Self-optimized single-nanowire photoluminescence thermometry

Zhang Liang; Jinhua Wu; Ying Cui; Hao Sun; Cun-Zheng Ning

doi:10.1038/s41377-023-01070-0

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Self-optimized single-nanowire photoluminescence thermometry

Original Articles

- Self-optimized single-nanowire photoluminescence thermometry
- Self-optimized single-nanowire photoluminescence thermometry
- 光：科学与应用 2023年12卷第2期页码：259-271
- Affiliations：
  
  1.Department of Electronic Engineering, Tsinghua University, 100084, Beijing, China
  2.College of Integrated Circuits and Optoelectronic Chips, Shenzhen Technology University, 518118, Shenzhen, Guangdong, China
- Author bio：
  
  Cun-Zheng Ning (ningcunzheng@sztu.edu.cn)
- Funds：
- DOI：10.1038/s41377-023-01070-0
  中图分类号：
- 纸质出版日期：2023-2-28，
  
  网络出版日期：2023-2-6，
  
  收稿日期：2022-10-14，
  
  修回日期：2022-12-22，
  
  录用日期：2023-1-2
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Self-optimized single-nanowire photoluminescence thermometry[J]. 光：科学与应用, 2023,12(2):259-271.

Liang, Z. et al. Self-optimized single-nanowire photoluminescence thermometry. Light: Science & Applications, 12, 259-271 (2023).
Self-optimized single-nanowire photoluminescence thermometry[J]. 光：科学与应用, 2023,12(2):259-271. DOI： 10.1038/s41377-023-01070-0.

Liang, Z. et al. Self-optimized single-nanowire photoluminescence thermometry. Light: Science & Applications, 12, 259-271 (2023). DOI： 10.1038/s41377-023-01070-0.

摘要

Abstract

Nanomaterials-based photoluminescence thermometry (PLT) is a new contact-free photonic approach for temperature sensing

important for applications ranging from quantum technology to biomedical imaging and diagnostics. Even though numerous new materials have been explored

great challenges and deficiencies remain that hamper many applications. In contrast to most of the existing approaches that use large ensembles of rare-earth-doped nanomaterials with large volumes and unavoidable inhomogeneity

we demonstrate the ultimate size reduction and simplicity of PLT by using only a single erbium-chloride-silicate (ECS) nanowire. Importantly

we propose and demonstrate a novel strategy that contains a self-optimization or "smart" procedure to automatically identify the best PL intensity ratio for temperature sensing. The automated procedure is used to self-optimize key sensing metrics

such as sensitivity

precision

or resolution to achieve an all-around superior PLT including several record-setting metrics including the first sensitivity exceeding 100% K

−1

(~138% K

−1

)

the highest resolution of 0.01 K

and the largest range of sensible temperatures 4–500 K operating completely within 1500–1800 nm (an important biological window). The high-quality ECS nanowire enables the use of well-resolved Stark-sublevels to construct a series of PL intensity ratios for optimization in infrared

allowing the completely Boltzmann-based sensing at cryogenic temperature for the first time. Our single-nanowire PLT and the proposed optimization strategy overcome many existing challenges and could fundamentally impact PL nano-thermometry and related applications such as single-cell thermometry.

关键词

Keywords

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