1.Center for Nanophase Materials Science, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA
2.Klipsch School of Electrical and Computer Engineering, New Mexico State University, Las Cruces, NM, 88003, USA
3.Department of Physics and Astronomy, Vanderbilt University, Nashville, TN, 37235, USA
4.Quantum Information Science Group, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA
5.Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA
6.Department of Electrical Engineering and Computer Science, Vanderbilt University Nashville, Nashville, TN, 37235, USA
7.Present address: Chemistry Division, U.S. Naval Research Laboratory, Washington, D.C. 20375, USA.
Jordan A. Hachtel (hachtelja@ornl.gov)
Sang-Yeon Cho (sangycho@nmsu.edu)
纸质出版日期:2019,
网络出版日期:2019-03-20,
收稿日期:2018-12-05,
修回日期:2019-02-02,
录用日期:2019-02-06
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Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators[J]. LSA, 2019,8(2):288-296.
Hachtel, J. A. et al. Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators. Light: Science & Applications, 8, 288-296 (2019).
Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators[J]. LSA, 2019,8(2):288-296. DOI: 10.1038/s41377-019-0136-z.
Hachtel, J. A. et al. Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators. Light: Science & Applications, 8, 288-296 (2019). DOI: 10.1038/s41377-019-0136-z.
Understanding the near-field electromagnetic interactions that produce optical orbital angular momentum (OAM) is crucial for integrating twisted light into nanotechnology. Here
we examine the cathodoluminescence (CL) of plasmonic vortices carrying OAM generated in spiral nanostructures. The nanospiral geometry defines a photonic local density of states that is sampled by the electron probe in a scanning transmission electron microscope (STEM)
thus accessing the optical response of the plasmonic vortex with high spatial and spectral resolution. We map the full spectral dispersion of the plasmonic vortex in spiral structures designed to yield increasing topological charge. Additionally
we fabricate nested nanospirals and demonstrate that OAM from one nanospiral can be coupled to the nested nanospiral
resulting in enhanced luminescence in concentric spirals of like handedness with respect to concentric spirals of opposite handedness. The results illustrate the potential for generating and coupling plasmonic vortices in chiral nanostructures for sensitive detection and manipulation of optical OAM.
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