In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging

Chen Xie; Remi Meyer; Luc Froehly; Remo Giust; Francois Courvoisier

doi:10.1038/s41377-021-00562-1

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In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging

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- In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging
- In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging
- LSA 2021年10卷第7期页码：1326-1338
- Affiliations：
  
  1.Ultrafast Laser Laboratory, Key Laboratory of Opto-electronic Information Technology of Ministry of Education, School of Precision Instruments and Opto-electronics Engineering, Tianjin University, 300072, Tianjin, China
  2.FEMTO-ST Institute, Univ. Bourgogne Franche-Comté, CNRS, 15B avenue des Montboucons, 25030, Besançon Cedex, France
- Author bio：
  
  Francois Courvoisier (francois.courvoisier@femto-st.fr)
- Funds：
- DOI：10.1038/s41377-021-00562-1
  中图分类号：
- 纸质出版日期：2021-07-31，
  
  网络出版日期：2021-06-16，
  
  收稿日期：2020-11-13，
  
  修回日期：2021-05-03，
  
  录用日期：2021-05-26
- Accepted：
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In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging[J]. LSA, 2021,10(7):1326-1338.

Xie, C. et al. In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging. Light: Science & Applications, 10, 1326-1338 (2021).
In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging[J]. LSA, 2021,10(7):1326-1338. DOI： 10.1038/s41377-021-00562-1.

Xie, C. et al. In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging. Light: Science & Applications, 10, 1326-1338 (2021). DOI： 10.1038/s41377-021-00562-1.

摘要

Abstract

Ultrafast imaging is essential in physics and chemistry to investigate the femtosecond dynamics of nonuniform samples or of phenomena with strong spatial variations. It relies on observing the phenomena induced by an ultrashort laser pump pulse using an ultrashort probe pulse at a later time. Recent years have seen the emergence of very successful ultrafast imaging techniques of single non-reproducible events with extremely high frame rate

based on wavelength or spatial frequency encoding. However

further progress in ultrafast imaging towards high spatial resolution is hampered by the lack of characterization of weak probe beams. For pump–probe experiments realized within solids or liquids

because of the difference in group velocities between pump and probe

the determination of the absolute pump–probe delay depends on the sample position. In addition

pulse-front tilt is a widespread issue

unacceptable for ultrafast imaging

but which is conventionally very difficult to evaluate for the low-intensity probe pulses. Here we show that a pump-induced micro-grating generated from the electronic Kerr effect provides a detailed in-situ characterization of a weak probe pulse. It allows solving the two issues of absolute pump–probe delay determination and pulse-front tilt detection. Our approach is valid whatever the transparent medium with non-negligible Kerr index

whatever the probe pulse polarization and wavelength. Because it is nondestructive and fast to perform

this in-situ probe diagnostic can be repeated to calibrate experimental conditions

particularly in the case where complex wavelength

spatial frequency or polarization encoding is used. We anticipate that this technique will enable previously inaccessible spatiotemporal imaging in a number of fields of ultrafast science at the micro- and nanoscale.

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