, Russia
5.Present address: Departamento de Optica, CICESE, Carretera Ensenada-Tijuana, 3918, 22860, Ensenada, Mexico
6.Present address: Laboratory for Optics & Biosciences, Ecole Polytechnique, CNRS UMR 7645, F-91128 Palaiseau, France
7.Present address: Department of Physics, University of North Florida, Jacksonville FL 32224, USA
Alexey V. Krasavin (alexey.krasavin@kcl.ac.uk)
Scan for full text
Krasavin, A. V. et al. Generalization of the optical theorem:experimental proof for radially polarized beams. Light: Science & Applications, 7, 408-417 (2018).
Krasavin, A. V. et al. Generalization of the optical theorem:experimental proof for radially polarized beams. Light: Science & Applications, 7, 408-417 (2018). DOI: 10.1038/s41377-018-0025-x.
The optical theorem, which is a consequence of the energy conservation in scattering processes, directly relates the forward scattering amplitude to the extinction cross-section of the object. Originally derived for planar scalar waves, it neglects the complex structure of the focused beams and the vectorial nature of the electromagnetic field. On the other hand, radially or azimuthally polarized fields and various vortex beams, essential in modern photonic technologies, possess a prominent vectorial field structure. Here, we experimentally demonstrate a complete violation of the commonly used form of the optical theorem for radially polarized beams at both visible and microwave frequencies. We show that a plasmonic particle illuminated by such a beam exhibits strong extinction, while the scattering in the forward direction is zero. The generalized formulation of the optical theorem provides agreement with the observed results. The reported effect is vital for the understanding and design of the interaction of complex vector beams carrying longitudinal field components with subwavelength objects important in imaging, communications, nanoparticle manipulation, and detection, as well as metrology.
Born, M. & Wolf, E. Principles of Optics 7th edn. (Cambridge University Press, New York, 1999).
Jackson, J. D. Classical Electrodynamics 3rd edn. (Wiley, New York, 1999).
Bohren, C. F. & Huffman, D. R. Absorption and Scattering of Light by Small Particles (Wiley, New York, 1998).
Mishchenko, M. I., Travis, L. D. & Lacis, A. A. Scattering, Absorption, and Emission of Light by Small Particles (Cambridge University Press, Cambridge, 2002).
Karlovets, D. V., Kotkin, G. L., Serbo, V. G. & Surzhykov, A. Scattering of twisted electron wave packets by atoms in the Born approximation. Phys. Rev. A 95, 032703 (2017).
Newton, R. G. Optical theorem and beyond. Am. J. Phys. 44, 639–642 (1976).
Lock, J. A., Hodges, J. T. & Gouesbet, G. Failure of the optical theorem for Gaussian-beam scattering by a spherical particle. J. Opt. Soc. Am. A 12, 2708–2715 (1995).
Şendur, K. & Şahinöz, A. Interaction of radially polarized focused light with a prolate spheroidal nanoparticle. Opt. Express 17, 10910–10925 (2009).
Normatov, A. et al. Efficient coupling and field enhancement for the nano-scale: plasmonic needle. Opt. Express 18, 14079–14086 (2010).
Lerman, G. M., Yanai, A. & Levy, U. Demonstration of nanofocusing by the use of plasmonic lens illuminated with radially polarized light. Nano. Lett. 9, 2139–2143 (2009).
Chen, W. B., Abeysinghe, D. C., Nelson, R. L. & Zhan, Q. W. Plasmonic lens made of multiple concentric metallic rings under radially polarized illumination. Nano. Lett. 9, 4320–4325 (2009).
Marengo, E. A. & Tu, J. Optical theorem for transmission lines. Prog. Electromagn. Res. B 61, 253–268 (2014).
Marengo, E. A. & Tu, J. Generalized optical theorem in the time domain. Prog. Electromagn. Res. B 65, 1–18 (2016).
Marengo, E. A. A new theory of the generalized optical theorem in anisotropic media. IEEE Trans. Antennas Propagat 61, 2164–2179 (2013).
Dacol, D. K. & Roy, D. G. Generalized optical theorem for scattering in inhomogeneous media. Phys. Rev. E 72, 036609 (2005).
Halliday, D. & Curtis, A. Generalized optical theorem for surface waves and layered media. Phys. Rev. E 79, 056603 (2008).
Carney, P. S. The optical cross-section theorem with incident fields containing evanescent components. J. Mod. Opt. 46, 891–899 (1999).
Johnson, P. B. & Christy, R. W. Optical constants of the noble metals. Phys. Rev. B 6, 4370–4379 (1972).
Mojarad, N. M. & Agio, M. Tailoring the excitation of localized surface plasmon-polariton resonances by focusing radially-polarized beams. Opt. Express 17, 117–122 (2009).
Gouesbet, G., Lock, J. A. & Gréhan, G. Generalized Lorenz–Mie theories and description of electromagnetic arbitrary shaped beams: Localized approximations and localized beam models, a review. J. Quant. Spectrosc. Radiat. Transf. 112, 1–27 (2011).
Parsons, J., Burrows, C. P., Sambles, J. R. & Barnes, W. L. A comparison of techniques used to simulate the scattering of electromagnetic radiation by metallic nanostructures. J. Mod. Opt. 57, 356–365 (2010).
Stratton, J. A. & Chu, L. J. Diffraction theory of electromagnetic waves. Phys. Rev. 56, 99–107 (1939).
Kapitanova, P. V. et al. Photonic spin Hall effect in hyperbolic metamaterials for polarization-controlled routing of subwavelength modes. Nat. Commun. 5, 3226 (2014).
Balanis, C. A. Antenna Theory: Analysis and Design 3rd edn (Wiley-Interscience, New York, 2005).
Bliokh, K. Y., Rodríguez-Fortuño, F. J., Nori, F. & Zayats, A. V. Spin–orbit interactions of light. Nat. Photonics 9, 796–808 (2015).
Martínez-Herrero, R., Mejías, P. M., Juvells, I. & Carnicer, A. Transverse and longitudinal components of the propagating and evanescent waves associated to radially polarized nonparaxial fields.Appl. Phys. B 106, 151–159 (2012).
Lytle, D. R. II, Carney, P. S., Schotland, J. C. & Wolf, E. Generalized optical theorem for reflection, transmission, and extinction of power for electromagnetic fields. Phys. Rev. E 71, 056610 (2005).
Liou, K. N., Cai, Q., Pollack, J. B. & Cuzzi, J. N. Light scattering by randomly oriented cubes and parallelepipeds. Appl. Opt. 22, 3001–3008 (1983).
Orlov, S., Peschel, U., Bauer, T. & Banzer, P. Analytical expansion of highly focused vector beams into vector spherical harmonics and its application to Mie scattering. Phys. Rev. A 85, 063825 (2012).
O'Connor, D., Ginzburg, P., Rodríguez-Fortuño, F. J., Wurtz, G. A. & Zayats, A. V. Spin–orbit coupling in surface plasmon scattering by nanostructures. Nat. Commun. 5, 5327 (2014).
Rodríguez-Fortuño, F. J., Engheta, N., Martínez, A. & Zayats, A. V. Lateral forces on circularly polarizable particles near a surface. Nat. Commun. 6, 8799 (2015).
Karlovets, D. V., Kotkin, G. L. & Serbo, V. G. Scattering of wave packets on atoms in the Born approximation. Phys. Rev. A 92, 052703 (2015).
Taylor, J. R. Scattering Theory: The Quantum Theory of Nonrelativistic Collisions (Dover Publications Inc., New York, 2006).
0
Views
0
Downloads
0
CSCD
Publicity Resources
Related Articles
Related Author
Related Institution
京公网安备11010802024621