Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution

Bao-Ying Wen; Jing-Yu Wang; Tai-Long Shen; Zhen-Wei Zhu; Peng-Cheng Guan; Jia-Sheng Lin; Wei Peng; Wei-Wei Cai; Huaizhou Jin; Qing-Chi Xu; Zhi-Lin Yang; Zhong-Qun Tian; Jian-Feng Li

doi:10.1038/s41377-022-00918-1

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Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution

Original Articles

- Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution
- Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution
- Light: Science & Applications 2022年11卷第9期页码：2107-2114
- Affiliations：
  
  1.Department of Physics, State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China
  2.Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), Xiamen, 361005, China
  3.College of Optical and Electronic Technology, Jiliang University, Hangzhou, 310018, China
- Author bio：
  
  Huaizhou Jin (jinhz@xmu.edu.cn)
  Qing-Chi Xu (xuqingchi@xmu.edu.cn)
  Zhi-Lin Yang (zlyang@xmu.edu.cn)
  Jian-Feng Li (li@xmu.edu.cn)
- Funds：
- DOI：10.1038/s41377-022-00918-1
  中图分类号：
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Bao-Ying Wen, Jing-Yu Wang, Tai-Long Shen, 等. Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution[J]. Light: Science & Applications, 2022,11(9):2107-2114.

Wen, B. Y. et al. Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution. Light: Science & Applications, 11, 2107-2114 (2022).
Bao-Ying Wen, Jing-Yu Wang, Tai-Long Shen, 等. Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution[J]. Light: Science & Applications, 2022,11(9):2107-2114. DOI： 10.1038/s41377-022-00918-1.

Wen, B. Y. et al. Manipulating the light-matter interactions in plasmonic nanocavities at 1 nm spatial resolution. Light: Science & Applications, 11, 2107-2114 (2022). DOI： 10.1038/s41377-022-00918-1.

摘要

Abstract

The light-matter interaction between plasmonic nanocavity and exciton at the sub-diffraction limit is a central research field in nanophotonics. Here, we demonstrated the vertical distribution of the light-matter interactions at ~1 nm spatial resolution by coupling A excitons of MoS,2, and gap-mode plasmonic nanocavities. Moreover, we observed the significant photoluminescence (PL) enhancement factor reaching up to 2800 times, which is attributed to the Purcell effect and large local density of states in gap-mode plasmonic nanocavities. Meanwhile, the theoretical calculations are well reproduced and support the experimental results.

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references

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