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    Vol. 6 , Issue 1 , 2017

      Original Articles

    • Ihar Babushkin,Ayhan Tajalli,Hakan Sayinc,Uwe Morgner,Günter Steinmeyer,Ayhan Demircan
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.218
      Abstract:Fiber supercontinua represent light sources of pivotal importance for a wide range of applications, ranging from optical communications to frequency metrology. Although spectra encompassing more than three octaves can be produced, the applicability of such spectra is strongly hampered due to coherence degradation during spectral broadening. Assuming pulse parameters at the cutting edge of currently available laser technology, we demonstrate the possibility of strongly coherent supercontinuum generation. In a fiber with two zero-dispersion wavelengths a higher-order soliton experiences a temporal breakdown, without any compression or splitting behavior, which leads to nearly complete conversion of input solitonic radiation into resonant nonsolitonic radiation in the dispersive wave regime. As the process is completely deterministic and shows little sensitivity to input noise, the resulting pulses appear to be compressible down to the sub-cycle level and may thus hold a new opportunity for direct generation of attosecond pulses in the visible to near ultraviolet wavelength range.  
      Keywords:attosecond pulses;optical solitons;supercontinuum;ultrashort pulses   
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      Published:2024-09-19
    • Alok Kumar Singh,Dinesh N Naik,Giancarlo Pedrini,Mitsuo Takeda,Wolfgang Osten
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.219
      Abstract:Scattering media, such as diffused glass and biological tissue, are usually treated as obstacles in imaging. To cope with the random phase introduced by a turbid medium, most existing imaging techniques recourse to either phase compensation by optical means or phase recovery using iterative algorithms, and their applications are often limited to two-dimensional imaging. In contrast, we utilize the scattering medium as an unconventional imaging lens and exploit its lens-like properties for lensless three-dimensional (3D) imaging with diffraction-limited resolution. Our spatially incoherent lensless imaging technique is simple and capable of variable focusing with adjustable depths of focus that enables depth sensing of 3D objects that are concealed by the diffusing medium. Wide-field imaging with diffraction-limited resolution is verified experimentally by a single-shot recording of the 1951 USAF resolution test chart, and 3D imaging and depth sensing are demonstrated by shifting focus over axially separated objects.  
      Keywords:intensity correlation technique;lensless imaging;scattering media;3D imaging   
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      Published:2024-09-19
    • Maria Principe,Marco Consales,Alberto Micco,Alessio Crescitelli,Giuseppe Castaldi,Emanuela Esposito,Vera La Ferrara,Antonello Cutolo,Vincenzo Galdi,Andrea Cusano
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.226
      Abstract:We report on the first demonstration of a proof-of-principle optical fiber 'meta-tip', which integrates a phase-gradient plasmonic metasurface on the fiber tip. For illustration and validation purposes, we present numerical and experimental results pertaining to various prototypes implementing generalized forms of the Snell's transmission/reflection laws at near-infrared wavelengths. In particular, we demonstrate several examples of beam steering and coupling with surface waves, in fairly good agreement with theory. Our results constitute a first step toward the integration of unprecedented (metasurface-enabled) light-manipulation capabilities in optical-fiber technology. By further enriching the emergent 'lab-on-fiber' framework, this may pave the way for the widespread diffusion of optical metasurfaces in real-world applications to communications, signal processing, imaging and sensing.  
      Keywords:Fiber optics;metasurfaces;plasmonics;wavefront manipulation   
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      Published:2024-09-19
    • Jiang-Lai Wu,Yi-Qing Xu,Jing-Jiang Xu,Xiao-Ming Wei,Antony CS Chan,Anson HL Tang,Andy KS Lau,Bob MF Chung,Ho Cheung Shum,Edmund Y Lam,Kenneth KY Wong,Kevin K Tsia
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.196
      Abstract:Optical time-stretch imaging enables the continuous capture of non-repetitive events in real time at a line-scan rate of tens of MHz—a distinct advantage for the ultrafast dynamics monitoring and high-throughput screening that are widely needed in biological microscopy. However, its potential is limited by the technical challenge of achieving significant pulse stretching (that is, high temporal dispersion) and low optical loss, which are the critical factors influencing imaging quality, in the visible spectrum demanded in many of these applications. We present a new pulse-stretching technique, termed free-space angular-chirp-enhanced delay (FACED), with three distinguishing features absent in the prevailing dispersive-fiber-based implementations: (1) it generates substantial, reconfigurable temporal dispersion in free space (> 1 ns nm−1) with low intrinsic loss (< 6 dB) at visible wavelengths; (2) its wavelength-invariant pulse-stretching operation introduces a new paradigm in time-stretch imaging, which can now be implemented both with and without spectral encoding; and (3) pulse stretching in FACED inherently provides an ultrafast all-optical laser-beam scanning mechanism at a line-scan rate of tens of MHz. Using FACED, we demonstrate not only ultrafast laser-scanning time-stretch imaging with superior bright-field image quality compared with previous work but also, for the first time, MHz fluorescence and colorized time-stretch microscopy. Our results show that this technique could enable a wider scope of applications in high-speed and high-throughput biological microscopy that were once out of reach.  
      Keywords:optical time-stretch imaging;pulse stretching;ultrafast laser scanning   
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      Published:2024-09-19
    • Jiahao Yan,Churong Ma,Pu Liu,Chengxin Wang,Guowei Yang
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.197
      Abstract:Effective interactions between excitons and resonating nanocavities are important for many emerging applications in nanophotonics. Although plasmonic nanocavities are considered promising substitutes for diffraction-limited dielectric microcavities, their practical applications are hindered by large ohmic loss and Joule heating. Other than plasmonic materials, high-refractive-index dielectric nanocavities is a new way to trap light in subwavelength scales. However, studies on the interaction between dielectric nanocavities and excitons are still scarce. Here, for the first time, we demonstrate that the Fano interference between molecular excitons and an individual silicon nanogroove can generate scattering dark modes. By placing J-aggregate excitons into a silicon nanogroove, the leaky magnetic resonant modes filling in the groove can tailor their scattering directivity and reduce the uncoupled radiation decay in a specific direction. This unidirectional 'dark state' brings a new approach to tailor the interaction between excitons and nanocavities without large near-field enhancement. By adjusting the resonant modes, the scattering spectra can change from a Fano asymmetric line shape to a significantly suppressed scattering dip. These findings indicate that silicon nanogrooves can provide a platform for integrated on-chip silicon–exciton hybrid optical systems in the future.  
      Keywords:excitons;light–matter interactions;magnetic mode;silicon nanogroove   
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      Published:2024-09-19
    • Yang Mei,Guo-En Weng,Bao-Ping Zhang,Jian-Ping Liu,Werner Hofmann,Lei-Ying Ying,Jiang-Yong Zhang,Zeng-Cheng Li,Hui Yang,Hao-Chung Kuo
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.199
      Abstract:Semiconductor vertical-cavity surface-emitting lasers (VCSELs) with wavelengths from 491.8 to 565.7 nm, covering most of the 'green gap', are demonstrated. For these lasers, the same quantum dot (QD) active region was used, whereas the wavelength was controlled by adjusting the cavity length, which is difficult for edge-emitting lasers. Compared with reports in the literature for green VCSELs, our lasers have set a few world records for the lowest threshold, longest wavelength and continuous-wave (CW) lasing at room temperature. The nanoscale QDs contribute dominantly to the low threshold. The emitting wavelength depends on the electron–photon interaction or the coupling between the active layer and the optical field, which is modulated by the cavity length. The green VCSELs exhibit a low-thermal resistance of 915 kW−1, which benefits the CW lasing. Such VCSELs are important for small-size, low power consumption full-color displays and projectors.  
      Keywords:GaN;InGaN;quantum dot;vertical-cavity surface-emitting laser;wide-gap semiconductor   
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      Published:2024-09-19
    • Victor Brasch,Erwan Lucas,John D Jost,Michael Geiselmann,Tobias J Kippenberg
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.202
      Abstract:Self-referencing turns pulsed laser systems into self-referenced frequency combs. Such frequency combs allow counting of optical frequencies and have a wide range of applications. The required optical bandwidth to implement self-referencing is typically obtained via nonlinear broadening in optical fibers. Recent advances in the field of Kerr frequency combs have provided a path toward the development of compact frequency comb sources that provide broadband frequency combs, exhibit microwave repetition rates and are compatible with on-chip photonic integration. These devices have the potential to significantly expand the use of frequency combs. Yet to date, self-referencing of such Kerr frequency combs has only been attained by applying conventional, fiber-based broadening techniques. Here we demonstrate external broadening-free self-referencing of a Kerr frequency comb. An optical spectrum spanning two-thirds of an octave is directly synthesized from a continuous wave laser-driven silicon nitride microresonator using temporal dissipative Kerr soliton formation and soliton Cherenkov radiation. Using this coherent bandwidth and two continuous wave transfer lasers in a 2f–3f self-referencing scheme, we are able to detect the offset frequency of the soliton Kerr frequency comb. By stabilizing the repetition rate to a radio frequency reference, the self-referenced frequency comb is used to count and track the continuous wave pump laser's frequency. This work demonstrates the principal ability of soliton Kerr frequency combs to provide microwave-to-optical clockworks on a chip.  
      Keywords:frequency combs;integrated optics;Kerr frequency combs;metrology;microresonator frequency combs;nonlinear optics   
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      Published:2024-09-19
    • Qingyang Xu,Teng Ma,Mohammad Danesh,Bannur Nanjunda Shivananju,Sheng Gan,Jingchao Song,Cheng-Wei Qiu,Hui-Ming Cheng,Wencai Ren,Qiaoliang Bao
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.204
      Abstract:We used scattering-type scanning near-field optical microscopy (s-SNOM) to investigate the plasmonic properties of edges in well-defined graphene nanostructures, including sharp tapers, nanoribbons and nanogaps, which were all fabricated via the growth-etching chemical vapor deposition (GECVD) method. The obtained near-field images revealed the localized plasmon modes along the graphene nanoribbon; these modes strongly depended on the size of the graphene pattern, the angle of the tapered graphene and the infrared excitation wavelength. These interesting plasmon modes were verified by numerical simulations and explained by the reflection, and interference of electromagnetic waves at the graphene–SiO2 edge. The constructive interference at the graphene nanogap caused by charge accumulation was demonstrated for the first time. Using the infrared nanoimaging technique, greater plasmon broadening was observed in the zigzag edge than in the armchair edge. Our study suggests that graphene edges should be separated by an effective working distance to avoid the overlapping of localized plasmon modes, which is very important for the design of graphene-based plasmonic circuits and devices.  
      Keywords:edge chirality;graphene;graphene plasmon;nanoribbon;nanogap;near-field microscopy;s-SNOM   
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      Published:2024-09-19
    • Zhi-Yu Chen,Lian-Shan Yan,Yan Pan,Lin Jiang,An-Lin Yi,Wei Pan,Bin Luo
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.207
      Abstract:Increasing the system capacity and spectral efficiency (SE) per unit bandwidth is one of the ultimate goals for data network designers, especially when using technologies compatible with current embedded fiber infrastructures. Among these, the polarization-division-multiplexing (PDM) scheme, which supports two independent data channels on a single wavelength with orthogonal polarization states, has become a standard one in most state-of-art telecommunication systems. Currently, however, only two polarization states (that is, PDM) can be used, setting a barrier for further SE improvement. Assisted by coherent detection and digital signal processing, we propose and experimentally demonstrate a scheme for pseudo-PDM of four states (PPDM-4) by manipulation of four linearly polarized data channels with the same wavelength. Without any modification of the fiber link, we successfully transmit a 100-Gb s−1 PPDM-4 differential-phase-shift-keying signal over a 150-km single-mode fiber link. Such a method is expected to open new possibilities to fully explore the use of polarization freedom for capacity and SE improvement over existing fiber systems.  
      Keywords:coherent detection;optical communication;pseudo-polarization-division multiplexing;spectral efficiency   
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      Published:2024-09-19
    • Raphael Florentin,Vincent Kermene,Joel Benoist,Agnès Desfarges-Berthelemot,Dominique Pagnoux,Alain Barthélémy,Jean-Pierre Huignard
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.208
      Abstract:Propagation of light in multimode optical fibers usually gives a spatial and temporal randomization of the transmitted field similar to the propagation through scattering media. Randomization still applies when scattering or multimode propagation occurs in gain media. We demonstrate that appropriate structuration of the input beam wavefront can shape the light amplified by a rare-earth-doped multimode fiber. Profiling of the wavefront was achieved by a deformable mirror in combination with an iterative optimization process. We present experimental results and simulations showing the shaping of a single sharp spot at different places in the output cross-section of an ytterbium-doped fiber amplifier. Cleaning and narrowing of the amplifier far-field pattern was realized as well. Tailoring the wavefront to shape the amplified light can also serve to improve the effective gain. The shaping approach still works under gain saturation, showing the robustness of the method. Modeling and experiments attest that the shaping is effective even with a highly multimode fiber amplifier carrying up to 127 modes.  
      Keywords:adaptive optics;amplification;beam shaping;complex media;multimode optical fiber   
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      Published:2024-09-19
    • Benjamin P Cumming,Gerd E Schröder-Turk,Sukanta Debbarma,Min Gu
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.192
      Abstract:The smooth and tailorable spectral response of Bragg mirrors has driven their pervasive use in optical systems requiring customizable spectral control of beam propagation. However, the simple nature of Bragg mirror reflection prevents their application to the control of important polarization states such as circular polarization. While helical and gyroid-based nanostructures exhibiting circular dichroism have been developed extensively to address this limitation, they are often restricted by the spectral inconsistency of their optical response. Here we present the fabrication and characterization of quadruple-gyroid 4srs nanostructures exhibiting bio-inspired Bragg-mirror-like circular dichroism: a smooth and uniform band of circular dichroism reminiscent of the spectrum of a simple multilayer Bragg-mirror. Furthermore, we demonstrate that the circular dichroism produced by 4srs nanostructures are robust to changes in incident angle and beam collimation, providing a new platform to create and engineer circular dichroism for functional circular polarization manipulation.  
      Keywords:Bio-inspired;Bragg-mirror;Chirality;Circular dichroism;Gyroid   
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      Published:2024-09-19
    • Kai-Kai Du,Qiang Li,Yan-Biao Lyu,Ji-Chao Ding,Yue Lu,Zhi-Yuan Cheng,Min Qiu
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.194
      Abstract:Controlling the emissivity of a thermal emitter has attracted growing interest, with a view toward a new generation of thermal emission devices. To date, all demonstrations have involved using sustained external electric or thermal consumption to maintain a desired emissivity. In the present study, we demonstrated control over the emissivity of a thermal emitter consisting of a film of phase-changing material Ge2Sb2Te5 (GST) on top of a metal film. This thermal emitter achieves broad wavelength-selective spectral emissivity in the mid-infrared. The peak emissivity approaches the ideal blackbody maximum, and a maximum extinction ratio of > 10 dB is attainable by switching the GST between the crystalline and amorphous phases. By controlling the intermediate phases, the emissivity can be continuously tuned. This switchable, tunable, wavelength-selective and thermally stable thermal emitter will pave the way toward the ultimate control of thermal emissivity in the field of fundamental science as well as for energy harvesting and thermal control applications, including thermophotovoltaics, light sources, infrared imaging and radiative coolers.  
      Keywords:absorptivity;emissivity;mid-infrared;switchable;thermal emitters   
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      Published:2024-09-19
    • Murad Omar,Johannes Rebling,Kai Wicker,Tobias Schmitt-Manderbach,Mathias Schwarz,Jérôme Gateau,Hérnan López-Schier,Timo Mappes,Vasilis Ntziachristos
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.186
      Abstract:Whole-body optical imaging of post-embryonic stage model organisms is a challenging and long sought-after goal. It requires a combination of high-resolution performance and high-penetration depth. Optoacoustic (photoacoustic) mesoscopy holds great promise, as it penetrates deeper than optical and optoacoustic microscopy while providing high-spatial resolution. However, optoacoustic mesoscopic techniques only offer partial visibility of oriented structures, such as blood vessels, due to a limited angular detection aperture or the use of ultrasound frequencies that yield insufficient resolution. We introduce 360° multi orientation (multi-projection) raster scan optoacoustic mesoscopy (MORSOM) based on detecting an ultra-wide frequency bandwidth (up to 160 MHz) and weighted deconvolution to synthetically enlarge the angular aperture. We report unprecedented isotropic in-plane resolution at the 9–17 μm range and improved signal to noise ratio in phantoms and opaque 21-day-old Zebrafish. We find that MORSOM performance defines a new operational specification for optoacoustic mesoscopy of adult organisms, with possible applications in the developmental biology of adulthood and aging.  
      Keywords:deconvolution;development;mesoscopy;multiview;optoacoustics;photoacoustics   
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      Published:2024-09-19
    • Xu Chen,Clément Chardin,Kevin Makles,Charles Caër,Sheon Chua,Rémy Braive,Isabelle Robert-Philip,Tristan Briant,Pierre-François Cohadon,Antoine Heidmann,Thibaut Jacqmin,Samuel Deléglise
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.190
      Abstract:Light scattering by a two-dimensional photonic-crystal slab (PCS) can result in marked interference effects associated with Fano resonances. Such devices offer appealing alternatives to distributed Bragg reflectors and filters for various applications, such as optical wavelength and polarization filters, reflectors, semiconductor lasers, photodetectors, bio-sensors and non-linear optical components. Suspended PCS also have natural applications in the field of optomechanics, where the mechanical modes of a suspended slab interact via radiation pressure with the optical field of a high-finesse cavity. The reflectivity and transmission properties of a defect-free suspended PCS around normal incidence can be used to couple out-of-plane mechanical modes to an optical field by integrating it in a free-space cavity. Here we demonstrate the successful implementation of a PCS reflector on a high-tensile stress Si3N4 nanomembrane. We illustrate the physical process underlying the high reflectivity by measuring the photonic-crystal band diagram. Moreover, we introduce a clear theoretical description of the membrane scattering properties in the presence of optical losses. By embedding the PCS inside a high-finesse cavity, we fully characterize its optical properties. The spectrally, angular- and polarization-resolved measurements demonstrate the wide tunability of the membrane's reflectivity, from nearly 0 to 99.9470±0.0025%, and show that material absorption is not the main source of optical loss. Moreover, the cavity storage time demonstrated in this work exceeds the mechanical period of low-order mechanical drum modes. This so-called resolved-sideband condition is a prerequisite to achieve quantum control of the mechanical resonator with light.  
      Keywords:Fano resonance;high-reflectivity membrane;low-loss optical reflector;nanomembrane resonator;photonic-crystal slab;quantum optomechanics   
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      Published:2024-09-19
    • Ming Xin,Kemal Şafak,Michael Y Peng,Aram Kalaydzhyan,Wen-Ting Wang,Oliver D Mücke,Franz X Kärtner
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.187
      Abstract:Synchronous laser-microwave networks delivering attosecond timing precision are highly desirable in many advanced applications, such as geodesy, very-long-baseline interferometry, high-precision navigation and multi-telescope arrays. In particular, rapidly expanding photon-science facilities like X-ray free-electron lasers and intense laser beamlines require system-wide attosecond-level synchronization of dozens of optical and microwave signals up to kilometer distances. Once equipped with such precision, these facilities will initiate radically new science by shedding light on molecular and atomic processes happening on the attosecond timescale, such as intramolecular charge transfer, Auger processes and their impacts on X-ray imaging. Here we present for the first time a complete synchronous laser-microwave network with attosecond precision, which is achieved through new metrological devices and careful balancing of fiber nonlinearities and fundamental noise contributions. We demonstrate timing stabilization of a 4.7-km fiber network and remote optical–optical synchronization across a 3.5-km fiber link with an overall timing jitter of 580 and 680 attoseconds root-mean-square, respectively, for over 40 h. Ultimately, we realize a complete laser-microwave network with 950-attosecond timing jitter for 18 h. This work can enable next-generation attosecond photon-science facilities to revolutionize many research fields from structural biology to material science and chemistry to fundamental physics.  
      Keywords:attosecond photonics;attosecond timing metrology;hard-X-ray free-electron laser;laser-microwave network;timing distribution   
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      Published:2024-09-19
    • Giovanni Lerario,Dario Ballarini,Antonio Fieramosca,Alessandro Cannavale,Armando Genco,Federica Mangione,Salvatore Gambino,Lorenzo Dominici,Milena De Giorgi,Giuseppe Gigli,Daniele Sanvitto
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.212
      Abstract:The strong coupling of an excitonic transition with an electromagnetic mode results in composite quasi-particles called exciton polaritons, which have been shown to combine the best properties of their individual components in semiconductor microcavities. However, the physics and applications of polariton flows in organic materials and at room temperature are still unexplored because of the poor photon confinement in such structures. Here, we demonstrate that polaritons formed by the hybridization of organic excitons with a Bloch surface wave are able to propagate for hundreds of microns showing remarkable third-order nonlinear interactions upon high injection density. These findings pave the way for the study of organic nonlinear light–matter fluxes and for a technologically promising route of the realization of dissipation-less on-chip polariton devices operating at room temperature.  
      Keywords:optical nonlinearity;organic materials;polaritons;surface waves;2D optics   
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      Published:2024-09-19
    • Rajib Ahmed,Ali K Yetisen,Seok Hyun Yun,Haider Butt
      Vol. 6, Issue 1, (2017) DOI: 10.1038/lsa.2016.214
      Abstract:Corner cube retroreflectors (CCRs) have applications in sensors, image processing, free space communication and wireless networks. The ability to construct low-loss wavelength filters embedded in CCRs can enable the development of wavelength multiplexing, tunable lasers and photonic integrated circuits. Here we created an ~10-μm-thick holographic corner cube retroreflector (HCCR) array that acted as a color-selective wavelength filter and diffracted light at broad angles. Angle-resolved spectral measurements showed that the Bragg peak of the diffracted light from the HCCR array could be tuned from 460 to 545 nm by varying the incident angle. The HCCR array also exhibited a wavelength-selective tuning capability based on the rotation angle in the visible spectrum. HCCRs projected holographic images with the rotational property in the far field. The utility of the HCCR was demonstrated as optical temperature and relative humidity sensors that produced a visible colorimetric response for rapid diagnostics.  
      Keywords:Bragg gratings;corner cube retroreflectors;diffraction optics;holography;sensors   
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      Published:2024-09-19
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