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Vol. 11 ， Issue 10 ， 2022
Editorial
- Abstract：Hollow upconversion nanoparticles with tunable central cavity size can be used as self-referenced luminescent thermometers over a wide temperature range.
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Published：2022-11-01 - Abstract：Existing single-cell adhesion kinetics methods are performed under conditions highly unlike the physiological cell adhesion conditions. Now, researchers have developed a new optical technique for high-precision measurement of cell lateral adhesion kinetics in complex clinical samples.
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Published：2022-11-01 - Abstract：An advanced method for hyperspectral imaging was combined with phase retrieval and standard pulse characterization techniques to characterize ultrashort laser pulses and ultrashort processes to a new level of precision in a single shot.
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Published：2022-11-01 - Abstract：Exploiting Fourier-domain optical coherence tomography, a high-speed and real-time inspection of multi-photon 3D laser printing has been reported. We expect that this technique can be further extended to single shot compressive 3D imaging for studying the ultrafast dynamics of laser-matter interaction.
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Published：2022-11-01 - Abstract：Recently, a new diffractive camera design based on transmissive surfaces structured using deep learning is proposed. It performs class-specific imaging of target objects and all-optical deletion of other classes of objects, which will promote the development of privacy-preserving digital cameras and mission-specific data.
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Published：2022-11-01 - Abstract：Lanthanide-doped nanoscintillators are taking the lead in several important fields including radiation detection, biomedicine, both at the level of diagnosis and therapy, and information encoding.
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Published：2022-11-01 - Abstract：High spatial resolution imaging of the mouse brain through the intact skull is challenging because of the skull-induced aberration and scattering. The research group of Dan Zhu from Huazhong University of Science and Technology has developed a skull-clearing technique that provides a long-term (~ weeks), stable, transparent window for high resolution optical imaging over a large field of view.
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Published：2022-11-01 - Abstract：The continuous supersymmetry transformation is applied to the silicon waveguides, and the guidance and conversion of any mode in a wide spectral range are successfully realized in experiments. This proves its great potential in optical spatial mode modulation and space division multiplexing in optical communication.
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Published：2022-11-01 - Abstract：A donut excitation moves around a single molecule with a zigzag configuration lattice by lattice. Such a method implemented in scanning fluorescence microscopy simplifies the conventional MINFLUX process. Consisting of hollow zero-intensity excitation, single-pixel detection, time-correlated single photon counting, and drift stabilization, the system achieves localization precision and resolution very close to conventional MINFLUX theoretically and experimentally. An averaged high-SNR reference, and pixel-registered intensity from a single molecule is essential to reconstruct localization in maximum likelihood estimation. With performance reaching nearly conventional MINFLUX's, the proposed raster-scanning MINFLUX can inspire researchers expertized in STED or confocal setup to quickly transform to MINFLUX and develop for further exploring on bio-specimens or optical applications.
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Published：2022-11-01
News & Views
Research Highlight
- Abstract：Integrated photonics means integrating multiple photonic functions on a single Photonic Integrated Chip (PIC). Empowered by various nanofabrication techniques on diverse innovative material platforms, remarkable advances have been made in integrated photonics in the last decade. Light: Advanced Manufacturing (LAM) is a new, highly selective, open-access, and free of charge international sister journal of the Nature Journal Light: Science & Applications (Light). LAM aims to publish original innovative research papers and timely, state-of-the-art reviews in all modern areas of preferred light-based manufacturing, including fundamental and applied research as well as industrial innovations. LAM is organizing a special issue on integrated photonics, in order to capture the most exciting cutting edge advances in integrated photonics, including new material platforms, new fabrication and characterization technologies, new device architectures, new design principle of miniaturized components, nanophotonic devices, and their potential applications. We are very honored to feature Prof. Baohua Jia, the lead guest editor of this special issue, as this issue's Light People. She is the Director of Center for Atomaterial Sciences and Technologies at Royal Melbourne Institute of Technology (RMIT) University and a top-level Future Fellow funded by the Australian Research Council. Her research focuses on fundamental light and nanomaterial interaction. In particular, her work on laser manipulation of two-dimensional materials has led to the design and fabrication of functional nanostructures and nanomaterials for effective harnessing and storage of clean energy from sunlight, purifying water and air for clean environment and imaging and spectroscopy and nanofabrication using ultrafast laser towards fast-speed all-optical communications and intelligent manufacturing. She is an elected Fellow of Optica (formally known as OSA) and an elected Fellow of the Institute of Materials, Minerals, and Mining. She serves on the College of Expert for the Australian Research Council since 2019. Now please follow Light scientific editor to enter Prof. Jia's academic world.
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Published：2022-11-01 - Abstract：As 5 G ever becomes a part of everyday life and 6 G is also on the agenda, terahertz technology has gradually become known by the public, and is referred to as the "third eye" for human beings to understand the world. Terahertz is considered one of the top ten technologies that will change the world due to its unique properties. In 2019, astronomers were able to observe a black hole for the first time, using a terahertz astronomical telescope. Terahertz is no longer far away from our lives, whether it is information, medicine, or food safety and other fields. It is everywhere, triggering major changes in people's work and lifestyle. Today's guest of Light People is an internationally renowned scholar who has been engaged in terahertz research for many years, Professor Xi-Cheng Zhang works at the University of Rochester, one of the three major optics educational centers in the United States. As a pioneer in the field of terahertz technology, after years of practice, he has successfully generated terahertz waves using water, changing how we see water with THz wave forever. Next, please follow the Light Science Editor into the terahertz world to learn about the latest and most cutting-edge science and technology and the "story" behind it.
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Published：2022-11-01 - Abstract：Mendeleev said: "Science begins where one begins to measure, " and "exact science is unthinkable without measure." During his more than 4-decades-long career, Prof. Wolfgang Osten has been devoted to optical metrology and inspection technologies. Osten and his research team developed the first automated system for the quantitative and qualitative evaluation of interferograms in the '80s, as well as the principle of tilted-wave interferometry for high-precision aspherical and free-form surface measurement. Both techniques have since been commercialized. His achievements have "lit the way" for research in optical metrology. The bond between Osten and Light Publishing Group can be traced back to 2012, when he first submitted a paper to Light: Science & Applications (LSA) as an author and published a paper
1 . Right after that, he was invited to join the Editorial Board for his enthusiasm. In 2019, he started the challenge of founding the new journal Light: Advanced Manufacturing (LAM) as the co-Editor-in-Chief. In this interview, Osten shared his insights on Optical Metrology, Holography, and the Founding of LAM with us. Follow the Q & As below and let us get closer to the "Holoknight".- 11
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Published：2022-11-01
Light People
- Abstract：We present a new label-free three-dimensional (3D) microscopy technique, termed transport of intensity diffraction tomography with non-interferometric synthetic aperture (TIDT-NSA). Without resorting to interferometric detection, TIDT-NSA retrieves the 3D refractive index (RI) distribution of biological specimens from 3D intensity-only measurements at various illumination angles, allowing incoherent-diffraction-limited quantitative 3D phase-contrast imaging. The unique combination of z-scanning the sample with illumination angle diversity in TIDT-NSA provides strong defocus phase contrast and better optical sectioning capabilities suitable for high-resolution tomography of thick biological samples. Based on an off-the-shelf bright-field microscope with a programmable light-emitting-diode (LED) illumination source, TIDT-NSA achieves an imaging resolution of 206 nm laterally and 520 nm axially with a high-NA oil immersion objective. We validate the 3D RI tomographic imaging performance on various unlabeled fixed and live samples, including human breast cancer cell lines MCF-7, human hepatocyte carcinoma cell lines HepG2, mouse macrophage cell lines RAW 264.7, Caenorhabditis elegans (C. elegans), and live Henrietta Lacks (HeLa) cells. These results establish TIDT-NSA as a new non-interferometric approach to optical diffraction tomography and 3D label-free microscopy, permitting quantitative characterization of cell morphology and time-dependent subcellular changes for widespread biological and medical applications.
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Published：2022-11-01 - Abstract：Human activity monitoring is an exciting research area to assist independent living among disabled and elderly population. Various techniques have been proposed to recognise human activities, such as exploiting sensors, cameras, wearables, and contactless microwave sensing. Among these, the microwave sensing has recently gained significant attention due to its merit to solve the privacy concerns of cameras and discomfort caused by wearables. However, the existing microwave sensing techniques have a basic disadvantage of requiring controlled and ideal settings for high-accuracy activity detections, which restricts its wide adoptions in non-line-of-sight (Non-LOS) environments. Here, we propose a concept of intelligent wireless walls (IWW) to ensure high-precision activity monitoring in complex environments wherein the conventional microwave sensing is invalid. The IWW is composed of a reconfigurable intelligent surface (RIS) that can perform beam steering and beamforming, and machine learning algorithms that can automatically detect the human activities with high accuracy. Two complex environments are considered: one is a corridor junction scenario with transmitter and receiver in separate corridor sections and the other is a multi-floor scenario wherein the transmitter and receiver are placed on two different floors of a building. In each of the aforementioned environments, three distinct body movements are considered namely, sitting, standing, and walking. Two subjects, one male and one female perform these activities in both environments. It is demonstrated that IWW provide a maximum detection gain of 28% in multi-floor scenario and 25% in corridor junction scenario as compared to traditional microwave sensing without RIS.
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Published：2022-11-01 - Abstract：Lanthanide-doped colloidal nanoparticles capable of photon upconversion (UC) offer long luminescence lifetimes, narrowband absorption and emission spectra, and efficient anti-Stokes emission. These features are highly advantageous for Förster Resonance Energy Transfer (FRET) based detection. Upconverting nanoparticles (UCNPs) as donors may solve the existing problems of molecular FRET systems, such as photobleaching and limitations in quantitative analysis, but these new labels also bring new challenges. Here we have studied the impact of the core-shell compositional architecture of upconverting nanoparticle donors and the mode of photoexcitation on the performance of UC-FRET from UCNPs to Rose Bengal (RB) molecular acceptor. We have quantitatively compared luminescence rise and decay kinetics of Er3+ emission using core-only NaYF4: 20% Yb, 2% Er and core-shell NaYF4: 20% Yb @ NaYF4: 20% Yb, 5% Er donor UCNPs under three photoexcitation schemes: (1) direct short-pulse photoexcitation of Er3+ at 520 nm; indirect photoexcitation of Er3+ through Yb3+ sensitizer with (2) 980 nm short (5–7 ns) or (3) 980 nm long (4 ms) laser pulses. The donor luminescence kinetics and steady-state emission spectra differed between the UCNP architectures and excitation schemes. Aiming for highly sensitive kinetic upconversion FRET-based biomolecular assays, the experimental results underline the complexity of the excitation and energy-migration mechanisms affecting the Er3+ donor responses and suggest ways to optimize the photoexcitation scheme and the architecture of the UCNPs used as luminescent donors.
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Published：2022-11-01 - Abstract：Cold spots are sub-wavelength regions which might emerge near a nanoantenna, should one or more components of some far-field illumination cancel out with scattered light. We show that by changing only the polarisation, amplitude, and phase of two plane waves, a unique, zero-magnitude and highly sub-wavelength cold spot can be created and moved anywhere in the space around a nanoantenna of any arbitrary shape. This can be achieved using ultra-fast modulated pulses, or a time-harmonic approximation. Easily disturbed by a change in the nanoantenna's material or position, a manufactured cold spot is fragile and could be used in nanoscale sensing. Our technique exploits the linearity of Maxwell's equations and could be adapted to manipulate any phenomena governed by the linear wave equation, including acoustic scattering. This is a means for potentially ultra-fast sub-wavelength electric field manipulation.
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Published：2022-11-01 - Abstract：Lidar techniques present a distinctive ability to resolve vertical structure of optical properties within the upper water column at both day- and night-time. However, accuracy challenges remain for existing lidar instruments due to the ill-posed nature of elastic backscatter lidar retrievals and multiple scattering. Here we demonstrate the high performance of, to the best of our knowledge, the first shipborne oceanic high-spectral-resolution lidar (HSRL) and illustrate a multiple scattering correction algorithm to rigorously address the above challenges in estimating the depth-resolved diffuse attenuation coefficient Kd and the particulate backscattering coefficient bbp at 532 nm. HSRL data were collected during day- and night-time within the coastal areas of East China Sea and South China Sea, which are connected by the Taiwan Strait. Results include vertical profiles from open ocean waters to moderate turbid waters and first lidar continuous observation of diel vertical distribution of thin layers at a fixed station. The root-mean-square relative differences between the HSRL and coincident in situ measurements are 5.6% and 9.1% for Kd and bbp, respectively, corresponding to an improvement of 2.7–13.5 and 4.9–44.1 times, respectively, with respect to elastic backscatter lidar methods. Shipborne oceanic HSRLs with high performance are expected to be of paramount importance for the construction of 3D map of ocean ecosystem.
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Published：2022-11-01 - Abstract：Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed, high spectral resolution, and broad optical bandwidth needed to accurately study complex, transient events in chemistry, combustion, and microscopy. However, such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here, we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 µm. This frequency comb is based on a commercially available 1.56 µm mode-locked laser, robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in χ(2) nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration, this source will simultaneously enable measurements with μs time resolution, 1 GHz (0.03 cm−1) spectral point spacing and a full bandwidth of > 5 THz (> 166 cm−1) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.
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Published：2022-11-01 - Abstract：Performing analog computations with metastructures is an emerging wave-based paradigm for solving mathematical problems. For such devices, one major challenge is their reconfigurability, especially without the need for a priori mathematical computations or computationally-intensive optimization. Their equation-solving capabilities are applied only to matrices with special spectral (eigenvalue) distribution. Here we report the theory and design of wave-based metastructures using tunable elements capable of solving integral/differential equations in a fully-reconfigurable fashion. We consider two architectures: the Miller architecture, which requires the singular-value decomposition, and an alternative intuitive direct-complex-matrix (DCM) architecture introduced here, which does not require a priori mathematical decomposition. As examples, we demonstrate, using system-level simulation tools, the solutions of integral and differential equations. We then expand the matrix inverting capabilities of both architectures toward evaluating the generalized Moore–Penrose matrix inversion. Therefore, we provide evidence that metadevices can implement generalized matrix inversions and act as the basis for the gradient descent method for solutions to a wide variety of problems. Finally, a general upper bound of the solution convergence time reveals the rich potential that such metadevices can offer for stationary iterative schemes.
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Published：2022-11-01 - Abstract：Most whole slide imaging (WSI) systems today rely on the "stop-and-stare" approach, where, at each field of view, the scanning stage is brought to a complete stop before the camera snaps a picture. This procedure ensures that each image is free of motion blur, which comes at the expense of long acquisition times. In order to speed up the acquisition process, especially for large scanning areas, such as pathology slides, we developed an acquisition method in which the data is acquired continuously while the stage is moving at high speeds. Using generative adversarial networks (GANs), we demonstrate this ultra-fast imaging approach, referred to as GANscan, which restores sharp images from motion blurred videos. GANscan allows us to complete image acquisitions at 30x the throughput of stop-and-stare systems. This method is implemented on a Zeiss Axio Observer Z1 microscope, requires no specialized hardware, and accomplishes successful reconstructions at stage speeds of up to 5000 μm/s. We validate the proposed method by imaging H & E stained tissue sections. Our method not only retrieves crisp images from fast, continuous scans, but also adjusts for defocusing that occurs during scanning within +/− 5 μm. Using a consumer GPU, the inference runs at < 20 ms/ image.
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Published：2022-11-01 - Abstract：Contrary to the common belief that the light-induced halide ion segregation in a mixed halide alloy occurs within the illuminated area, we find that the Br ions released by light are expelled from the illuminated area, which generates a macro/mesoscopic size anion ring surrounding the illuminated area, exhibiting a photoluminescence ring. This intriguing phenomenon can be explained as resulting from two counter-balancing effects: the outward diffusion of the light-induced free Br ions and the Coulombic force between the anion deficit and surplus region. Right after removing the illumination, the macro/mesoscopic scale ion displacement results in a built-in voltage of about 0.4 V between the ring and the center. Then, the displaced anions return to the illuminated area, and the restoring force leads to a damped ultra-low-frequency oscillatory ion motion, with a period of about 20–30 h and lasting over 100 h. This finding may be the first observation of an ionic plasma oscillation in solids. Our understanding and controlling the "ion segregation" demonstrate that it is possible to turn this commonly viewed "adverse phenomenon" into novel electronic applications, such as ionic patterning, self-destructive memory, and energy storage.
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Published：2022-11-01 - Abstract：Secure information retrieval is an essential task in today's highly digitised society. In some applications, it may be necessary that user query's privacy and database content's security are enforced. For these settings, symmetric private information retrieval (SPIR) could be employed, but its implementation is known to be demanding, requiring a private key-exchange network as the base layer. Here, we report for the first time a realisation of provably-secure SPIR supported by a quantum-secure key-exchange network. The SPIR scheme looks at biometric security, offering secure retrieval of 582-byte fingerprint files from a database with 800 entries. Our experimental results clearly demonstrate the feasibility of SPIR with quantum secure communications, thereby opening up new possibilities in secure distributed data storage and cloud computing over the future Quantum Internet.
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Published：2022-11-01 - Abstract：Full pump depletion corresponds to the upper limit of the generated signal photons relative to the pump pulse; this allows the highest peak power to be produced in a unit area of ultraintense laser amplifiers. In practical systems based on optical parametric chirped-pulse amplification, however, the typical pump depletion is only ~35%. Here, we report quasi-parametric chirped-pulse amplification (QPCPA) with a specially designed 8-cm-thick Sm: YCOB crystal that highly dissipates the idler and hence improves pump depletion. We demonstrate 56% QPCPA energy efficiency for an 810-nm signal converted from a 532-nm pump, or equivalently 85% pump depletion. As another advantage, such a record high depletion greatly suppresses the parametric superfluorescence noise in QPCPA to only ~1.5 × 10−6 relative to the amplified signal energy. These results pave the way to beyond the ten-petawatt peak power of the currently most intense lasers.
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Published：2022-11-01 - Abstract：Quantum entanglement has emerged as a great resource for spectroscopy and its importance in two-photon spectrum and microscopy has been demonstrated. Current studies focus on the two-photon absorption, whereas the Raman spectroscopy with quantum entanglement still remains elusive, with outstanding issues of temporal and spectral resolutions. Here we study the new capabilities provided by entangled photons in coherent Raman spectroscopy. An ultrafast frequency-resolved Raman spectroscopy with entangled photons is developed for condensed-phase molecules, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal shows the capability of both temporal and spectral resolutions not accessible by either classical pulses or the fields without entanglement. We develop a microscopic theory for this Raman spectroscopy, revealing the electronic coherence dynamics even at timescale of 50fs. This suggests new paradigms of optical signals and spectroscopy, with potential to push detection below standard quantum limit.
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Published：2022-11-01 - Abstract：The rapid development of space-time-coding metasurfaces (STCMs) offers a new avenue to manipulate spatial electromagnetic beams, waveforms, and frequency spectra simultaneously with high efficiency. To date, most studies are primarily focused on harmonic generations and independent controls of finite-order harmonics and their spatial waves, but the manipulations of continuously temporal waveforms that include much rich frequency spectral components are still limited in both theory and experiment based on STCM. Here, we propose a theoretical framework and method to generate frequency-modulated continuous waves (FMCWs) and control their spatial propagation behaviors simultaneously via a novel STCM with nonlinearly periodic phases. Since the carrier frequency of FMCW changes with time rapidly, we can produce customized time-varying reflection phases at will by the required FMCW under the illumination of a monochromatic wave. More importantly, the propagation directions of the time-varying beams can be controlled by encoding the metasurface with different initial phase gradients. A programmable STCM prototype with a full-phase range is designed and fabricated to realize reprogrammable FMCW functions, and experimental results show good agreement with the theoretical analyses.
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Published：2022-11-01 - Abstract：Colloidal quantum dots (QDs) are excellent optical gain materials that combine high material gain, a strong absorption of pump light, stability under strong light exposure and a suitability for solution-based processing. The integration of QDs in laser cavities that fully exploit the potential of these emerging optical materials remains, however, a challenge. In this work, we report on a vertical cavity surface emitting laser, which consists of a thin film of QDs embedded between two layers of polymerized chiral liquid crystal. Forward directed, circularly polarized defect mode lasing under nanosecond-pulsed excitation is demonstrated within the photonic band gap of the chiral liquid crystal. Stable and long-term narrow-linewidth lasing of an exfoliated free-standing, flexible film under water is obtained at room temperature. Moreover, we show that the lasing wavelength of this flexible cavity shifts under influence of pressure, strain or temperature. As such, the combination of solution processable and stable inorganic QDs with high chiral liquid crystal reflectivity and effective polymer encapsulation leads to a flexible device with long operational lifetime, that can be immersed in different protic solvents to act as a sensor.
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Published：2022-11-01 - Abstract：Negative refraction, an unnatural optical phenomenon in which the incident and the refracted waves reside on the same side of the surface normal, has been demonstrated with the invention of negative index media based on artificially engineered photonic structures called metamaterials. It has received wide attention due to its potential applications in imaging, nonlinear optics, and electromagnetic cloaking. However, it is highly challenging to realize negative refraction operating at all angles and with the perfect transmission. In this work, leveraging the recent development in topological photonics, we propose to realize reflectionless negative refraction for all incident angles with a topological metamaterial. The proposed metamaterial possesses two Weyl points of opposite topological charges. By interfacing the metamaterial with a perfect electric conductor (PEC) or a perfect magnetic conductor (PMC), the Fermi arc connecting the two Weyl points can take the form of a half-circle possessing a positive or a negative refractive index. Importantly, due to the topological protection, there is no reflection at the interface between the PEC and PMC covered areas, leading to the observation of all-angle negative refraction without reflection at the boundary. Our work provides a new platform for manipulating the propagation of surface waves, which may find applications in the construction of integrated photonic devices.
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Published：2022-11-01 - Abstract：Nonlinear autocorrelation was one of the earliest and simplest tools for obtaining partial temporal information about an ultrashort optical pulse by gating it with itself. However, since the spectral phase is lost in a conventional autocorrelation measurement, it is insufficient for a full characterization of an ultrafast electric field, requiring additional spectral information for phase retrieval. Here, we show that introducing an intensity asymmetry into a conventional nonlinear interferometric autocorrelation preserves some spectral phase information within the autocorrelation signal, which enables the full reconstruction of the original electric field, including the direction of time, using only a spectrally integrating detector. We call this technique Phase-Enabled Nonlinear Gating with Unbalanced Intensity (PENGUIN). It can be applied to almost any existing nonlinear interferometric autocorrelator, making it capable of complete optical field characterization and thus providing an inexpensive and less complex alternative to methods relying on spectral measurements, such as frequency-resolved optical gating (FROG) or spectral phase interferometry for direct electric-field reconstruction (SPIDER). More importantly, PENGUIN allows the precise characterization of ultrafast fields in non-radiative (e.g., plasmonic) nonlinear optical interactions where spectral information is inaccessible. We demonstrate this novel technique through simulations and experimentally by measuring the electric field of ~6-fs laser pulses from a Ti: sapphire oscillator. The results are validated by comparison with the well-established FROG method.
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Published：2022-11-01 - Abstract：The near-infrared luminescence of Ca6Ba(PO4)4O: Mn5+ is demonstrated and explained. When excited into the broad and strong absorption band that spans the 500–1000 nm spectral range, this phosphor provides an ultranarrow (FWHM = 5 nm) emission centered at 1140 nm that originates from a spin-forbidden 1E → 3A2 transition with a 37.5% internal quantum efficiency and an excited-state lifetime of about 350 μs. We derived the crystal field and Racah parameters and calculated the appropriate Tanabe–Sugano diagram for this phosphor. We found that 1E emission quenches due to the thermally-assisted cross-over with the 3T2 state and that the relatively high Debye temperature of 783 K of Ca6Ba(PO4)4O facilitates efficient emission. Since Ca6Ba(PO4)4O also provides efficient yellow emission of the Eu2+ dopant, we calculated and explained its electronic band structure, the partial and total density of states, effective Mulliken charges of all ions, elastic constants, Debye temperature, and vibrational spectra. Finally, we demonstrated the application of phosphor in a luminescence intensity ratio thermometry and obtained a relative sensitivity of 1.92%K−1 and a temperature resolution of 0.2 K in the range of physiological temperatures.
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Published：2022-11-01 - Abstract：Nanomaterials capable of confining light are desirable for enhancing spectroscopies such as Raman scattering, infrared absorption, and nonlinear optical processes. Plasmonic superlattices have shown the ability to host collective resonances in the mid-infrared, but require stringent fabrication processes to create well-ordered structures. Here, we demonstrate how short-range-ordered Au nanoparticle multilayers on a mirror, self-assembled by a sub-nm molecular spacer, support collective plasmon-polariton resonances in the visible and infrared, continuously tunable beyond 11 µm by simply varying the nanoparticle size and number of layers. The resulting molecule-plasmon system approaches vibrational strong coupling, and displays giant Fano dip strengths, SEIRA enhancement factors ~ 106, light-matter coupling strengths g ~ 100 cm−1, Purcell factors ~ 106, and mode volume compression factors ~ 108. The collective plasmon-polariton mode is highly robust to nanoparticle vacancy disorder and is sustained by the consistent gap size defined by the molecular spacer. Structural disorder efficiently couples light into the gaps between the multilayers and mirror, enabling Raman and infrared sensing of sub-picolitre sample volumes.
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Published：2022-11-01 - Abstract：The rapid development of high-QM macroscopic mechanical resonators has enabled great advances in optomechanics. Further improvements could allow for quantum-limited or quantum-enhanced applications at ambient temperature. Some of the remaining challenges include the integration of high-QM structures on a chip, while simultaneously achieving large coupling strengths through an optical read-out. Here, we present a versatile fabrication method, which allows us to build fully integrated optomechanical structures. We place a photonic crystal cavity directly above a mechanical resonator with high-QM fundamental out-of-plane mode, separated by a small gap. The highly confined optical field has a large overlap with the mechanical mode, enabling strong optomechanical interaction strengths. Furthermore, we implement a novel photonic crystal design, which allows for a very large cavity photon number, a highly important feature for optomechanical experiments and sensor applications. Our versatile approach is not limited to our particular design but allows for integrating an out-of-plane optical read-out into almost any device layout. Additionally, it can be scaled to large arrays and paves the way to realizing quantum experiments and applications with mechanical resonators based on high-QM out-of-plane modes alike.
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Published：2022-11-01 - Abstract：Currently, artificial enzymes-based photodynamic therapy (PDT) is attractive due to its efficient capacity to change the immunosuppressive tumor microenvironment (TME). It is of great significance to study the therapeutic mechanism of novel artificial enzymes in TME through a monitoring strategy and improve the therapeutic effect. In this study, Au@carbon dots (Au@CDs) nanohybrids with a core-shell structure are synthesized, which not only exhibit tunable enzyme-mimicking activity under near-infrared (NIR) light, but also excellent surface-enhanced Raman scattering (SERS) properties. Therefore, Au@CDs show a good capability for monitoring NIR-photoinduced peroxidase-like catalytic processes via a SERS strategy in tumor. Moreover, the Au@CDs deplete glutathione with the cascade catalyzed reactions, thus elevating intratumor oxidative stress amplifying the reactive oxygen species damage based on the NIR-photoinduced enhanced peroxidase and glutathione oxidase-like activities, showing excellent and fast PDT therapeutic effect promoted by photothermal property in 3 min, finally leading to apoptosis in cancer cells. Through SERS monitoring, it is further found that after removing the NIR light source for 33 min, the reactive oxygen species (ROS) activity of the TME is counteracted and eliminated due to the presence of glutathione. This work presents a guidance to rationally design of artificial enzyme for ROS-involved therapeutic strategies and a new spectroscopic tool to evaluate the tumor catalytic therapy.
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Published：2022-11-01 - Abstract：Topological spin structures of light, including the Skyrmion, Meron, and bi-Meron, are intriguing optical phenomena that arise from spin–orbit coupling. They have promising potential applications in nano-metrology, data storage, super-resolved imaging and chiral detection. Aside from the electric part of optical spin, of equal importance is the magnetic part, particularly the H-type electromagnetic modes for which the spin topological properties of the field are dominated by the magnetic field. However, their observation and measurement remains absent and faces difficult challenges. Here, we design a unique type of anapole probe to measure specifically the photonic spin structures dominated by magnetic fields. The probe is composed of an Ag-core and Si-shell nanosphere, which manifests as a pure magnetic dipole with no electric response. The effectiveness of the method was validated by characterizing the magnetic field distributions of various focused vector beams. It was subsequently employed to measure the magnetic topological spin structures, including individual Skyrmions and Meron/Skyrmion lattices for the first time. The proposed method may be a powerful tool to characterize the magnetic properties of optical spin and valuable in advancing spin photonics.
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Published：2022-11-01 - Abstract：Photonic neural network has been sought as an alternative solution to surpass the efficiency and speed bottlenecks of electronic neural network. Despite that the integrated Mach–Zehnder Interferometer (MZI) mesh can perform vector-matrix multiplication in photonic neural network, a programmable in-situ nonlinear activation function has not been proposed to date, suppressing further advancement of photonic neural network. Here, we demonstrate an efficient in-situ nonlinear accelerator comprising a unique solution-processed two-dimensional (2D) MoS2 Opto-Resistive RAM Switch (ORS), which exhibits tunable nonlinear resistance switching that allow us to introduce nonlinearity to the photonic neuron which overcomes the linear voltage-power relationship of typical photonic components. Our reconfigurable scheme enables implementation of a wide variety of nonlinear responses. Furthermore, we confirm its feasibility and capability for MNIST handwritten digit recognition, achieving a high accuracy of 91.6%. Our accelerator constitutes a major step towards the realization of in-situ photonic neural network and pave the way for the integration of photonic integrated circuits (PIC).
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Published：2022-11-01 - Abstract：The moiré superlattice of misaligned atomic bilayers paves the way for designing a new class of materials with wide tunability. In this work, we propose a photonic analog of the moiré superlattice based on dielectric resonator quasi-atoms. In sharp contrast to van der Waals materials with weak interlayer coupling, we realize the strong coupling regime in a moiré superlattice, characterized by cascades of robust flat bands at large twist-angles. Surprisingly, we find that these flat bands are characterized by a non-trivial band topology, the origin of which is the moiré pattern of the resonator arrangement. The physical manifestation of the flat band topology is a robust one-dimensional conducting channel on edge, protected by the reflection symmetry of the moiré superlattice. By explicitly breaking the underlying reflection symmetry on the boundary terminations, we show that the first-order topological edge modes naturally deform into higher-order topological corner modes. Our work pioneers the physics of topological phases in the designable platform of photonic moiré superlattices beyond the weakly coupled regime.
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Published：2022-11-01 - Abstract：Cold atoms provide a flexible platform for synthesizing and characterizing topological matter, where geometric phases play a central role. However, cold atoms are intrinsically prone to thermal noise, which can overwhelm the topological response and hamper promised applications. On the other hand, geometric phases also determine the energy spectra of particles subjected to a static force, based on the polarization relation between Wannier-Stark ladders and geometric Zak phases. By exploiting this relation, we develop a method to extract geometric phases from energy spectra of room-temperature superradiance lattices, which are momentum-space lattices of timed Dicke states. In such momentum-space lattices the thermal motion of atoms, instead of being a source of noise, provides effective forces which lead to spectroscopic signatures of the Zak phases. We measure Zak phases directly from the anti-crossings between Wannier-Stark ladders in the Doppler-broadened absorption spectra of superradiance lattices. Our approach paves the way of measuring topological invariants and developing their applications in room-temperature atoms.
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Published：2022-11-01 - Abstract：Micro or submicron scale light-emitting diodes (µLEDs) have been extensively studied recently as the next-generation display technology. It is desired that µLEDs exhibit high stability and efficiency, submicron pixel size, and potential monolithic integration with Si-based complementary metal-oxide-semiconductor (CMOS) electronics. Achieving such µLEDs, however, has remained a daunting challenge. The polar nature of Ⅲ-nitrides causes severe wavelength/color instability with varying carrier concentrations in the active region. The etching-induced surface damages and poor material quality of high indium composition InGaN quantum wells (QWs) severely deteriorate the performance of µLEDs, particularly those emitting in the green/red wavelength. Here we report, for the first time, µLEDs grown directly on Si with submicron lateral dimensions. The µLEDs feature ultra-stable, bright green emission with negligible quantum-confined Stark effect (QCSE). Detailed elemental mapping and numerical calculations show that the QCSE is screened by introducing polarization doping in the active region, which consists of InGaN/AlGaN QWs surrounded by an AlGaN/GaN shell with a negative Al composition gradient along the c-axis. In comparison with conventional GaN barriers, AlGaN barriers are shown to effectively compensate for the tensile strain within the active region, which significantly reduces the strain distribution and results in enhanced indium incorporation without compromising the material quality. This study provides new insights and a viable path for the design, fabrication, and integration of high-performance µLEDs on Si for a broad range of applications in on-chip optical communication and emerging augmented reality/mixed reality devices, and so on.
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Published：2022-11-01
Original Articles
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