1.Department of Optics and Mechatronics Engineering, College of Nanoscience and Nanotechnology, Pusan National University, 2 Busandaehak-ro 63beon-gil, Busan 46241, South Korea
2.Department of Cogno Mechatronics Engineering, College of Nanoscience and Nanotechnology, Pusan National University, 2 Busandaehak-ro 63beon-gil, Busan 46241, South Korea
3.Max Planck Center for Attosecond Science, Max Planck POSTECH/Korea Research Initiative, 77 Cheongam-ro, Pohang 37673, South Korea
4.Department of Physics, Center for Attosecond Science and Technology, Pohang University of Science and Technology, 77 Cheongam-ro, Pohang 37673, South Korea
Alexander Gliserin (alex@mpk.or.kr)
Seungchul Kim (s.kim@pusan.ac.kr)
Dong Eon Kim (kimd@postech.ac.kr)
纸质出版日期:2022-10-31,
网络出版日期:2022-09-20,
收稿日期:2022-04-04,
修回日期:2022-08-23,
录用日期:2022-08-31
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Complete characterization of ultrafast optical fields by phase-preserving nonlinear autocorrelation[J]. LSA, 2022,11(10):2451-2462.
Gliserin, A. et al. Complete characterization of ultrafast optical fields by phase-preserving nonlinear autocorrelation. Light: Science & Applications, 11, 2451-2462 (2022).
Complete characterization of ultrafast optical fields by phase-preserving nonlinear autocorrelation[J]. LSA, 2022,11(10):2451-2462. DOI: 10.1038/s41377-022-00978-3.
Gliserin, A. et al. Complete characterization of ultrafast optical fields by phase-preserving nonlinear autocorrelation. Light: Science & Applications, 11, 2451-2462 (2022). DOI: 10.1038/s41377-022-00978-3.
Nonlinear autocorrelation was one of the earliest and simplest tools for obtaining partial temporal information about an ultrashort optical pulse by gating it with itself. However
since the spectral phase is lost in a conventional autocorrelation measurement
it is insufficient for a full characterization of an ultrafast electric field
requiring additional spectral information for phase retrieval. Here
we show that introducing an intensity asymmetry into a conventional nonlinear interferometric autocorrelation preserves some spectral phase information within the autocorrelation signal
which enables the full reconstruction of the original electric field
including the direction of time
using only a spectrally integrating detector. We call this technique
Phase
-
Enabled Nonlinear Gating with Unbalanced Intensity
(PENGUIN). It can be applied to almost any existing nonlinear interferometric autocorrelator
making it capable of complete optical field characterization and thus providing an inexpensive and less complex alternative to methods relying on spectral measurements
such as frequency-resolved optical gating (FROG) or spectral phase interferometry for direct electric-field reconstruction (SPIDER). More importantly
PENGUIN allows the precise characterization of ultrafast fields in non-radiative (e.g.
plasmonic) nonlinear optical interactions where spectral information is inaccessible. We demonstrate this novel technique through simulations and experimentally by measuring the electric field of ~6-fs laser pulses from a Ti: sapphire oscillator. The results are validated by comparison with the well-established FROG method.
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