Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system
Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system
- Light: Science & Applications 2022年11卷第9期 页码：2065-2076
- Affiliations：
1.Laboratory of All-solid-state Light Sources, Beijing Engineering Research Center, Institute of Semiconductors, Chinese Academy of Sciences, 100083 Beijing, China
2.Synlumin Conuninex (Shanghai) Enterprise Development Co., Ltd., 201401 Shanghai, China
3.Time-wave-space Optical Technology (Xiaogan) Co., Ltd., 432012 Xiaogan, Hubei, China
4.High-dimensional Plasma Sources Technology (Xiaogan) Co., Ltd., 432012 Xiaogan, Hubei, China
- Author bio：
Xuechun Lin (xclin@semi.ac.cn)
- Funds：
DOI：10.1038/s41377-022-00848-y
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Linde Zhang, Jingyuan Zhang, Xiang Wang, 等. Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system[J]. Light: Science & Applications, 2022,11(9):2065-2076.
Zhang, L. D. et al. Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system. Light: Science & Applications, 11, 2065-2076 (2022).
Linde Zhang, Jingyuan Zhang, Xiang Wang, 等. Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system[J]. Light: Science & Applications, 2022,11(9):2065-2076. DOI： 10.1038/s41377-022-00848-y.
Zhang, L. D. et al. Design of coherent wideband radiation process in a Nd3+-doped high entropy glass system. Light: Science & Applications, 11, 2065-2076 (2022). DOI： 10.1038/s41377-022-00848-y.
摘要
Abstract
We discover that the spatially coherent radiation within a certain frequency range can be obtained without a common nonlinear optical process. Conventionally, the emission spectra were obtained by de-exciting excited centers from real excited energy levels to the ground state. Our findings are achieved by deploying a high-entropy glass system (HEGS) doped with neodymium ions. The HEGS exhibits a much broader infrared absorption than common glass systems, which can be attributed to be high-frequency optical branch phonons or allowable multi-phonon processes caused by phonon broadening in the system. A broadened phonon-assisted wideband radiation (BPAWR) is induced if the pump laser is absorbed by the system. The subsequent low-threshold self-absorption coherence modulation (SACM) can be controlled by changing excitation wavelengths, sample size, and doping concentrations. The SACM can be red-shifted through the emission of phonons of the excited species and be blue-shifted by absorbing phonons before they are de-excited. There is a time delay up to 1.66 ns between the pump pulse and the BPAWR when measured after traveling through a 35 mm long sample, which is much longer than the Raman process. The BPAWR-SACM can amplify the centered non-absorption band with a gain up to 26.02 dB. These results reveal that the shift of the novel radiation is determined by the frequency of the non-absorption band near the absorption region, and therefore the emission shifts can be modulated by changing the absorption spectrum. When used in fiber lasers, the BPAWR-SACM process may help to achieve tunability.
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references
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