Xiaohui Ling,Xinxing Zhou,Xunong Yi,Weixing Shu,Yachao Liu,Shizhen Chen,Hailu Luo,Shuangchun Wen,Dianyuan Fan
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.63
Abstract:The photonic spin Hall effect (SHE) in the reflection and refraction at an interface is very weak because of the weak spin-orbit interaction. Here, we report the observation of a giant photonic SHE in a dielectric-based metamaterial. The metamaterial is structured to create a coordinate-dependent, geometric Pancharatnam–Berry phase that results in an SHE with a spin-dependent splitting in momentum space. It is unlike the SHE that occurs in real space in the reflection and refraction at an interface, which results from the momentum-dependent gradient of the geometric Rytov–Vladimirskii–Berry phase. We theorize a unified description of the photonic SHE based on the two types of geometric phase gradient, and we experimentally measure the giant spin-dependent shift of the beam centroid produced by the metamaterial at a visible wavelength. Our results suggest that the structured metamaterial offers a potential method of manipulating spin-polarized photons and the orbital angular momentum of light and thus enables applications in spin-controlled nanophotonics.
Keywords:geometric phase;metamaterial;photonic spin Hall effect
Abstract:Although vast amounts of information are conveyed by photons in optical fibers, the majority of data processing is performed electronically, creating the infamous 'information bottleneck' and consuming energy at an increasingly unsustainable rate. The potential for photonic devices to directly manipulate light remains unfulfilled due largely to a lack of materials with strong, fast optical nonlinearities. In this paper, we show that small-signal amplifier, summator and invertor functions for optical signals may be realized using a four-port device that exploits the coherent interaction of beams on a planar plasmonic metamaterial, assuming no intrinsic nonlinearity. The redistribution of energy among ports can provide nonlinear input-output signal dependencies and may be coherently controlled at very low intensity levels, with multi-THz bandwidth and without introducing signal distortion, thereby presenting powerful opportunities for novel optical data processing architectures, complexity oracles and the locally coherent networks that are becoming part of the mainstream telecommunications agenda.
Keywords:all-optical data processing;coherent control;photonic metamaterials
SoonGweon Hong,Mi Yeon Lee,Andrew O Jackson,Luke P Lee
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.40
Abstract:The ability to capture the chemical signatures of biomolecules (i.e., electron-transfer dynamics) in living cells will provide an entirely new perspective on biology and medicine. This can be accomplished using nanoscale optical antennas that can collect, resonate and focus light from outside the cell and emit molecular spectra. Here, we describe biologically inspired nanoscale optical antennas that utilize the unique topologies of plant viruses (and thus, are called gold plant viruses) for molecular fingerprint detection. Our electromagnetic calculations for these gold viruses indicate that capsid morphologies permit high amplification of optical scattering energy compared to a smooth nanosphere. From experimental measurements of various gold viruses based on four different plant viruses, we observe highly enhanced optical cross-sections and the modulation of the resonance wavelength depending on the viral morphology. Additionally, in label-free molecular imaging, we successfully obtain higher sensitivity (by a factor of up to 106) than can be achieved using similar-sized nanospheres. By virtue of the inherent functionalities of capsids and the plasmonic characteristics of the gold layer, a gold virus-based antenna will enable cellular targeting, imaging and drug delivery.
Keywords:molecular sensor;nanophotonics;optical antenna;optical spectroscopy;plant virus;plasmonics;plasmonic resonant energy transfer (PRET);surface enhanced Raman scattering (SERS)
Abstract:High frame rate and highly sensitive imaging of refractive index changes on a surface is very promising for studying the dynamics of dissolution, mixing and biological processes without the need for labeling. Here, a highly sensitive distributed feedback (DFB) dye laser sensor for high frame rate imaging refractometry without moving parts is presented. DFB dye lasers are low-cost and highly sensitive refractive index sensors. The unique multi-wavelength DFB laser structure presented here comprises several areas with different grating periods. Imaging in two dimensions of space is enabled by analyzing laser light from all areas in parallel with an imaging spectrometer. With this multi-resonance imaging refractometry method, the spatial position in one direction is identified from the horizontal, i.e., spectral position of the multiple laser lines which is obtained from the spectrometer charged coupled device (CCD) array. The orthogonal spatial position is obtained from the vertical spatial position on the spectrometer CCD array as in established spatially resolved spectroscopy. Here, the imaging technique is demonstrated by monitoring the motion of small sucrose molecules upon dissolution of solid sucrose in water. The omission of moving parts improves the robustness of the imaging system and allows a very high frame rate of up to 12 Hz.
Keywords:distributed feedback laser;label-free imaging;laser sensor;refractive index sensor
Xinchen Li,Fengxian Xie,Shaoqing Zhang,Jianhui Hou,Wallace CH Choy
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.46
Abstract:To achieve fabrication and cost competitiveness in organic optoelectronic devices that include organic solar cells (OSCs) and organic light-emitting diodes (OLEDs), it is desirable to have one type of material that can simultaneously function as both the electron and hole transport layers (ETLs and HTLs) of the organic devices in all device architectures (i.e., normal and inverted architectures). We address this issue by proposing and demonstrating Cs-intercalated metal oxides (with various Cs mole ratios) as both the ETL and HTL of an organic optoelectronic device with normal and inverted device architectures. Our results demonstrate that the new approach works well for widely used transition metal oxides of molybdenum oxide (MoOx) and vanadium oxide (V2Ox). Moreover, the Cs-intercalated metal-oxide-based ETL and HTL can be easily formed under the conditions of a room temperature, water-free and solution-based process. These conditions favor practical applications of OSCs and OLEDs. Notably, with the analyses of the Kelvin Probe System, our approach of Cs-intercalated metal oxides with a wide mole ratio range of transition metals (Mo or V)/Cs from 1∶0 to 1∶0.75 can offer significant and continuous work function tuning as large as 1.31 eV for functioning as both an ETL and HTL. Consequently, our method of intercalated metal oxides can contribute to the emerging large-scale and low-cost organic optoelectronic devices.
Keywords:metal oxides carrier transport layers;normal and inverted device architectures;organic light-emitting diodes;organic solar cells;room-temperature solution process
Abstract:A photonic lab on a chip (PhLOC), comprising a solid-state light emitter (SSLE) aligned with a biofunctionalized optofluidic multiple internal reflection (MIR) system, is presented. The SSLE is obtained by filling a microfluidic structure with a phenyltrimethoxysilane (PhTMOS) aqueous sol solution containing a fluorophore organic dye. After curing, the resulting xerogel solid structure retains the emitting properties of the fluorophore, which is evenly distributed in the xerogel matrix. Photostability studies demonstrate that after a total dose (at λ=365 nm) greater than 24 J cm−2, the xerogel emission decay is only 4.1%. To re-direct the emitted light, the SSLE includes two sets of air mirrors that surround the xerogel. Emission mapping of the SSLE demonstrates that alignment variations of 150 µm (between the SSLE and the external pumping light source) provide fluctuations in emitted light smaller than 5%. After this verification, the SSLE is monolithically implemented with a MIR, forming the PhLOC. Its performance is assessed by measuring quinolone yellow, obtaining a limit of detection (LOD) of (0.60±0.01) µM. Finally, the MIR is selectively biofunctionalized with horseradish peroxidase (HRP) for the detection of hydrogen peroxide (H2O2) target analyte, obtaining a LOD of (0.7±0.1) µM for H2O2, confirming, for the first time, that solid-state xerogel-based emitters can be massively implemented in biofunctionalized PhLOCs.
Keywords:medical devices;photonic lab on a chip;polymer technology;solid-state light emitters;sol–gel
Alessandro Tonello,Alain Barthélémy,Katarzyna Krupa,Vincent Kermène,Agnès Desfarges-Berthelemot,Badr Mohamed Shalaby,Sonia Boscolo,Sergei K Turitsyn,Juan Diego Ania-Castañón
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.49
Abstract:We propose a new approach to the generation of an alphabet for secret key exchange relying on small variations in the cavity length of an ultralong fiber laser. This new concept is supported by experimental results showing how the radiofrequency spectrum of the laser can be exploited as a carrier to exchange information. The test bench for our proof of principle is a 50-km-long fiber laser linking two users, Alice and Bob, where each user can randomly add an extra 1-km-long segment of fiber. The choice of laser length is driven by two independent random binary values, which makes such length become itself a random variable. The security of key exchange is ensured whenever the two independent random choices lead to the same laser length and, hence, to the same free spectral range.
Keywords:fiber lasers;fiber optics communications;optical security and encryption
Abstract:The determination of optical force as a consequence of momentum transfer is inevitably subject to the use of the proper momentum density and stress tensor. It is imperative and valuable to consider the intrinsic scheme of photon momentum transfer, particularly when a particle is embedded in a complex dielectric environment. Typically, we consider a particle submerged in an inhomogeneous background composed of different dielectric materials, excluding coherent illumination or hydrodynamic effects. A ray-tracing method is adopted to capture the direct process of momentum transfer from the complex background medium, and this approach is validated using the modified Einstein–Laub method, which uses only the interior fields of the particle in the calculation. In this way, debates regarding the calculation of the force with different stress tensors using exterior fields can be avoided. Our suggested interpretation supports only the Minkowski approach for the optical momentum transfer to the embedded scatterer while rejecting Peierls's and Abraham's approaches, though the momentum of a stably moving photon in a continuous background medium should be considered to be of the Abraham type. Our interpretation also provides a novel method of realizing a tractor beam for the exertion of negative force that offers an alternative to the use of negative-index materials, optical gain, or highly non-paraxial or multiple-light interference.
Abstract:Whispering gallery mode (WGM) resonators made from dielectrics like glass or polymers have outstanding optical properties like huge cavity quality (Q) factors which can be achieved on scales compatible with on-chip integration. However, tunability of these resonances is typically difficult to achieve or not suitable for robust device applications. We report here on the fabrication of polymeric micro-goblet WGM resonators with an optically controlled and stable reversible tunability over a large spectral range. This tunability is achieved by integration of photo-responsive liquid crystalline elastomers (LCEs) into micro-goblet cavities. The optical response of the elastomer allows reshaping the goblet by employing low pump power, leading to a fully reversible tuning of the modes. The structure can be realistically implemented in on-chip devices, combining the ultra-high Q factors, typical of WGM resonators, with reliable, optical tunability. This result serves as an example of how light can control light, by invoking a physical reshaping of the structure. This way of optical tuning creates interesting possibilities for all-optical control in circuits, enabling interaction between signal and control beams and the realization of self-tuning cavities.
Dominik Floess,Jessie Y Chin,Akihito Kawatani,Daniel Dregely,Hanns-Ulrich Habermeier,Thomas Weiss,Harald Giessen
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.57
Abstract:We experimentally demonstrate an ultra-thin plasmonic optical rotator in the visible regime that induces a polarization rotation that is continuously tunable and switchable by an external magnetic field. The rotator is a magneto-plasmonic hybrid structure consisting of a magneto-optical EuSe slab and a one-dimensional plasmonic gold grating. At low temperatures, EuSe possesses a large Verdet constant and exhibits Faraday rotation, which does not saturate over a regime of several Tesla. By combining these properties with plasmonic Faraday rotation enhancement, a large tuning range of the polarization rotation of up to 8.4° for a film thickness of 220 nm is achieved. Furthermore, through experiments and simulations, we demonstrate that the unique dispersion properties of the structure enable us to tailor the wavelengths of the tunable polarization rotation to arbitrary spectral positions within the transparency window of the magneto-optical slab. The demonstrated concept might lead to important, highly integrated, non-reciprocal, photonic devices for light modulation, optical isolation, and magnetic field optical sensing. The simple fabrication of EuSe nanostructures by physical vapor deposition opens the way for many potentially interesting magneto-plasmonic systems and three-dimensional magneto-optical metamaterials.
Abstract:Data transmission rates in optical communication systems are approaching the limits of conventional multiplexing methods. Orbital angular momentum (OAM) in optical vortex beams offers a new degree of freedom and the potential to increase the capacity of free-space optical communication systems, with OAM beams acting as information carriers for OAM division multiplexing (OAM-DM). We demonstrate independent collinear OAM channel generation, transmission and simultaneous detection using Dammann optical vortex gratings (DOVGs). We achieve 80/160 Tbit s−1 capacity with uniform power distributions along all channels, with 1600 individually modulated quadrature phase-shift keying (QPSK)/16-QAM data channels multiplexed by 10 OAM states, 80 wavelengths and two polarizations. DOVG-enabled OAM multiplexing technology removes the bottleneck of massive OAM state parallel detection and offers an opportunity to raise optical communication systems capacity to Pbit s−1 level.
Kyusang Lee,Jaesang Lee,Bryan A Mazor,Stephen R Forrest
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.61
Abstract:Practical solar energy solutions must not only reduce the cost of the module, but also address the substantial balance of system costs. Here, we demonstrate a counter-intuitive approach based on gallium arsenide solar cells that can achieve extremely low-cost solar energy conversion with an estimated cost of only 3% that of conventional gallium arsenide solar cells using an accelerated, non-destructive epitaxial lift-off wafer recycling process along with a lightweight, thermoformed plastic, truncated mini-compound parabolic concentrator that avoids the need for active solar tracking. Using solar cell/concentrator assemblies whose orientations are adjusted only a few times per year, the annual energy harvesting is increased by 2.8 times compared with planar solar cells without solar tracking. These results represent a potentially drastic cost reduction in both the module and the balance of system costs compared with heavy, rigid conventional modules and trackers that are subject to wind loading damage and high installation costs.
Keywords:concentrator;cost per Watt;epitaxial lift-off;plastic substrate;thin-film GaAs solar cell
Chien-Sheng Liao,Mikhail N Slipchenko,Ping Wang,Junjie Li,Seung-Young Lee,Robert A Oglesbee,Ji-Xin Cheng
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.38
Abstract:Real-time vibrational spectroscopic imaging is desired for monitoring cellular states and cellular processes in a label-free manner. Raman spectroscopic imaging of highly dynamic systems is inhibited by relatively slow spectral acquisition on millisecond to second scale. Here, we report microsecond scale vibrational spectroscopic imaging by lock-in free parallel detection of spectrally dispersed stimulated Raman scattering signal. Using a homebuilt tuned amplifier array, our method enables Raman spectral acquisition, within the window defined by the broadband pulse, at the speed of 32 µs and with close to shot-noise limited detection sensitivity. Incorporated with multivariate curve resolution analysis, our platform allows compositional mapping of lipid droplets in single live cells, observation of intracellular retinoid metabolism, discrimination of fat droplets from protein-rich organelles in Caenorhabditis elegans, spectral detection of fast flowing tumor cells and monitoring drug diffusion through skin tissue in vivo. The reported technique opens new opportunities for compositional analysis of cellular compartment in a microscope setting and high-throughput spectral profiling of single cells in a flow cytometer setting.
Abstract:Wide field-of-view (FOV) and high-resolution imaging requires microscopy modalities to have large space-bandwidth products. Lensfree on-chip microscopy decouples resolution from FOV and can achieve a space-bandwidth product greater than one billion under unit magnification using state-of-the-art opto-electronic sensor chips and pixel super-resolution techniques. However, using vertical illumination, the effective numerical aperture (NA) that can be achieved with an on-chip microscope is limited by a poor signal-to-noise ratio (SNR) at high spatial frequencies and imaging artifacts that arise as a result of the relatively narrow acceptance angles of the sensor's pixels. Here, we report, for the first time, a synthetic aperture-based on-chip microscope in which the illumination angle is scanned across the surface of a dome to increase the effective NA of the reconstructed lensfree image to 1.4, achieving e.g., ~250-nm resolution at 700-nm wavelength under unit magnification. This synthetic aperture approach not only represents the largest NA achieved to date using an on-chip microscope but also enables color imaging of connected tissue samples, such as pathology slides, by achieving robust phase recovery without the need for multi-height scanning or any prior information about the sample. To validate the effectiveness of this synthetic aperture-based, partially coherent, holographic on-chip microscope, we have successfully imaged color-stained cancer tissue slides as well as unstained Papanicolaou smears across a very large FOV of 20.5 mm2. This compact on-chip microscope based on a synthetic aperture approach could be useful for various applications in medicine, physical sciences and engineering that demand high-resolution wide-field imaging.
Abstract:An optically addressed spatial light modulator (OASLM) can modulate the wavefront of a read light by displaying a phase pattern or a hologram configured by the intensity distribution of a write light. Using ZnO nanoparticles (NPs) as a novel photoconductor, a high-resolution OASLM was fabricated. A ZnO NP suspension was spin-coated on an indium tin oxide (ITO)-coated glass substrate and annealed to form a photosensitive layer. The device was characterized electrically and optically. The device was operated at low driving voltages in the transmission mode. Updatable recording of a diffraction grating up to 825 lp mm−1 with a diffraction efficiency (DE) of 0.05% and binary holograms with pixel sizes from 2 µm down to 0.72 µm were demonstrated using a 405 nm wavelength write laser and a 635 nm wavelength read laser.
Dong Yeong Kim,Jun Hyuk Park,Jong Won Lee,Sunyong Hwang,Seung Jae Oh,Jungsub Kim,Cheolsoo Sone,E. Fred Schubert,Jong Kyu Kim
Vol. 4, Issue 2, (2015) DOI: 10.1038/lsa.2015.36
Abstract:While the demand for deep ultraviolet (DUV) light sources is rapidly growing, the efficiency of current AlGaN-based DUV light-emitting diodes (LEDs) remains very low due to their fundamentally limited light-extraction efficiency (LEE), calling for a novel LEE-enhancing approach to deliver a real breakthrough. Here, we propose sidewall emission-enhanced (SEE) DUV LEDs having multiple light-emitting mesa stripes to utilize inherently strong transverse-magnetic polarized light from the AlGaN active region and three-dimensional reflectors between the stripes. The SEE DUV LEDs show much enhanced light output power with a strongly upward-directed emission due to the exposed sidewall of the active region and Al-coated selective-area-grown n-type GaN micro-reflectors. The devices also show reduced operating voltage due to better n-type ohmic contact formed on the regrown n-GaN stripes when compared with conventional LEDs. Accordingly, the proposed approach simultaneously improves optical and electrical properties. In addition, strategies to further enhance the LEE up to the theoretical optimum value and control emission directionality are discussed.
Abstract:Single-photon detectors (SPDs) are the most sensitive instruments for light detection. In the near-infrared range, SPDs based on Ⅲ–Ⅴ compound semiconductor avalanche photodiodes have been extensively used during the past two decades for diverse applications due to their advantages in practicality including small size, low cost and easy operation. In the past decade, the rapid developments and increasing demands in quantum information science have served as key drivers to improve the device performance of single-photon avalanche diodes and to invent new avalanche quenching techniques. This Review aims to introduce the technology advances of InGaAs/InP single-photon detector systems in the telecom wavelengths and the relevant quantum communication applications, and particularly to highlight recent emerging techniques such as high-frequency gating at GHz rates and free-running operation using negative-feedback avalanche diodes. Future perspectives of both the devices and quenching techniques are summarized.