Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames

Yogeshwar Nath Mishra; Peng Wang; Florian J. Bauer; Yide Zhang; Dag Hanstorp; Stefan Will; Lihong V. Wang

doi:10.1038/s41377-023-01095-5

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Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames

Original Articles

- Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames
- Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames
- 光：科学与应用 2023年12卷第3期页码：379-390
- Affiliations：
  
  1.Caltech Optical Imaging Laboratory, Andrew and Peggy Cherng Department of Medical Engineering, Department of Electrical Engineering, California Institute of Technology, 1200 East California Boulevard, Mail Code 138-78, Pasadena, CA, 91125, USA
  2.NASA-Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Drive, Pasadena, CA, 91109, USA
  3.Department of Physics, University of Gothenburg, SE 41296, Gothenburg, Sweden
  4.Institute of Engineering Thermodynamics (LTT) and Erlangen Graduate School in Advanced Optical Technologies (SAOT), Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), 91058, Erlangen, Germany
- Author bio：
  
  Lihong V. Wang (LVW@caltech.edu)
- Funds：
- DOI：10.1038/s41377-023-01095-5
  中图分类号：
- 纸质出版日期：2023-3-31，
  
  网络出版日期：2023-2-21，
  
  收稿日期：2022-11-21，
  
  修回日期：2023-1-27，
  
  录用日期：2023-2-5
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Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames[J]. 光：科学与应用, 2023,12(3):379-390.

Mishra, Y. N. et al. Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames. Light: Science & Applications, 12, 379-390 (2023).
Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames[J]. 光：科学与应用, 2023,12(3):379-390. DOI： 10.1038/s41377-023-01095-5.

Mishra, Y. N. et al. Single-pulse real-time billion-frames-per-second planar imaging of ultrafast nanoparticle-laser dynamics and temperature in flames. Light: Science & Applications, 12, 379-390 (2023). DOI： 10.1038/s41377-023-01095-5.

摘要

Abstract

Unburnt hydrocarbon flames produce soot

which is the second biggest contributor to global warming and harmful to human health. The state-of-the-art high-speed imaging techniques

developed to study non-repeatable turbulent flames

are limited to million-frames-per-second imaging rates

falling short in capturing the dynamics of critical species. Unfortunately

these techniques do not provide a complete picture of flame-laser interactions

important for understanding soot formation. Furthermore

thermal effects induced by multiple consecutive pulses modify the optical properties of soot nanoparticles

thus making single-pulse imaging essential. Here

we report single-shot laser-sheet compressed ultrafast photography (LS-CUP) for billion-frames-per-second planar imaging of flame-laser dynamics. We observed laser-induced incandescence

elastic light scattering

and fluorescence of soot precursors - polycyclic aromatic hydrocarbons (PAHs) in real-time using a single nanosecond laser pulse. The spatiotemporal maps of the PAHs emission

soot temperature

primary nanoparticle size

soot aggregate size

and the number of monomers

present strong experimental evidence in support of the theory and modeling of soot inception and growth mechanism in flames. LS-CUP represents a generic and indispensable tool that combines a portfolio of ultrafast combustion diagnostic techniques

covering the entire lifecycle of soot nanoparticles

for probing extremely short-lived (picoseconds to nanoseconds) species in the spatiotemporal domain in non-repeatable turbulent environments. Finally

LS-CUP's unparalleled capability of ultrafast wide-field temperature imaging in real-time is envisioned to unravel mysteries in modern physics such as hot plasma

sonoluminescence

and nuclear fusion.

关键词

Keywords

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