Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion

Alexandros K. Spiliotis; Michalis Xygkis; Michail E. Koutrakis; Konstantinos Tazes; Gregoris K. Boulogiannis; Chrysovalantis S. Kannis; Georgios E. Katsoprinakis; Dimitrios Sofikitis; T. Peter Rakitzis

doi:10.1038/s41377-021-00476-y

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Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion

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- Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion
- Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion
- LSA 2021年10卷第3期页码：341-351
- Affiliations：
  
  1.Foundation for Research and Technology Hellas, Institute of Electronic Structure and Laser, N. Plastira 100, Heraklion, Crete GR-71110, Greece
  2.University of Crete, Department of Physics, Herakleio, Greece Full list of author information is available at the end of the article
  3.Department of Physics, Atomic and Molecular Physics Laboratory, University of Ioannina, University Campus, Ioannina GR-45110, Greece
- Author bio：
  
  T. Peter Rakitzis (ptr@iesl.forth.gr)
- Funds：
- DOI：10.1038/s41377-021-00476-y
  中图分类号：
- 纸质出版日期：2021-03-31，
  
  网络出版日期：2021-02-12，
  
  收稿日期：2020-05-30，
  
  修回日期：2021-01-08，
  
  录用日期：2021-01-18
- Accepted：
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Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion[J]. LSA, 2021,10(3):341-351.

Spiliotis, A. K. et al. Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion.Light: Science & Applications 10, 341-351 (2021).
Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion[J]. LSA, 2021,10(3):341-351. DOI： 10.1038/s41377-021-00476-y.

Spiliotis, A. K. et al. Ultrahigh-density spin-polarized hydrogen isotopes from the photodissociation of hydrogen halides: new applications for laser-ion acceleration, magnetometry, and polarized nuclear fusion.Light: Science & Applications 10, 341-351 (2021). DOI： 10.1038/s41377-021-00476-y.

摘要

Abstract

Recently

our group produced spin-polarized hydrogen (SPH) atoms at densities of at least 10

-3

from the photodissociation of hydrogen halide molecules with circularly polarized UV light and measured them via magnetization-quantum beats with a pickup coil. These densities are approximately 7 orders of magnitude higher than those produced using conventional methods

opening up new fields of application

such as ultrafast magnetometry

the production of polarized MeV and GeV particle beams

such as electron beams with intensities approximately 10

higher than current sources

and the study of polarized nuclear fusion

for which the reaction cross sections of D-T and D-

He reactions are expected to increase by 50% for fully polarized nuclear spins. We review the production

detection

depolarization mechanisms

and potential applications of high-density SPH.

关键词

Keywords

references

Steffens, E.&Haeberli, W. Polarized gas targets.Rep. Prog. Phys.66, 1887-1935 (2003)..

Leader, E.Spin in Particle Physics(Cambridge University Press, 2001).

Paetz gen. Schieck, H. The status of "polarized fusion".Eur. Phys. J. A44, 321-354 (2010)..

Delgado, F.&Fernández-Rossier, J. Spin decoherence of magnetic atoms on surfaces.Prog. Surf. Sci.92, 40-82 (2017)..

Leggett, A. J. Bose-Einstein condensation in the alkali gases: some fundamental concepts.Rev. Mod. Phys.73, 307-356 (2001)..

Budker, D.&Romalis, M. Optical magnetometry.Nat. Phys.3, 227-234 (2007)..

Ardenkjaer-Larsen, J. H. et al. Facing and overcoming sensitivity challenges in biomolecular NMR spectroscopy.Angew. Chem. Int. Ed.54, 9162-9185 (2015)..

Oros, A. M.&Shah, N. J. Hyperpolarized xenon in NMR and MRI.Phys. Med. Biol.49, R105-R153 (2004)..

Sofikitis, D. et al. Ultrahigh-density spin-polarized H and D observed via magnetization quantum beats.Phys. Rev. Lett.121, 083001 (2018)..

Wen, M., Tamburini, M.&Keitel, C. H. Polarized laser-WakeField-accelerated Kiloampere electron beams.Phys. Rev. Lett.122, 214801 (2019)..

Szczerba, D. et al. A polarized hydrogen/deuterium atomic beam source for internal target experiments.Nucl. Instrum. Methods Phys. Res. A: Accelerators, Spectrometers, Detect. Associated Equip.455, 769-781 (2000)..

Clasie, B. et al. Laser-driven target of high-density nuclear-polarized hydrogen gas.Phys. Rev. A73, 020703 (2006)..

Redsun, S. G. et al. Production of highly spin-polarized atomic hydrogen and deuterium by spin-exchange optical pumping.Phys. Rev. A42, 1293-1301 (1990)..

Eppink, A. T. J. B. et al. Production of maximally aligned O(1D) atoms from two-step photodissociation of molecular oxygen.J. Chem. Phys.108, 1305-1308 (1998)..

Rakitzis, T. P.&Kitsopoulos, T. N. Measurement of Cl and Br photofragment alignment using slice imaging.J. Chem. Phys.116, 9228-9231 (2002)..

Chestakov, D. A. et al. Photofragment alignment in the photodissociation of I2from 450 to 510 nm.J. Chem. Phys.124, 024315 (2006)..

Van Brunt, R. J.&Zare, R. N. Polarization of atomic fluorescence excited by molecular dissociation.J. Chem. Phys.48, 4304-4308 (1968)..

Vasyutinskiǐ, O. S. Orientation of atoms during photodissociation of molecules.JETP Lett.31, 428-430 (1980)..

Rakitzis, T. P. et al. Spin-polarized hydrogen atoms from molecular Photodissociation.Science300, 1936-1938 (2003)..

Rakitzis, T. P. Pulsed-laser production and detection of spin-polarized hydrogen atoms.ChemPhysChem5, 1489-1494 (2004)..

Rakitzis, T. P. et al. Measurement of Br photofragment orientation and alignment from HBr photodissociation: production of highly spin-polarized hydrogen atoms.J. Chem. Phys.121, 7222-7227 (2004)..

Rubio-Lago, L. et al. Laser preparation of spin-polarized atoms from molecular photodissociation.Phys. Scr.73, C71-C75 (2006)..

Sofikitis, D. et al. Nanosecond control and high-density production of spin-polarized hydrogen atoms.EPL (Europhys. Lett. )81, 68002 (2008)..

Sofikitis, D. et al. Laser detection of spin-polarized hydrogen from HCl and HBr photodissociation: Comparison of H- and halogen-atom polarizations.J. Chem. Phys.129, 144302 (2008)..

Bougas, L. et al. (2 + 1) laser-induced fluorescence ofspin-polarized hydrogen atoms.J. Chem. Phys.133, 174308 (2010)..

Broderick, B. M. et al. Velocity distribution of hydrogen atom spin polarization.J. Phys. Chem. Lett.4, 3489-3493 (2013)..

Broderick, B. M. et al. Spin-polarized hydrogen Rydberg time-of-flight: experimental measurement of the velocity-dependent H atom spin-polarization.Rev. Sci. Instrum.85, 053103 (2014)..

Broderick, B. M. et al. Imaging detection of spin-polarized hydrogen atoms.Chem. Phys. Lett.635, 350-354 (2015)..

Sofikitis, D. et al. Highly nuclear-spin-polarized deuterium atoms from the UV photodissociation of deuterium Iodide.Phys. Rev. Lett.118, 233401 (2017)..

Balint-Kurti, G. G. et al. Vector correlations and alignment parameters in the photodissociation of HF and DF.J. Chem. Phys.116, 10760-10771 (2002)..

Brown, A., Balint-Kurti, G. G.&Vasyutinskii, O. S. Photodissociation of HCL and DCL: polarization of atomic photofragments.J. Phys. Chem. A108, 7790-7800 (2004)..

Brown, A. Photodissociation of HI and DI: polarization of atomic photofragments.J. Chem. Phys.122, 084301 (2005)..

Jodoin, D. N.&Brown, A. Photodissociation of HI and DI: testing models for electronic structure via polarization of atomic photofragments.J. Chem. Phys.123, 054301 (2005)..

Sofikitis, D. et al. Photofragment spin-polarization measurementsviamagnetization quantum beats: dynamics of DI photodissociation.Phys. Chem. Chem. Phys.21, 14000-14004 (2019)..

Boulogiannis, G. K. et al. Spin-polarized hydrogen depolarization rates at high hydrogen halide pressures: hyperfine depolarization via the HY-H complex.J. Phys. Chem. A123, 8130-8134 (2019)..

Milner, A. A., Korobenko, A.&Milner, V. Ultrafast magnetization of a dense molecular gas with an optical centrifuge.Phys. Rev. Lett.118, 243201 (2017)..

Zelenski, A. N.&Kokhanovski, S. A. A study of spin‐exchange polarization transfer in hydrogen‐rubidium collisions.AIP Conf. Proc.293, 164-172 (1993)..

Ip, J. K. K.&Burns, G. Recombination of iodine atoms by flash photolysis over a wide temperature range. Ⅱ I2in He, Ar, Xe, N2, CO.J. Chem. Phys.56, 3155-3161 (1972)..

Kemaneci, E. et al. Global (volume-averaged) model of inductively coupled chlorine plasma: influence of Cl wall recombination and external heating on continuous and pulse-modulated plasmas.Plasma Sources Sci. Technol.23, 045002 (2014)..

Bykhalo, I. B. et al. Kinetics study of two-channel hydrogen and deuterium atom reactions with interhalogen molecules.Russian Chem. Bull.43, 1637-1645 (1994)..

Baulch, D. L. et al. Evaluated kinetic data for high temperature reactions. Volume 4: homogeneous gas phase reactions of halogen- and cyanide-containing species.J. Phys. Chem. Ref. Data1, 10 (1981)..

Gallagher, A. Collisional depolarization of the Rb 5pand Cs 6pdoublets.Phys. Rev.157, 68-72 (1967)..

Bayram, S. B. et al. Collisional depolarization of Zeeman coherences in the133Cs 6p2P3/2level: double-resonance two-photon polarization spectroscopy.Phys. Rev. A73, 042713 (2006)..

Spiliotis, A. K. et al. Depolarization of spin-polarized hydrogen via spin-exchange collisions with chlorine atoms at ultrahigh density. Preprint athttps://arxiv.org/abs/2101.02675https://arxiv.org/abs/2101.02675(2021).

Jiménez-Martínez, R. et al. High-bandwidth optical magnetometer.J. Optical Soc. Am. B29, 3398-3403 (2012)..

Zheng, H. J. et al. Microwave-free vector magnetometry with nitrogen-vacancy centers along a single axis in diamond.Phys. Rev. Appl.13, 044023 (2020)..

Sirotti, F. et al. Time-resolved surface magnetometry in the nanosecond scale using synchrotron radiation.J. Appl. Phys.83, 1563-1568 (1998)..

Link, G. et al. High time resolution multifrequency EPR of radical pair intermediates in photosynthetic reaction centers: Structure determination on a nanosecond time scale.Z. Physik. Chem.218, 171-191 (2004)..

Zhu, B. J. et al. Ultrafast pulsed magnetic fields generated by a femtosecond laser.Appl. Phys. Lett.113, 072405 (2018)..

Spiliotis, A. K. et al. A nanosecond-resolved atomic hydrogen magnetometer. Preprint athttps://arxiv.org/abs/2010.14579https://arxiv.org/abs/2010.14579(2020).

Wu, Y. T. et al. Polarized electron-beam acceleration driven by vortex laser pulses.N. J. Phys.21, 073052 (2019)..

Hützen, A. et al. Polarized proton beams from laser-induced plasmas.High Power Laser Sci. Eng.7, e16 (2019)..

Jin, L. L. et al. Spin-polarized proton beam generation from gas-jet targets by intense laser pulses.Phys. Rev. E102, 011201 (2020)..

Büscher, M. et al. Polarized beams from laser-plasma accelerators.High. Power Laser Sci. Eng.8, e36 (2020)..

Temporal, M. et al. Ramis. Ignition conditions for inertial confinement fusion targets with a nuclear spin-polarized DT fuel.Nucl. Fusion52, 103011 (2012)..

Hupin, G., Quaglioni, S.&Navrátil, P. Ab initio predictions for polarized deuterium-tritium thermonuclear fusion.Nat. Commun.10, 351 (2019)..

Engels, R. et al. Polarized fusion.Phys. Part. Nucl.45, 341-343 (2014)..

More, R.M. Nuclear spin-polarized fuel in inertial fusion.Phys. Rev. Lett.51, 396-399 (1983)..

Kulsrud, R. M. et al. Fusion reactor plasmas with polarized nuclei.Phys. Rev. Lett.49, 1248-1251 (1982)..

Batz, M. et al.3He spin filter for neutrons.J. Res. Natl Inst. Stand. Technol.110, 293-298 (2005)..

Walker, T. G.&Happer, W. Spin-exchange optical pumping of noble-gas nuclei.Rev. Mod. Phys.69, 629-642 (1997)..

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