
1.Precision Laser Diagnostics Laboratory, University of Colorado, Boulder, CO, 80309, USA
2.Time and Frequency Division, National Institute of Standards and Technology, Boulder, CO, 80305, USA
3.Department of Physics, University of Colorado, Boulder, CO, 80309, USA
4.Department of Chemistry, University of Colorado, Boulder, CO, 80309, USA
5.Electrical Computer and Energy Engineering, University of Colorado, Boulder, CO, 80309, USA
Nazanin Hoghooghi (nazanin.hoghooghi@colorado.edu)
Scott Diddams (scott.diddams@nist.gov)
Published:31 October 2022,
Published Online:07 September 2022,
Received:18 January 2022,
Revised:18 July 2022,
Accepted:28 July 2022
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Hoghooghi, N. et al. Broadband 1-GHz mid-infrared frequency comb. Light: Science & Applications, 11, 2358-2364 (2022).
Hoghooghi, N. et al. Broadband 1-GHz mid-infrared frequency comb. Light: Science & Applications, 11, 2358-2364 (2022). DOI: 10.1038/s41377-022-00947-w.
Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches
GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed
high spectral resolution
and broad optical bandwidth needed to accurately study complex
transient events in chemistry
combustion
and microscopy. However
such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here
we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 µm. This frequency comb is based on a commercially available 1.56 µm mode-locked laser
robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in
χ
(2)
nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration
this source will simultaneously enable measurements with μs time resolution
1 GHz (0.03 cm
−1
) spectral point spacing and a full bandwidth of
>
5 THz (
>
166 cm
−1
) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.
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