
Optoelectronics Research Centre, University of Southampton, Southampton SO17 1BJ, UK
Masaaki Sakakura (M.Sakakura@soton.ac.uk)
Lei Wang (L.Wang@soton.ac.uk)
Published:2020,
Published Online:04 February 2020,
Received:13 August 2019,
Revised:27 December 2019,
Accepted:14 January 2020
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Sakakura, M. et al. Ultralow-loss geometric phase and polarization shaping by ultrafast laser writing in silica glass. Light: Science & Applications, 9, 141–150 (2020).
Sakakura, M. et al. Ultralow-loss geometric phase and polarization shaping by ultrafast laser writing in silica glass. Light: Science & Applications, 9, 141–150 (2020). DOI: 10.1038/s41377-020-0250-y.
Polarization and geometric phase shaping via a space-variant anisotropy has attracted considerable interest for fabrication of flat optical elements and generation of vector beams with applications in various areas of science and technology. Among the methods for anisotropy patterning
imprinting of self-assembled nanograting structures in silica glass by femtosecond laser writing is promising for the fabrication of space-variant birefringent optics with high thermal and chemical durability and high optical damage threshold. However
a drawback is the optical loss due to the light scattering by nanograting structures
which has limited the application. Here
we report a new type of ultrafast laser-induced modification in silica glass
which consists of randomly distributed nanopores elongated in the direction perpendicular to the polarization
providing controllable birefringent structures with transmittance as high as 99% in the visible and near-infrared ranges and >90% in the UV range down to 330 nm. The observed anisotropic nanoporous silica structures are fundamentally different from the femtosecond laser-induced nanogratings and conventional nanoporous silica. A mechanism of nanocavitation via interstitial oxygen generation mediated by multiphoton and avanlanche defect ionization is proposed. We demonstrate ultralow-loss geometrical phase optical elements
including geometrical phase prism and lens
and a vector beam convertor in silica glass.
Bomzon, Z. et al. Space-variant Pancharatnam-Berry phase optical elements with computer-generated subwavelength gratings.Opt. Lett.27, 1141-1143 (2002)..
Marrucci, L., Manzo, C.&Paparo, D. Pancharatnam-Berry phase optical elements for wave front shaping in the visible domain: switchable helical mode generation.Appl. Phys. Lett.88, 221102 (2006)..
Kim, J. et al. Fabrication of ideal geometric-phase holograms with arbitrary wavefronts.Optica.2, 958-964 (2015)..
Miskiewicz, M. N.&Escuti, M. J. Direct-writing of complex liquid crystal patterns.Opt. Express22, 12691-12706 (2014)..
Genevet, P.&Capasso, F. Holographic optical metasurfaces: a review of current progress.Rep. Prog. Phys.78, 024401 (2015)..
Zheng, G. X. et al. Metasurface holograms reaching 80% efficiency.Nat. Nanotechnol.10, 308-312 (2015)..
Wang, X. W. et al. Dielectric geometric phase optical elements fabricated by femtosecond direct laser writing in photoresists.Appl. Phys. Lett.110, 181101 (2017)..
Zhan, Q. W. Cylindrical vector beams: from mathematical concepts to applications.Adv. Opt. Photonics1, 1-57 (2009)..
D'Ambrosio, V. et al. Arbitrary, direct and deterministic manipulation of vector beams via electrically-tuned q-plates.Sci. Rep.5, 7840 (2015)..
Dorn, R., Quabis, S.&Leuchs, G. Sharper focus for a radially polarized light beam.Phys. Rev. Lett.91, 233901 (2003)..
Hnatovsky, C. et al. Revealing local field structure of focused ultrashort pulses.Phys. Rev. Lett.106, 123901 (2011)..
Karedla, N. et al. Simultaneous measurement of the three-dimensional orientation of excitation and emission dipoles.Phys. Rev. Lett.115, 173002 (2015)..
Salamin, Y. I., Harman, Z.&Keitel, C. H. Direct high-power laser acceleration of ions for medical applications.Phys. Rev. Lett.100, 155004 (2008)..
Guclu, C., Veysi, M.&Capolino, F. Photoinduced magnetic nanoprobe excited by an azimuthally polarized vector beam.ACS Photonics3, 2049-2058 (2016)..
Hernández-García, C. et al. Extreme ultraviolet vector beams driven by infrared lasers.Optica.4, 520-526 (2017)..
Parigi, V. et al. Storage and retrieval of vector beams of light in a multiple-degree-of-freedom quantum memory.Nat. Commun.6, 7706 (2015)..
Milione, G. et al. Higher order Pancharatnam-Berry phase and the angular momentum of light.Phys. Rev. Lett.108, 190401 (2012)..
Della Valle, G., Osellame, R.&Laporta, P. Micromachining of photonic devices by femtosecond laser pulses.J. Opt. A11, 013001 (2009)..
Sugioka, K.&Cheng, Y. Ultrafast lasers—reliable tools for advanced materials processing.Light: Sci. Appl.3, e149 (2014)..
Gattass, R. R.&Mazur, E. Femtosecond laser micromachining in transparent materials.Nat. Photonics2, 219-225 (2008)..
Meany, T. et al. Laser written circuits for quantum photonics.Laser Photonics Rev.9, 363-384 (2015)..
Sotillo, B. et al. Diamond photonics platform enabled by femtosecond laser writing.Sci. Rep.6, 35566 (2016)..
Beresna, M. et al. Radially polarized optical vortex converter created by femtosecond laser nanostructuring of glass.Appl. Phys. Lett.98, 201101 (2011)..
Drevinskas, R.&Kazansky, P. G. High-performance geometric phase elements in silica glass.APL Photonics2, 066104 (2017)..
Shimotsuma, Y. et al. Self-organized nanogratings in glass irradiated by ultrashort light pulses.Phys. Rev. Lett.91, 247405 (2003)..
Bricchi, E., Klappauf, B. G.&Kazansky, P. G. Form birefringence and negative index change created by femtosecond direct writing in transparent materials.Opt. Lett.29, 119-121 (2004)..
Bhardwaj, V. R. et al. Optically produced arrays of planar nanostructures inside fused silica.Phys. Rev. Lett.96, 057404 (2006)..
Richter, S. et al. Nanogratings in fused silica: formation, control, and applications.J. Laser Appl.24, 042008 (2012)..
Drevinskas, R. et al. Ultrafast laser-induced metasurfaces for geometric phase manipulation.Adv. Opt. Mater.5, 1600575 (2017)..
Hnatovsky, C. et al. Pulse duration dependence of femtosecond-laser-fabricated nanogratings in fused silica.Appl. Phys. Lett.87, 014104 (2005)..
Liao, Y. et al. High-fidelity visualization of formation of volume nanogratings in porous glass by femtosecond laser irradiation.Optica.2, 329-334 (2015)..
Brückner, R. Properties and structure of vitreous silica. I.J. Non-Cryst. Solids5, 123-175 (1970)..
Ohfuchi, T. et al. The characteristic of birefringence and optical loss in femtosecond-laser-induced region in terms of nanogratings distribution.J. Laser micro/Nanoen.12, 217-221 (2017)..
Drevinskas, R., Kazansky, P., Cerkauskaite, A. Nanostructured optical element, method for fabrication and uses thereof (2019).
Tsai, T.&Griscom, D. Experimental evidence forexcitonic mechanism of defect generation in high-purity silica.Phys. Rev. Lett.67, 2517-2520 (1991)..
Rudenko, A., Colombier, J. P.&Itina, T. E. Nanopore-mediated ultrashort laser-induced formation and erasure of volume nanogratings in glass.Phys. Chem. Chem. Phys.20, 5887-5899 (2018)..
Canning, J. et al. Anatomy of a femtosecond laser processed silica waveguide [Invited].Optical Mater. Express1, 998-1008 (2011)..
Davis, K. M. et al. Writing waveguides in glass with a femtosecond laser.Opt. Lett.21, 1729-1731 (1996)..
Bellouard, Y. et al. Stress-state manipulation in fused silica via femtosecond laser irradiation.Optica.3, 1285-1293 (2016)..
Sihvola, A. H.&Kong, J. A. Effective permittivity of dielectric mixtures.IEEE Trans. Geosci. Remote Sens.26, 420-429 (1988)..
Cox, A. J., DeWeerd, A. J.&Linden, J. An experiment to measure Mie and Rayleigh total scattering cross sections.Am. J. Phys.70, 620-625 (2002)..
Atkins, P.&De Paula, J.Atkins' Physical Chemistry.10th edn (Oxford University Press, Oxford, 2014).
Lancry, M. et al. Ultrafast nanoporous silica formation driven by femtosecond laser irradiation.Laser Photonics Rev.7, 953-962 (2013)..
El Hamzaoui, H. et al. From porous silica xerogels to bulk optical glasses: the control of densification.Mater. Chem. Phys.121, 83-88 (2010)..
Saeta, P. N.&Greene, B. I. Primary relaxation processes at the band edge of SiO2.Phys. Rev. Lett.70, 3588-3591 (1993)..
Skuja, L. et al. Infrared photoluminescence of preexisting or irradiation-induced interstitial oxygen molecules in glassy SiO2and α-quartz.Phys. Rev. B58, 14296-14304 (1998)..
Mishchik, K. et al. Ultrafast laser induced electronic and structural modifications in bulk fused silica.J. Appl. Phys.114, 133502 (2013)..
Devine, R. A. B.&Arndt, J. Defect pair creation through ultraviolet radiation in dense, amorphous SiO2.Phys. Rev. B42, 2617-2620 (1990)..
Mermillod-Blondin, A. et al. Flipping the sign of refractive index changes in ultrafast and temporally shaped laser-irradiated borosilicate crown optical glass at high repetition rates.Phys. Rev. B77, 104205 (2008)..
Zhang, J. Y. et al. Seemingly unlimited lifetime data storage in nanostructured glass.Phys. Rev. Lett.112, 033901 (2014)..
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