1.University of Pécs, Pécs 7624, Hungary
2.Szentágothai Research Centre, Pécs 7624, Hungary
3.HUN-REN-PTE High-Field Terahertz Research Group, Pécs 7624, Hungary
János Hebling (hebling@fizika.ttk.pte.hu)
纸质出版日期:2023-11-30,
网络出版日期:2023-10-24,
收稿日期:2023-05-31,
修回日期:2023-09-08,
录用日期:2023-09-21
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Tilted pulse front pumping techniques for efficient terahertz pulse generation[J]. LSA, 2023,12(11):2291-2308.
Tóth, G., Polónyi, G. & Hebling, J. Tilted pulse front pumping techniques for efficient terahertz pulse generation. Light: Science & Applications, 12, 2291-2308 (2023).
Tilted pulse front pumping techniques for efficient terahertz pulse generation[J]. LSA, 2023,12(11):2291-2308. DOI: 10.1038/s41377-023-01293-1.
Tóth, G., Polónyi, G. & Hebling, J. Tilted pulse front pumping techniques for efficient terahertz pulse generation. Light: Science & Applications, 12, 2291-2308 (2023). DOI: 10.1038/s41377-023-01293-1.
Optical rectification of femtosecond laser pulses has emerged as the dominant technique for generating single- and few-cycle terahertz (THz) pulses. The advent of the tilted pulse front pumping (TPFP) velocity matching technique
proposed and implemented two decades ago
has ushered in significant advancements of these THz sources
which are pivotal in the realm of THz pump-probe and material control experiments
which need THz pulses with microjoule energies and several hundred kV/cm electric field strengths. Furthermore
these THz sources are poised to play a crucial role in the realization of THz-driven particle accelerators
necessitating millijoule-level pulses with tens of MV/cm electric field strengths. TPFP has enabled the efficient velocity matching in lithium niobate crystals renowned for their extraordinary high nonlinear coefficient. Moreover
its adaptation to semiconductor THz sources has resulted in a two-hundred-times enhancement in conversion efficiency. In this comprehensive review
we present the seminal achievements of the past two decades. We expound on the conventional TPFP setup
delineate its scaling limits
and elucidate the novel generation TPFP configurations proposed to surmount these constraints
accompanied by their preliminary outcomes. Additionally
we provide an in-depth analysis of the THz absorption
refractive index
and nonlinear coefficient spectra of lithium niobate and widely used semiconductors employed as THz generators
which dictate their suitability as THz sources. We underscore the far-reaching advantages of tilted pulse front pumping
not only for LN and semiconductor-based THz sources but also for selected organic crystal-based sources and Yb-laser-pumped GaP sources
previously regarded as velocity-matched in the literature.
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