
1.Institute of Materials Research and Engineering, A*STAR (Agency for Science, Technology and Research), 2 Fusionopolis Way, #08-03 Innovis, 138634, Singapore, Singapore
2.Department of Materials Science and Engineering, National University of Singapore, 9 Engineering Drive 1, 117575, Singapore, Singapore
3.Singapore University of Technology and Design, 8 Somapah Road, 487372, Singapore, Singapore
4.Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center, Universidad Autónoma de Madrid, 28049, Madrid, Spain
5.Singapore Institute of Food and Biotechnology Innovation, A*STAR (Agency for Science, Technology and Research), 31 Biopolis Way, #01-02 Nanos, 138669, Singapore, Singapore
Zhaogang Dong (dongz@imre.a-star.edu.sg)
Michel Bosman (msemb@nus.edu.sg)
Joel K. W. Yang (joel_yang@sutd.edu.sg)
Published:28 February 2022,
Published Online:20 January 2022,
Received:26 June 2021,
Revised:01 December 2021,
Accepted:30 December 2021
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Dong, Z. G. et al. Nanoscale mapping of optically inaccessible bound-states-in-the-continuum. Light: Science & Applications, 11, 188-196 (2022).
Dong, Z. G. et al. Nanoscale mapping of optically inaccessible bound-states-in-the-continuum. Light: Science & Applications, 11, 188-196 (2022). DOI: 10.1038/s41377-021-00707-2.
Bound-states-in-the-continuum (BIC) is an emerging concept in nanophotonics with potential impact in applications
such as hyperspectral imaging
mirror-less lasing
and nonlinear harmonic generation. As true BIC modes are non-radiative
they cannot be excited by using propagating light to investigate their optical characteristics. In this paper
for the 1st time
we map out the strong near-field localization of the true BIC resonance on arrays of silicon nanoantennas
via electron energy loss spectroscopy with a sub-1-nm electron beam. By systematically breaking the designed antenna symmetry
emissive quasi-BIC resonances become visible. This gives a unique experimental tool to determine the coherent interaction length
which we show to require at least six neighboring antenna elements. More importantly
we demonstrate that quasi-BIC resonances are able to enhance localized light emission via the Purcell effect by at least 60 times
as compared to unpatterned silicon. This work is expected to enable practical applications of designed
ultra-compact BIC antennas such as for the controlled
localized excitation of quantum emitters.
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