Controlled on-chip fabrication of large-scale perovskite single crystal arrays for high-performance laser and photodetector integration

Zhangsheng Xu; Xun Han; Wenqiang Wu; Fangtao Li; Ru Wang; Hui Lu; Qiuchun Lu; Binghui Ge; Ningyan Cheng; Xiaoyi Li; Guangjie Yao; Hao Hong; Kaihui Liu; Caofeng Pan

doi:10.1038/s41377-023-01107-4

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Controlled on-chip fabrication of large-scale perovskite single crystal arrays for high-performance laser and photodetector integration

Original Articles

- Controlled on-chip fabrication of large-scale perovskite single crystal arrays for high-performance laser and photodetector integration
- Light: Science & Applications Vol. 12, Issue 4, Pages: 558-569(2023)
- Affiliations：
  
  1.CAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of Sciences, Beijing 101400, China
  2.School of Nanoscience and Technology, University of Chinese Academy of Sciences, Beijing 100049, China
  3.College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, China
  4.College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
  5.Center on Nanoenergy Research, School of Physical Science and Technology, Guangxi University, Nanning 530004, China
  6.Information Materials and Intelligent Sensing Laboratory of Anhui Province, Key Laboratory of Structure and Functional Regulation of Hybrid Materials of Ministry of Education, Institutes of Physical Science and Information Technology, Anhui University, Hefei 230601, China
  7.College of Materials Science and Engineering, Ocean University of China, Qingdao 266100, China
  8.State Key Laboratory for Mesoscopic Physics, Frontiers Science Centre for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, China
  9.Songshan Lake Materials Laboratory, Dongguan 523808, China
- Author bio：
  
  Xun Han (hanxun@szu.edu.cn)
  Caofeng Pan (cfpan@binn.cas.cn)
- Funds：
- DOI：10.1038/s41377-023-01107-4
  CLC：
- Published：30 April 2023，
  
  Published Online：8 March 2023，
  
  Received：22 November 2022，
  
  Revised：9 February 2023，
  
  Accepted：15 February 2023
Scan for full text
Xu, Z. S.et al. Controlled on-chip fabrication of large-scale perovskite single crystal arrays for high-performance laser and photodetector integration.Light: Science & Applications,12, 558-569 (2023).
DOI：

Xu, Z. S.et al. Controlled on-chip fabrication of large-scale perovskite single crystal arrays for high-performance laser and photodetector integration.Light: Science & Applications,12, 558-569 (2023). DOI： 10.1038/s41377-023-01107-4.

摘要

Abstract

Metal halide perovskites possess intriguing optoelectronic properties

however

the lack of precise control of on-chip fabrication of the large-scale perovskite single crystal arrays restricts its application in integrated devices. Here

we report a space confinement and antisolvent-assisted crystallization method for the homogeneous perovskite single crystal arrays spanning 100 square centimeter areas. This method enables precise control over the crystal arrays

including different array shapes and resolutions with less than 10%-pixel position variation

tunable pixel dimensions from 2 to 8 μm as well as the in-plane rotation of each pixel. The crystal pixel could serve as a high-quality whispering gallery mode (WGM) microcavity with a quality factor of 2915 and a threshold of 4.14 μJ cm

−2

. Through directly on-chip fabrication on the patterned electrodes

a vertical structured photodetector array is demonstrated with stable photoswitching behavior and the capability to image the input patterns

indicating the potential application in the integrated systems of this method.

关键词

Keywords

references

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