
1.State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai, China
2.Institute of Photonics, TU Wien, Gusshausstrasse 27/387, Vienna, Austria
3.Department of Applied Physics, Nanjing University of Science and Technology, Nanjing, Jiangsu 210094, China
Zhensheng Tao (zhenshengtao@fudan.edu.cn)
Published:30 April 2021,
Published Online:10 March 2021,
Received:12 November 2020,
Revised:07 February 2021,
Accepted:15 February 2021
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Zhang, S. et al. Solitary beam propagation in periodic layered Kerr media enables high-efficiency pulse compression and mode self-cleaning. Light: Science & Applications, 10, 464-474 (2021).
Zhang, S. et al. Solitary beam propagation in periodic layered Kerr media enables high-efficiency pulse compression and mode self-cleaning. Light: Science & Applications, 10, 464-474 (2021). DOI: 10.1038/s41377-021-00495-9.
Generating intense ultrashort pulses with high-quality spatial modes is crucial for ultrafast and strong-field science and can be achieved by nonlinear supercontinuum generation (SCG) and pulse compression. In this work
we propose that the generation of quasi-stationary solitons in periodic layered Kerr media can greatly enhance the nonlinear light-matter interaction and fundamentally improve the performance of SCG and pulse compression in condensed media. With both experimental and theoretical studies
we successfully identify these solitary modes and reveal their unified condition for stability. Space-time coupling is shown to strongly influence the stability of solitons
leading to variations in the spectral
spatial and temporal profiles of femtosecond pulses. Taking advantage of the unique characteristics of these solitary modes
we first demonstrate single-stage SCG and the compression of femtosecond pulses from 170 to 22 fs with an efficiency > 85%. The high spatiotemporal quality of the compressed pulses is further confirmed by high-harmonic generation. We also provide evidence of efficient mode self-cleaning
which suggests rich spatiotemporal self-organization of the laser beams in a nonlinear resonator. This work offers a route towards highly efficient
simple
stable and highly flexible SCG and pulse compression solutions for state-of-the-art ytterbium laser technology.
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