1.College of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha, Hunan 410073, China
2.Department of Optics and Optical Engineering, University of Science and Technology of China, Hefei, Anhui 230026, China
3.College of Intelligence Science and Technology, National University of Defense Technology, Changsha, Hunan 410073, China
4.State Key Laboratory of Low Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing 100084, China
5.Department of Physics, Clarendon Laboratory, University of Oxford, Oxford, UK
6.School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China
Chaofan Zhang (c.zhang@nudt.edu.cn)
Kun Huang (huangk17@ustc.edu.cn)
Yulin Chen (yulin.chen@physics.ox.ac.uk)
纸质出版日期:2021-03-31,
网络出版日期:2021-01-21,
收稿日期:2020-08-10,
修回日期:2020-12-25,
录用日期:2020-12-31
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A vacuum ultraviolet laser with a submicrometer spot for spatially resolved photoemission spectroscopy[J]. LSA, 2021,10(3):371-378.
Mao, Y. H. et al. A vacuum ultraviolet laser with a submicrometer spot for spatially resolved photoemission spectroscopy. Light: Science & Applications 10, 371-378 (2021).
A vacuum ultraviolet laser with a submicrometer spot for spatially resolved photoemission spectroscopy[J]. LSA, 2021,10(3):371-378. DOI: 10.1038/s41377-021-00463-3.
Mao, Y. H. et al. A vacuum ultraviolet laser with a submicrometer spot for spatially resolved photoemission spectroscopy. Light: Science & Applications 10, 371-378 (2021). DOI: 10.1038/s41377-021-00463-3.
Vacuum ultraviolet (VUV) lasers have demonstrated great potential as the light source for various spectroscopies
which
if they can be focused into a small beam spot
will not only allow investigation of mesoscopic materials a
nd structures but also find application in the manufacture of nano-objects with excellent precision. In this work
we report the construction of a 177 nm VUV laser that can achieve a record-small (~0.76 μm) focal spot at a long focal length (~45 mm) by using a flat lens without spherical aberration. The size of the beam spot of this VUV laser was tested using a metal grating and exfoliated graphene flakes
and we demonstrated its application in a fluorescence spectroscopy study on pure and Tm
3+
-doped NaYF
4
microcrystals
revealing a new emission band that cannot be observed in the traditional up-conversion process. In addition
this laser system would be an ideal light source for spatially and angle-resolved photoemission spectroscopy.
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