1.ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
2.ICREA-Institució Catalana de Recerca i Estudis Avançats, Passeig Lluís Companys 23, 08010 Barcelona, Spain
Renwen Yu (renwen.yu@icloud.com)
Javier García de Abajo (javier.garciadeabajo@nanophotonics.es)
纸质出版日期:2020,
网络出版日期:2020-05-18,
收稿日期:2019-12-12,
修回日期:2020-04-20,
录用日期:2020-04-25
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Thermal manipulation of plasmons in atomically thin films[J]. LSA, 2020,9(3):828-838.
Dias, E. J. C., Yu, R. W. & de Abajo, F. J. G. et al. Thermal manipulation of plasmons in atomically thin films. Light: Science & Applications, 9, 828-838 (2020).
Thermal manipulation of plasmons in atomically thin films[J]. LSA, 2020,9(3):828-838. DOI: 10.1038/s41377-020-0322-z.
Dias, E. J. C., Yu, R. W. & de Abajo, F. J. G. et al. Thermal manipulation of plasmons in atomically thin films. Light: Science & Applications, 9, 828-838 (2020). DOI: 10.1038/s41377-020-0322-z.
Nanoscale photothermal effects enable important applications in cancer therapy
imaging and catalysis. These effects also induce substantial changes in the optical response experienced by the probing light
thus suggesting their application in all-optical modulation. Here
we demonstrate the ability of graphene
thin metal films
and graphene/metal hybrid systems to undergo photothermal optical modulation with depths as large as > 70% over a wide spectral range extending from the visible to the terahertz frequency domains. We envision the use of ultrafast pump laser pulses to raise the electron temperature of graphene during a picosecond timescale in which its mid-infrared plasmon resonances undergo dramatic shifts and broadenings
while visible and near-infrared plasmons in the neighboring metal films are severely attenuated by the presence of hot graphene electrons. Our study opens a promising avenue toward the active photothermal manipulation of the optical response in atomically thin materials with potential applications in ultrafast light modulation.
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