1.Catalan Institute of Nanoscience and Nanotechnology (ICN2), BIST and CSIC, Campus UAB, Bellaterra, Barcelona 08193, Spain
2.Department of Applied Physics, TU Eindhoven, Den Dolech 2, 5612 AZ Eindhoven, The Netherlands
3.School of Physics and Astronomy, University of Manchester, M13 9PL Manchester, UK
4.Physikalisches Institut (EP3), Universität Würzburg, Am Hubland, 97074 Würzburg, Germany
5.Institute of Physics, Polish Academy of Science, Al. Lotnikow 32/46, PL-02668 Warsaw, Poland
6.Helmholtz-Zentrum Dresden-Rossendorf, Bautzner Landstr. 400, 01328 Dresden, Germany
7.ICREA, Pg. Lluís Companys 23, 08010 Barcelona, Spain
8.Institute for Topological Insulators, Am Hubland, D-97074 Würzburg, Germany
Klaas-Jan Tielrooij (klaas.tielrooij@icn2.cat)
Georgy V. Astakhov (g.astakhov@hzdr.de)
Sergey Kovalev (s.kovalev@hzdr.de)
纸质出版日期:2022-11-30,
网络出版日期:2022-11-01,
收稿日期:2022-06-29,
修回日期:2022-09-07,
录用日期:2022-10-08
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Milliwatt terahertz harmonic generation from topological insulator metamaterials[J]. LSA, 2022,11(11):2766-2773.
Tielrooij, K. J. et al. Milliwatt terahertz harmonic generation from topological insulator metamaterials. Light: Science & Applications, 11, 2766-2773 (2022).
Milliwatt terahertz harmonic generation from topological insulator metamaterials[J]. LSA, 2022,11(11):2766-2773. DOI: 10.1038/s41377-022-01008-y.
Tielrooij, K. J. et al. Milliwatt terahertz harmonic generation from topological insulator metamaterials. Light: Science & Applications, 11, 2766-2773 (2022). DOI: 10.1038/s41377-022-01008-y.
Achieving efficient
high-power harmonic generation in the terahertz spectral domain has technological applications
for example
in sixth generation (6G) communication networks. Massless Dirac fermions possess extremely large terahertz nonlinear susceptibilities and harmonic conversion efficiencies. However
the observed maximum generated harmonic power is limited
because of saturation effects at increasing incident powers
as shown recently for graphene. Here
we demonstrate room-temperature terahertz harmonic generation in a Bi
2
Se
3
topological insulator and topological-insulator-grating metamaterial structures with surface-selective terahertz field enhancement. We obtain a third-harmonic power approaching the milliwatt range for an incident power of 75 mW—an improvement by two orders of magnitude compared to a benchmarked graphene sample. We establish a framework in which this exceptional performance is the result of thermodynamic harmonic generation by the massless topological surface states
benefiting from ultrafast dissipation of electronic heat via surface-bulk Coulomb interactions. These results are an important step towards on-chip terahertz (opto)electronic applications.
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